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arXiv:0910.3419

Response to comment by Tin-Lun Ho on "Itinerant Ferromagnetism in a Strongly Interacting Fermi Gas of Ultracold Atoms", Science 325, 1521 (2009)

Gyu-Boong Jo, Ye-Ryoung Lee, Choi, Jae-Hoon, Caleb A. Christensen, Tony Hyun Kim, Joseph H. Thywissen, David E. Pritchard, Wolfgang Ketterle

Published Oct 18, 2009• 2 citations
arXivHTMLPDF

Abstract

Ho claims in his comment that our experiment is direct evidence that itinerant ferromagnetism does not exist in ultracold Fermi gases. This claim is incorrect and based on an invalid estimate of relaxation times and an erroneous interpretation of the detectability of ferromagnetic domains. We point out that the experimental evidence is consistent with the existence of ferromagnetism, but further experiments are needed to distinguish a ferromagnetic ground state from a non-magnetic ground state with ferromagnetic correlations.

DOI
10.48550/arxiv.0910.3419

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Ho claims in his comment that our experiment is direct evidence that itinerant ferromagnetism does not exist in ultracold Fermi gases. This claim is incorrect and based on an invalid estimate of relaxation times and an erroneous interpretation of the detectability of ferromagnetic domains. We point out that the experimental evidence is consistent with the existence of ferromagnetism, but further experiments are needed to distinguish a ferromagnetic ground state from a non-magnetic ground state with ferromagnetic correlations.
In the 1930s, two main paradigms for the theoretical description of ferromagnetism were developed: Heisenberg ferromagnetism of localized fermions (e.g., in a lattice), and Bloch or Stoner ferromagnetism of nonlocalized fermions (i.e., in a gas), also called itinerant ferromagnetism. Despite many theoretical predictions, itinerant ferromagnetism has remained elusive in experiments. This ferromagnetic state is predicted to occur for strong repulsive interactions, corresponding to a regime that is very challenging to describe theoretically because there are multiple competing physical effects, including superfluid pairing. In this paper, we point out that the problem of itinerant ferromagnetism for atomic Fermi gases is different from that of electron gases in metals due to the short-range nature of the interatomic interactions. We also show that the standard saddle point used to describe itinerant ferromagnetism of the electron gas in metals does not apply, because in the short-range limit of this approximation the Pauli exclusion principle is violated. As a remedy, we introduce a modified interaction pseudopotential for ultracold gases which includes both local (Hartree) and nonlocal (Fock) terms while preserving the Pauli exclusion principle in the short-range regime. Furthermore, we demonstrate the usefulness of this method to study the existence and stability of itinerant ferromagnetism in ultracold atomic gases. Lastly, we obtain the critical temperature for the ferromagnetic transition as a function of the opposite-spin interaction strength and find a rather good agreement with recent experimental results.
Whether a spin-1/2 Fermi gas will become ferromagnetic as the strength of repulsive interaction increases is a long-standing controversial issue. Recently this problem has been studied experimentally by Jo et al. [Science 325, 1521 (2009)] in which the authors claim a ferromagnetic transition is observed. This work is to point out the results of this experiment cannot distinguish whether the system is in a ferromagnetic state or in a nonmagnetic but strongly short-range correlated state. A conclusive experimental demonstration of ferromagnetism relies on the observation of ferromagnetic domains.
We address the possible occurrence of ultracold atom ferromagnetism by evaluating the free energy of a spin polarized Fermi gas to second order in its interaction parameter. We find that Hartree-Fock theory underestimates the tendency toward ferromagnetism, predict that the ferromagnetic transition is first order at low temperatures, and point out that the spin coherence time of gases prepared in a ferromagnetic state is strongly enhanced as the transition is approached. We relate our results to recent experiments.
Ultracold atomic Fermi gases close to Feshbach resonances represent the ideal platform to study strongly correlated fermionic states [1]. Up to now, most of the experimental efforts have been dedicated to the study of the famous BEC-BCS crossover, i.e. the transition from a Bose-Einstein condensate of tightly bound molecules to a BCS superfluid of long-range fermion pairs. However, such fermionic gases are the ideal environment to explore also the effects of strong, repulsive interactions. The interest in studying repulsive Fermi gases is manifold, since many phase transitions are driven by the strong repulsion between electrons in solids. One notable example is represented by the onset of itinerant ferromagnetism in metals, as envisioned by Stoner almost ninety years ago.
Recent experiments [Jo, Science 325, 1521 (2009)] have presented evidence of ferromagnetic correlations in a two-component ultracold Fermi gas with strong repulsive interactions. Motivated by these experiments we consider spin drag, i.e., frictional drag due to scattering of particles with opposite spin, in such systems. We show that when the ferromagnetic state is approached from the normal side, the spin drag relaxation rate is strongly enhanced near the critical point. We also determine the temperature dependence of the spin diffusion constant. In a trapped gas the spin drag relaxation rate determines the damping of the spin dipole mode, which therefore provides a precursor signal of the ferromagnetic phase transition that may be used to experimentally determine the proximity to the ferromagnetic phase.
We theoretically investigate the itinerant ferromagnetic transition of a spherically trapped ultracold Fermi gas with spin imbalance under strongly repulsive interatomic interactions. Our study is based on a self-consistent solution of the Hartree-Fock mean-field equations beyond the widely used local-density approximation. We demonstrate that, while the local-density approximation holds in the paramagnetic phase, after the ferromagnetic transition it leads to a quantitative discrepancy in various thermodynamic quantities even with large atom numbers. We determine the position of the phase transition by monitoring the shape change of the free-energy curve with increasing the polarization at various interaction strengths.