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arXiv:0909.5396 · Physical Review A

Degenerate Landau-Zener model: Analytical solution

G. S. Vasilev, Svetoslav S. Ivanov, Nikolay V. Vitanov

Published Jan 23, 2007• 44 citations
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Abstract

The exact analytical solution of the degenerate Landau-Zener model, wherein two bands of degenerate energies cross in time, is presented. The solution is derived by using the Morris-Shore transformation, which reduces the fully coupled system to a set of independent nondegenerate two-state systems and a set of decoupled states. Due to the divergence of the phase of the off-diagonal element of the propagator in the original Landau-Zener model, not all transition probabilities exist for infinite time duration. In general, apart from some special cases, only the transition probabilities between states within the same degenerate set exist, but not between states of different sets. An illustration is presented for the transition between the magnetic sublevels of two atomic levels with total angular momenta $J=2$ and 1.

DOI
10.1103/physreva.75.013417

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The exact analytical solution of the degenerate Landau-Zener model, wherein two bands of degenerate energies cross in time, is presented. The solution is derived by using the Morris-Shore transformation, which reduces the fully coupled system to a set of independent nondegenerate two-state systems and a set of decoupled states. Due to the divergence of the phase of the off-diagonal element of the propagator in the original Landau-Zener model, not all transition probabilities exist for infinite time duration. In general, apart from some special cases, only the transition probabilities between states within the same degenerate set exist, but not between states of different sets. An illustration is presented for the transition between the magnetic sublevels of two atomic levels with total angular momenta J=2J=2J=2 and 1.
The Morris-Shore (MS) transformation is a powerful tool for decomposition of the dynamics of multistate quantum systems to a set of two-state systems and uncoupled single states. It assumes two sets of states wherein any state in the first set can be coupled to any state in the second set, but the states within each set are not coupled between themselves. Another important condition is the degeneracy of the states in each set, although all couplings between the states from different sets can be detuned from resonance by the same detuning. The degeneracy condition limits the application of the MS transformation in various physically interesting situations, e.g., in the presence of electric and/or magnetic fields or light shifts, which lift the degeneracy in each set of states, e.g., when these sets comprise the magnetic sublevels of levels with nonzero angular momentum. This paper extends the MS transformation to such situations, in which the states in each of the two sets are nondegenerate. To this end, we develop an alternative way for the derivation of Morris-Shore transformation, which can be applied to nondegenerate sets of states. We present an approximated eigenvalue approach, by which, in the limit of small detunings from degeneracy, we are able to generate an effective Hamiltonian that is dynamically equivalent to the nondegenerate Hamiltonian. The effective Hamiltonian can be mapped to the Morris-Shore basis with a two-step similarity transformation. After the derivation of the general framework, we demonstrate the application of this technique to the popular $\mathrm{\ensuremath{\Lambda}}$ three-state system, and the four-state tripod, double-$\mathrm{\ensuremath{\Lambda}}$, and diamond systems. In all of these systems, our formalism allows us to reduce their quantum dynamics to simpler two-state systems even in the presence of various detunings, e.g., generated by external fields of frequency drifts.
Two aspects of the classic two-level Landau-Zener (LZ) problem are considered. First, we address the LZ problem when one or both levels decay, i.e., ${\ensuremath{\varepsilon}}_{j}(t)\ensuremath{\rightarrow}{\ensuremath{\varepsilon}}_{j}(t)\ensuremath{-}i{\ensuremath{\Gamma}}_{j}/2$. We find that if the system evolves from an initial time $\ensuremath{-}T$ to a final time +T+T+T such that $|{\ensuremath{\varepsilon}}_{1}(\ifmmode\pm\else\textpm\fi{}T)\ensuremath{-}{\ensuremath{\varepsilon}}_{2}(\ifmmode\pm\else\textpm\fi{}T)|$ is not too large, the LZ survival probability of a state $|j\ensuremath{\rangle}$ can increase with increasing decay rate of the other state $|i\ensuremath{\ne}j\ensuremath{\rangle}$. This surprising result occurs because the decay results in crossing of the two eigenvalues of the instantaneous non-Hermitian Hamiltonian. On the other hand, if $|{\ensuremath{\varepsilon}}_{1}(\ifmmode\pm\else\textpm\fi{}T)\ensuremath{-}{\ensuremath{\varepsilon}}_{2}(\ifmmode\pm\else\textpm\fi{}T)|\ensuremath{\rightarrow}\ensuremath{\infty}$ as $T\ensuremath{\rightarrow}\ensuremath{\infty}$, the probability is independent of the decay rate. These results are based on analytic solutions of the time-dependent Schr\"odinger equations for two cases: (a) the energy levels depend linearly on time, and (b) the energy levels are bounded and of the form ${\ensuremath{\varepsilon}}_{1,2}(t)=\ifmmode\pm\else\textpm\fi{}\ensuremath{\varepsilon}tanh(t/\mathcal{T})$. Second, we study LZ transitions affected by dephasing by formulating the Landau-Zener problem with noise in terms of a Schr\"odinger-Langevin stochastic coupled set of differential equations. The LZ survival probability then becomes a random variable whose probability distribution is shown to behave very differently for long and short dephasing times. We also discuss the combined effects of decay and dephasing on the LZ probability.
We formulate a perturbative approach for studying a class of multilevel time-dependent quantum systems with constant off-diagonal couplings and diabatic energies being odd functions of time. Applying this approach to a general multistate Landau-Zener (MLZ) model with all diabatic levels crossing at one point (named the one-crossing MLZ model), we derive analytical formulas of all its transition probabilities up to fourth order in the couplings. For one-crossing MLZ models it is difficult to obtain such analytical results by other kinds of approximation methods; thus, these perturbative results can serve as reliable benchmarks for future studies of any one-crossing MLZ models that have not been exactly solved.
The Schrodinger equation i Psi =(A+Bt) Psi with constant Hermitian matrices A and B is studied. In the form where B is diagonalized, this equation is a generalization of the Landau-Zener problem to an arbitrary number of crossing energy levels. An approach-the independent crossing approximation-leading to a partial understanding of the general case in terms of the two-level problem is introduced. It is found that certain S-matrix elements (and thus the corresponding transition probabilities) for the general problem are exactly given by formulae of unexpected simplicity, suggesting that some kind of general analytic solution might exist. The full S-matrix is calculated for a solvable special case of the problem. The solution of another special case, previously discovered for systems with three states, is generalized to any number of states. The asymptotic behaviour of the system is discussed in general and given explicitly to lowest order in 1/t.
We present an asymptotic approach towards the standard Landau-Zener problem based on two linearly independent elementary waves of constant amplitude but time-dependent phase. The two contributions to this phase are quadratic and logarithmic in time and result from the linear chirp of the energies and the lowest order correction in the coupling between the two levels in the long-time limit. Indeed, our solutions subjected to initial conditions at a large but finite time in the past, are valid for large negative and large positive times. Due to their asymptotic nature they are not valid in the neighborhood of the moment when the levels cross. However, as the starting point of the dynamics moves further into the past, the time interval of the break-down of our asymptotic solutions shrinks and vanishes in the limit of the infinite past which corresponds to the standard Landau-Zener situation. Our approach explains not only every feature of the exact solution but yields deeper insights into the origin of the effects. In particular, it (i) brings to light the subtleties involved in the asymptotic limit leading to the standard expressions for the Landau-Zener transition amplitudes, (ii) identifies the logarithmic phase as the origin of the exponential transition probability amplitude, and (iii) reveals the structure of the lowest order corrections to the Landau-Zener result when the starting point is not in the infinite past.
During the adiabatic time evolution levels crossing violates the adiabaticity and makes transitions between levels possible. Conventionally only two energy levels cross simultaneously. The transition probabilities for this case were found by Landau and Zener. However, the multilevel crossing happens systematically rather than occasionally if the Hamiltonian possesses a special symmetry. The simplest physical realization of the multilevel crossing are the Zeeman multiplet in a varying magnetic field and an electron in one-dimensional chain driven by the time-dependent electric field. We present asymptotics of the transition amplitudes for these kinds of the multilevel crossing. They are based on an exact solution for a model n-state, time-dependent Schrödinger equation.