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arXiv:0909.3825 · Physical Review Letters

Clock Shifts of Optical Transitions in Ultracold Atomic Gases

Zhenhua Yu, C. J. Pethick

Published Jan 4, 2010• 30 citations
arXivHTMLPDF

Abstract

We calculate the shift, due to interatomic interactions, of an optical transition in an atomic Fermi gas trapped in an optical lattice, as in recent experiments of Campbell et al. [Science 324, 360 (2009)]. Using a pseudospin formalism to describe the density matrix of atoms, we derive a Bloch equation which incorporates both spatial inhomogeneity of the probe laser field and interatomic interactions. Expressions are given for the frequency shift as a function of pulse duration, detuning of the probe laser, and the spatial dependence of the electric field of the probe beam. In the low temperature semiclassical regime, we find that the magnitude of the shift is proportional to the temperature.

DOI
10.1103/physrevlett.104.010801

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We calculate the shift, due to interatomic interactions, of an optical transition in an atomic Fermi gas trapped in an optical lattice, as in recent experiments of Campbell et al. [Science 324, 360 (2009)]. Using a pseudospin formalism to describe the density matrix of atoms, we derive a Bloch equation which incorporates both spatial inhomogeneity of the probe laser field and interatomic interactions. Expressions are given for the frequency shift as a function of pulse duration, detuning of the probe laser, and the spatial dependence of the electric field of the probe beam. In the low temperature semiclassical regime, we find that the magnitude of the shift is proportional to the temperature.
A recent realization of three-dimensional optical lattice clocks circumvents short-range collisional clock shifts which have been the bottle neck towards higher precision; the long-range electronic dipole-dipole interaction between the atoms becomes the primary source of clock shift due to interatomic interactions. We study the Rabi spectroscopy of three-dimensional optical lattice clocks with unity filling. From the Lindblad equation governing the time evolution of the density matrix of the atoms, we derive the Bloch equations in the presence of the external Rabi driving laser field, and solve the equations approximately to the first order of the coupling strength of the dipole-dipole interaction between the atoms. We find that the clock shift equals the product of the coupling strength, a factor determined by the parameters of the Rabi pulse, and another factor depending on the configuration of the three-dimensional optical lattice. Our result on the clock shift within the Rabi spectroscopy can be checked by measurements in a future experiment.
At ultracold temperatures, the Pauli exclusion principle suppresses collisions between identical fermions. This has motivated the development of atomic clocks with fermionic isotopes. However, by probing an optical clock transition with thousands of lattice-confined, ultracold fermionic strontium atoms, we observed density-dependent collisional frequency shifts. These collision effects were measured systematically and are supported by a theoretical description attributing them to inhomogeneities in the probe excitation process that render the atoms distinguishable. This work also yields insights for zeroing the clock density shift.
An important new development in the field of ultracold atomic gases is the study of the properties of these gases in a so-called optical lattice. An optical lattice is a periodic trapping potential for the atoms that is formed by the interference pattern of a few laser beams. A reason for the interest in these systems is that the effects of the interatomic interactions can be strongly enhanced. More specifically, it has been shown in a beautiful experiment by Greiner et al. in 2002 that by loading a Bose-Einstein condensate into an optical lattice it is possible for the system to undergo a quantum phase transition to a new quantum phase of matter, the so-called Mott insulator phase. Within this Mott insulator phase each lattice site is occupied by exactly one atom. This makes the Mott insulator phase especially well suited for applications in the field of quantum computation and quantum information processing. We have theoretically investigated the above mentioned quantum phase transition and our formalism allows for a description of the Mott insulator phase at nonzero temperatures. Another important experimental development in the field of ultracold atomic gases is the use of Feshbach resonances to control the interatomic interactions. Such a resonance occurs whenever two colliding atoms form a long-lived molecule for some time. The crucial point of a Feshbach resonance is that the above mentioned molecule has a magnetic moment that is not equal to twice the magnetic moment of the atom. As a consequence the energy difference between the two atoms and the molecule and hence the interactions between the atoms can be controlled by using an external magnetic field. By combining these two techniques, i.e, by trapping ultracold atomic gases in an optical lattice and by tuning a magnetic field near a Feshbach resonance there can be a new quantum phase transition between two superfluid phases. We gave derived the the theory for the description of these Feshbach resonances in optical lattices and applied it to various systems. To be a bit more precise, if we tune the external magnetic field such that the energy difference between a molecule and two atoms is sufficiently negative, then the gas consists of a Bose-Einstein condensate of molecules. In contrast, if the energy difference is large enough and positive we have a gas that consists primarily of a Bose-Einstein condensate of atoms. It turns out that these two limits are separated by an Ising-like quantum phase transition. By using atomic Bose gases near a Feshbach resonance detailed experimental studies which test the theoretical predictions of the statistical and dynamical properties of these quantum phase transitions can be made.
We develop the theory of propagation of laser wave in a gas of two-level atoms (with an optical transition frequency ω0\omega^{}_0ω0​) under the condition of inhomogeneous Doppler broadening, considering the self-consistent solution of the Maxwell-Bloch equations in the mean-field approximation and for one-atomic density matrix. The nonlinear effects in the atomic density nnn, caused by the free motion of atoms, are found. These effects distort the lineshape (shift, asymmetry, broadening), but are not associated with atom-atom interaction. Moreover, in the case nk0−3<1nk^{-3}_0<1nk0−3​<1 (where k0=ω0/ck^{}_0=\omega^{}_0/ck0​=ω0​/c) and temperatures T≳300T\gtrsim 300T≳300~K, these quasi-collective effects exceed the well-known influence of the dipole-dipole interatomic interaction (e.g., Lorentz-Lorenz shift) by more than one order of magnitude. It was also found that for some area of parameters, the frequency interval appears, within which the non-trivial self-consistent solution of the Maxwell-Bloch equations is absent at all. Thus, the physical picture of collective effects in a gas medium should be substantially revised.
We investigate the influence of atomic motion on precision Rabi spectroscopy of ultracold fermionic atoms confined in a deep one-dimensional optical lattice. We analyze the spectral components of longitudinal sideband spectra and present a model to extract information about the transverse motion and sample temperature from their structure. Rabi spectroscopy of the clock transition itself is also influenced by atomic motion in the weakly confined transverse directions of the optical lattice. By deriving Rabi flopping and Rabi line shapes of the carrier transition, we obtain a model to quantify trap-state-dependent excitation inhomogeneities. The inhomogeneously excited ultracold fermions become distinguishable, which allows sss-wave collisions. We derive a detailed model of this process and explain observed density shift data in terms of a dynamic mean-field shift of the clock transition.
We excite spin waves with spatially inhomogeneous Ramsey pulses and study the resulting frequency shifts of a chip-scale atomic clock of trapped 87Rb. The density-dependent frequency shifts of the hyperfine transition simulate the s-wave collisional frequency shifts of fermions, including those of optical lattice clocks. As the spin polarizations oscillate in the trap, the frequency shift reverses and it depends on the area of the second Ramsey pulse, exhibiting a predicted beyond mean-field frequency shift. Numerical and analytic models illustrate these observed behaviors.