We present a theory of spin waves in a non-condensed gas of spin-1 bosons: providing both analytic calculations of the linear theory, and full numerical simulations of the nonlinear response. We highlight the role of spin-dependent contact interactions in the dynamics of a thermal gas. Although these interactions are small compared to the thermal energy, they set the scale for low energy long wavelength spin waves. In particular, we find that the polar state of Rb-87 is unstable to collisional mixing of magnetic sublevels even in the normal state. We augment our analytic calculations by providing full numerical simulations of a trapped gas, explicitly demonstrating this instability. Further we show that for strong enough anti-ferromagnetic interactions, the polar gas is unstable. Finally we explore coherent population dynamics in a collisionless transversely polarized gas.
We present a theory of spin waves in a non-condensed gas of spin-1 bosons: providing both analytic calculations of the linear theory, and full numerical simulations of the nonlinear response. We highlight the role of spin-dependent contact interactions in the dynamics of a thermal gas. Although these interactions are small compared to the thermal energy, they set the scale for low energy long wavelength spin waves. In particular, we find that the polar state of Rb-87 is unstable to collisional mixing of magnetic sublevels even in the normal state. We augment our analytic calculations by providing full numerical simulations of a trapped gas, explicitly demonstrating this instability. Further we show that for strong enough anti-ferromagnetic interactions, the polar gas is unstable. Finally we explore coherent population dynamics in a collisionless transversely polarized gas.
We present a theory of spin waves in a noncondensed gas of spin-1 bosons and provide both analytic calculations of the linear theory and full numerical simulations of the nonlinear response. We highlight the role of spin-dependent contact interactions in the dynamics of a thermal gas. Although these interactions are small compared to the thermal energy, they set the scale for low-energy, long-wavelength spin waves. In particular, we find that the polar state of {sup 87}Rb is unstable to collisional mixing of magnetic sublevels even in the normal state. We augment our analytic calculations by providing full numerical simulations of a trapped gas, explicitly demonstrating this instability. Further, we show that for strong antiferromagnetic interactions, the polar gas is unstable. Finally, we explore coherent population dynamics in a collisionless transversely polarized gas.
We present a theory of spin waves in a noncondensed gas of spin-1 bosons and provide both analytic calculations of the linear theory and full numerical simulations of the nonlinear response. We highlight the role of spin-dependent contact interactions in the dynamics of a thermal gas. Although these interactions are small compared to the thermal energy, they set the scale for low-energy, long-wavelength spin waves. In particular, we find that the polar state of 87Rb is unstable to collisional mixing of magnetic sublevels even in the normal state. We augment our analytic calculations by providing full numerical simulations of a trapped gas, explicitly demonstrating this instability. Further, we show that for strong antiferromagnetic interactions, the polar gas is unstable. Finally, we explore coherent population dynamics in a collisionless transversely polarized gas.
We consider a trapped ultra-cold gas of (non-condensed) bosons with two internal states (described by a pseudo spin) and study the stability of a longitudinal pseudo spin polarization gradient. For this purpose, we numerically solve a kinetic equation corresponding to a situation close to an experiment at JILA. It shows the presence of Castaing's instability of transverse spin polarization fluctuations at long wavelengths. This phenomenon could be used to create spontaneous transverse spin waves.
Bose-Einstein condensation (BEC) is a phenomenon in which identical bosons occupy the same quantum state below a certain critical temperature. A hallmark of BEC is the coherence between particles every particle shares the same quantum wavefunction and phase. This coherence has been demonstrated for the external (motional) degrees of freedom of the atomic condensates by interfering two condensates. In this thesis, the coherence is shown to extend to the internal spin degrees of freedom of a spin-1 Bose gas evidenced by the observed coherent and reversible spin-changing collisions. The observed coherent dynamics are analogous to Josephson oscillations in weakly connected superconductors and represent a type of matter-wave four-wave mixing. Control of the coherent evolution of the system using magnetic fields is also demonstrated. The studies on spinor condensates begin by creating spinor condensates directly using all-optical approaches that were first developed in our laboratory. All-optical formation of Bose-Einstein condensates (BEC) in 1D optical lattice and single focus trap geometries are developed and presented. These techniques offer considerable flexibility and speed compared to magnetic trap approaches, and the trapping potential can be essentially spin-independent and are ideally suited for studying spinor condensates. Using condensates with well-defined initial non-equilibrium spin configuration, spin mixing of F = 1 and F = 2 spinor condensates of rubidium-87 atoms confined in an optical trap is observed. The equilibrium spin configuration in the F = 1 manifold confirms that 87Rb is ferromagnetic. The coherent spinor dynamics are demonstrated by initiating spin mixing deterministically with a non-stationary spin population configuration. Finally, the interplay between the coherent spin mixing and spatial dynamics in spin-1 condensates with ferromagnetic interactions is investigated.
The study of out-of-equilibrium dynamics in ultra-cold gases is a new and exciting field, driven largely by the recent experimental advances in controlling and imaging cold clouds. The experimental and theoretical work thus far has been somewhat exploratory and largely numerical in nature, as the very paradigms for thinking about these systems are not well established. In this thesis I consider several different scenarios of ultra-cold bosonic and fermionic gases driven out of equilibrium and study their properties. In Chapter 1, I provide an overview of the phenomenology of ultra-cold gases, highlighting the timescales governing these systems and how the experimentalist can tune them. I discuss how cold gases can be cooled and trapped and discuss the basic physics behind optical lattices. I also discuss experimental probes of these gases, in particular the new high resolution imaging techniques developed recently at Chicago, Munich and Harvard. In Chapter 2, I discuss an early experiment (circa. 2008) which observed long lived spin dynamics in a thermal spin-1/2 Fermi gas. This experiment is an nice illustration of interesting physics resulting from the separation of timescales between spin and collisional dynamics. In my opinion, it is an excellent example of why cold gases are naturally suited to studying non-equilibrium dynamics. I simulate the experiment numerically using a collisionless Boltzmann equation and explain the observed spin dynamics both qualitatively and quantitively. In Chapter 3, I continue the discussion of spin waves in thermal gases by extending previous works on spin-1/2 gases to spin-1 Bose gases. In contrast to Chapter 2, the bulk of the work in this Chapter is analytic in nature. In particular, I find a spin wave instability in the thermal spin-1 Bose gas, which is the high temperature analog of the polar to ferromagnetic transition in a spin-1 Bose Einstein condensate. In Chapter 3, I turn my attention to bosonic systems and briefly review the the Bogoliubov mean-field theory. I calculate the momentum distribution and density-density correlation function of an interacting Bose gas within the Bogoliubov framework. Then I consider bosons in an optical lattice, and introduce the Bose Hubbard model. I calculate the mean-field phase diagram of the Bose Hubbard model and then consider fluctuations about the mean field, and derive the excitation spectrum of the lattice gas in the superfluid and insulating regimes. In Chapter 4, I ask what we learn by studying the dynamics of correlation functions following a sudden change in the interactions in a superfluid. Using the Bogoliubov theory developed in Chapter 3, I will show how the underlying excitation spectrum influences the long and short time behavior of the correlation functions. By considering a lattice dispersion, I study the analogous problem in a weak optical lattice and discuss how the lattice dispersion leads to additional features in the correlation functions. I will also discuss the timescale governing the revival of the condensate fraction in a quantum depleted gas. In Chapter 5, I derive equations of motion governing the dynamics of one and two body correlation functions in the single-band Bose Hubbard model, applicable to bosons in deep lattices. I then consider a simple quench from a Mott insulating initial state to a weakly interacting final state and produce analytic expressions describing the dynamics of correlations following such a quench. I discuss the timescale for the development of long range order following such a quench. I study the problem of chapter 4 using an equations of motion approach. This approach complements the Bogoliubov approach of Chapter 4. First, I derive exact expressions for a quench to a non-interacting state. I then consider how interactions redistribute quasi-momentum to first order in perturbation theory in different dimensions. In Chapter 6, I calculate the relevant timescales for local and global dynamics in trapped lattice Bose gases, a work done in collaboration with Dr. Kaden R. A Hazzard. Using a time-dependent Gutzwiller mean-field theory, I show that the timescale for local equilibration in these systems is fast in experimental terms. I then show that due to the spatial inhomogeneities inherent to cold gases, achieving global equilibrium can be quite complicated, sometimes taking longer than the lifetime of the experiment, an issue of practical importance to current day experiments. I continue this discussion in Chapter 7 which is a collaborative work with experimentalists David McKay and Prof. Brian DeMarco from the University of Toronto and the University of Illinois, Urbana Champaign. Using experimental and numerical methods, we show that the rapid timescales for local dynamics in interacting systems invalidates a frequently used cold atom technique for mapping out the momentum distribution of atoms in an optical lattice.
We present experimental observations of coherent spin-population oscillations in a cold thermal, Bose gas of spin-1 23Na atoms. The population oscillations in a multi-spatial-mode thermal gas have the same behavior as those observed in a single-spatial-mode antiferromagnetic spinor Bose-Einstein condensate. We demonstrate this by showing that the two situations are described by the same dynamical equations, with a factor of 2 change in the spin-dependent interaction coefficient, which results from the change to particles with distinguishable momentum states in the thermal gas. We compare this theory to the measured spin population evolution after times up to a few hundreds of ms, finding quantitative agreement with the amplitude and period. We also measure the damping time of the oscillations as a function of magnetic field.