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arXiv:0910.3699 · Physical Review A

Comparative study of BCS-BEC crossover theories above Tc : The nature of the pseudogap in ultracold atomic Fermi gases

Chih-Chun Chien, Hao Guo, Yan He, Kathryn Levin

Published Feb 24, 2010• 48 citations
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Abstract

This article presents a comparison of two finite-temperature BCS--Bose-Einstein condensation (BEC) crossover theories above the transition temperature: Nozieres--Schmitt-Rink (NSR) theory and finite-$T$ extended BCS-Leggett theory. The comparison is cast in the form of numerical studies of the behavior of the fermionic spectral function both theoretically and as constrained by (primarily) radio frequency (rf) experiments. Both theories include pair fluctuations and exhibit pseudogap effects, although the nature of this pseudogap is very different. The pseudogap in finite-$T$ extended BCS-Leggett theory is found to follow a BCS-like dispersion which, in turn, is associated with a broadened BCS-like self-energy, rather more similar to what is observed in high-temperature superconductors (albeit, for a $d$-wave case). The fermionic quasiparticle dispersion is different in NSR theory and the damping is considerably larger. We argue that the two theories are appropriate in different temperature regimes with the BCS-Leggett approach being more suitable nearer to condensation. There should, in effect, be little difference at higher $T$ as the pseudogap becomes weaker and where the simplifying approximations used in the BCS-Leggett approach break down. On the basis of momentum-integrated rf studies of unpolarized gases, it would be difficult to distinguish which theory is the better one. A full comparison for polarized gases is not possible since it is claimed that there are inconsistencies in the NSR approach (not found in the BCS-Leggett scheme). Future experiments along the lines of momentum-resolved experiments look to be very promising in distinguishing the two theories.

DOI
10.1103/physreva.81.023622

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Richard H. Squire, Norman Henry March

Abstract The pioneering works by Eagles, Leggett, and Nozieres/Schmitt‐Rink [Eagles, Phys Rev, 1969, 186, 456; Leggett, In: Modern Trends in the Theory of Condensed Matter, Springer‐Verlag: Berlin, 1980; Nozieres and Schmitt‐Rink, Low Temp Phys, 1985, 59, 980] (reviewed and augmented by Randeria [Randeria, Bose‐Einstein Condensation, Cambridge University Press, Cambridge, 1995, p 255]) emphasize that in the limits of the models studied both at T = 0 and T ≠ 0, the “cross‐over” from a BCS‐type to a BEC‐type superconductor is continuous. The BCS and BEC “end points” seem to be well‐established. However, in the intermediate region—home to fulleride and high temperature superconductors—considerable extrapolation of the models must be done as there still is no exact theory. Yet, considerable current literature is devoted to what appears to be more “singular‐type phenomena” such as quantum critical points, “stripe” formation, insulator to superconductor phase transitions, loss of validity of the Fermi liquid theory, etc. Using a connection we have made with “cold” atom fermion‐boson crossover theory [Chen, Stajic, Levin, 2005, e‐print cond‐mat/0508603], we can establish that the resonance previously discussed [Squire and March, Int J Quant Chem, 2006, 106, 3343] is a result of the crossing of the fermion band by the boson band. While the ground state appears to remain continuous, the paired energy gap becomes transformed. We discuss features of the resonance and the experimentally observed pre‐formed “BEC Cooper pair” formation, essential to the boson‐fermion resonance theory. In addition some of the various singular phenomena discussed above can be put more into perspective. Finally, in both limits the relation of characteristic lengths to the inverse Fermi momentum is strongly emphasized, as is the role of the chemical potential near the pseudogap regime. © 2007 Wiley Periodicals, Inc. Int J Quantum Chem, 2007

International Journal of Quantum Chemistry•Jan 1, 2007•5 citations
This article presents a comparison of two finite-temperature BCS--Bose-Einstein condensation (BEC) crossover theories above the transition temperature: Nozieres--Schmitt-Rink (NSR) theory and finite-TTT extended BCS-Leggett theory. The comparison is cast in the form of numerical studies of the behavior of the fermionic spectral function both theoretically and as constrained by (primarily) radio frequency (rf) experiments. Both theories include pair fluctuations and exhibit pseudogap effects, although the nature of this pseudogap is very different. The pseudogap in finite-TTT extended BCS-Leggett theory is found to follow a BCS-like dispersion which, in turn, is associated with a broadened BCS-like self-energy, rather more similar to what is observed in high-temperature superconductors (albeit, for a ddd-wave case). The fermionic quasiparticle dispersion is different in NSR theory and the damping is considerably larger. We argue that the two theories are appropriate in different temperature regimes with the BCS-Leggett approach being more suitable nearer to condensation. There should, in effect, be little difference at higher TTT as the pseudogap becomes weaker and where the simplifying approximations used in the BCS-Leggett approach break down. On the basis of momentum-integrated rf studies of unpolarized gases, it would be difficult to distinguish which theory is the better one. A full comparison for polarized gases is not possible since it is claimed that there are inconsistencies in the NSR approach (not found in the BCS-Leggett scheme). Future experiments along the lines of momentum-resolved experiments look to be very promising in distinguishing the two theories.
The pseudogap phenomenon is a hallmark of strongly interacting Fermi systems, from high-temperature superconductors to ultracold atomic gases, yet its precise origin remains debated. Here we calculate the spectral function and rf spectra of ultracold atomic gases across the BCS-BEC crossover to quantitatively investigate the pairing mechanism of the pseudogap. We advance our pairing fluctuation theory by incorporating particle-hole fluctuations, which renormalize the effective interaction in the particle-particle channel. To achieve quantitative accuracy, we employ a full numerical convolution for the pair susceptibility and self-energy, moving beyond previous analytic pseudogap approximations. This convolution approach automatically captures two critical effects: (i) the full spectral broadening of fermions due to finite pair lifetime, and (ii) the previously neglected pair-hole scattering effect, which manifests as a substantial Hartree energy. We calculate the spectral function, and use rf spectral intensity maps and energy distribution curves to determine the quasiparticle dispersion. From these, we extract the pseudogap ΔΔΔ, Hartree energy, and chemical potential, mapping their evolution across the crossover. Our results show that the pseudogap emerges continuously as the system moves from the BCS regime toward BEC. Furthermore, the pair spectral function reveals that pairs become diffusive at energies above 2ΔΔΔ, indicating that the pair lifetime is governed by virtual binding and unbinding processes. Our calculations achieve quantitative agreement with recent experiments across the BCS-BEC crossover, including at unitarity, providing strong support for a pairing-based origin of the pseudogap as described by our pairing fluctuation theory.
We investigate magnetic properties and effects of pairing fluctuations in the Bardeen-Cooper-Schrieffer--Bose-Einstein condensation (BCS-BEC) crossover regime of an ultracold Fermi gas. Recently, Liu and Hu [Europhys. Lett. 75, 364 (2006)], and Parish et al. [Nat. Phys. 3, 124 (2007)], pointed out that the strong-coupling theory developed by Nozi\`eres and Schmitt-Rink (NSR), which has been extensively used to successfully clarify various physical properties of cold Fermi gases, unphysically gives negative spin susceptibility in the BCS-BEC crossover region. The same problem also exists in the ordinary non-self-consistent TTT-matrix approximation. In this paper, we clarify that this serious problem comes from incomplete treatment in term of pseudogap phenomena originating from strong pairing fluctuations, as well as effects of spin fluctuations on the spin susceptibility. Including these two key issues, we construct an extended TTT-matrix theory which can overcome this problem. The resulting positive spin susceptibility agrees well with the recent experiment on a 6{}^{6}6Li Fermi gas done by Sanner et al. [Phys. Rev. Lett. 106, 010402 (2011)]. We also apply our theory to a polarized Fermi gas to examine the superfluid phase transition temperature Tc{T}_{\mathrm{c}}Tc​, as a function of the polarization rate. Since the spin susceptibility is an important physical quantity, especially in singlet Fermi superfluids, our results would be useful in considering how singlet pairs appear above and below Tc{T}_{\mathrm{c}}Tc​ in the BCS-BEC crossover regime of cold Fermi gases.
Due to the large neutron–neutron scattering length, dilute neutron matter resembles the unitary Fermi gas, which lies half-way in the crossover from the BCS phase of weakly coupled Cooper pairs to the Bose–Einstein condensate of dimers. We discuss crossover effects in analogy with the T-matrix theory used in the physics of ultracold atoms, which we generalize to the case of a non-separable finite-range interaction. A problem of the standard Nozières–Schmitt-Rink approach and different ways to solve it are discussed. It is shown that in the strong-coupling regime, the spectral function exhibits a pseudo-gap at temperatures above the critical temperature Tc. The effect of the correlated density on the density dependence of Tc is found to be rather weak, but a possibly important effect due to the reduced quasiparticle weight is identified.
This review is written at the time of the twentieth anniversary of the discovery of high-temperature superconductors, which nearly coincides with the important discovery of the superfluid phases of ultracold trapped fermionic atoms. We show how these two subjects have much in common. Both have been addressed from the perspective of the BCS—Bose–Einstein condensation (BEC) crossover scenario, which is designed to treat short coherence length superfluids with transition temperatures which are “high” with respect to the Fermi energy. A generalized mean field treatment of BCS–BEC crossover at general temperatures T, based on the BCS–Leggett ground state, has met with remarkable success in the fermionic atomic systems. Here we summarize this success in the context of four different cold atom experiments, all of which provide indications, direct or indirect, for the existence of a pseudogap. This scenario also provides a physical picture of the pseudogap phase in the underdoped cuprates which is a central focus of high Tc research. We summarize successful applications of BCS–BEC crossover to key experiments in high Tc systems, including the phase diagram, specific heat, and vortex core STM data, along with the Nernst effect, and exciting recent data on the superfluid density in very underdoped samples.
This article is written as a Lecture given in the 2006 Varenna Summer School on "Ultracold Fermi Gases". Here we present a review of BCS--Bose Einstein condensation (BEC) crossover theory with emphasis on finite temperature effects. We discuss the role of temperature TTT as it enters a theoretical formalism which is based on the standard BCS-Leggett ground state. We also discuss the role of temperature in the context of experiments ranging from thermometric issues to signatures of superfluidity. Particularly important to this discussion is the novel normal state associated with the crossover regime, intermediate between BCS and BEC. The experimental evidence for this unusual normal state (associated with pre-formed pairs) and its counterpart below TcT_cTc​ (associated with non-condensed pairs) is presented in the context of different experiments. We end with a discussion of finite temperature effects in spin polarized superfluids, where TTT is found to play a crucial role in both theory and experiment.
Abstract The pioneering works by Eagles, Leggett, and Nozieres/Schmitt‐Rink [Eagles, Phys Rev, 1969, 186, 456; Leggett, In: Modern Trends in the Theory of Condensed Matter, Springer‐Verlag: Berlin, 1980; Nozieres and Schmitt‐Rink, Low Temp Phys, 1985, 59, 980] (reviewed and augmented by Randeria [Randeria, Bose‐Einstein Condensation, Cambridge University Press, Cambridge, 1995, p 255]) emphasize that in the limits of the models studied both at T = 0 and T ≠ 0, the “cross‐over” from a BCS‐type to a BEC‐type superconductor is continuous. The BCS and BEC “end points” seem to be well‐established. However, in the intermediate region—home to fulleride and high temperature superconductors—considerable extrapolation of the models must be done as there still is no exact theory. Yet, considerable current literature is devoted to what appears to be more “singular‐type phenomena” such as quantum critical points, “stripe” formation, insulator to superconductor phase transitions, loss of validity of the Fermi liquid theory, etc. Using a connection we have made with “cold” atom fermion‐boson crossover theory [Chen, Stajic, Levin, 2005, e‐print cond‐mat/0508603], we can establish that the resonance previously discussed [Squire and March, Int J Quant Chem, 2006, 106, 3343] is a result of the crossing of the fermion band by the boson band. While the ground state appears to remain continuous, the paired energy gap becomes transformed. We discuss features of the resonance and the experimentally observed pre‐formed “BEC Cooper pair” formation, essential to the boson‐fermion resonance theory. In addition some of the various singular phenomena discussed above can be put more into perspective. Finally, in both limits the relation of characteristic lengths to the inverse Fermi momentum is strongly emphasized, as is the role of the chemical potential near the pseudogap regime. © 2007 Wiley Periodicals, Inc. Int J Quantum Chem, 2007