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arXiv:0907.3904 · Physical Review Letters

Localization of Metal-Induced Gap States at the Metal-Insulator Interface: Origin of Flux Noise in SQUIDs and Superconducting Qubits

Sangkook Choi, D. H. Lee, Steven G. Louie, John L. Clarke

Published Nov 3, 2009• 101 citations
arXivHTMLPDF

Abstract

The origin of magnetic flux noise in superconducting quantum interference devices with a power spectrum scaling as 1/f (f is frequency) has been a puzzle for over 20 years. This noise limits the decoherence time of superconducting qubits. A consensus has emerged that the noise arises from fluctuating spins of localized electrons with an areal density of 5x10(17) m(-2). We show that, in the presence of potential disorder at the metal-insulator interface, some of the metal-induced gap states become localized and produce local moments. A modest level of disorder yields the observed areal density.

DOI
10.1103/physrevlett.103.197001

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For over three decades, the presence of magnetic flux noise with a power spectral density scaling roughly as $S_Phi(f) propto 1/f^alpha$, where $alpha lesssim 1$, has been known to limit the low-frequency performance of dc superconducting quantum interference devices (SQUIDs). In recent years, experiments indicate that this same noise persists to frequencies up to 1~GHz and is a dominant source of dephasing in flux-sensitive superconducting quantum bits (qubits). Thus, the reduction of flux noise presents a major hurdle towards the successful realization of scalable quantum computers that are based on flux-based qubits. In this thesis, we present experimental measurements, theoretical analyses, and numerical simulations that support a more detailed understanding of both the microscopic and macroscopic properties of flux noise.Our experimental work begins with flux noise measurements of a large number of SQUIDs in the temperature range from 0.1~K to 4~K. We report on measurements of ten SQUIDs with systematically varied geometries and show that $alpha$ increases as the temperature is lowered; in so doing, each spectrum pivots about a nearly constant frequency. The mean square flux noise, inferred by integrating the power spectra, grows rapidly with temperature and at a given temperature is approximately independent of the outer dimension of a given SQUID washer. We show that these results are incompatible with a model based on the random reversal of independent, spins that are located at the surface of the SQUID washer.In the course of our flux noise measurements, we became aware of a spurious contribution to low-frequency critical current noise in Josephson junctions---normally attributed to charge trapping in the barrier---arising from temperature instabilities inherent in cryogenic systems. These temperature fluctuations modify the critical current via its temperature dependence. By computing cross-correlations between measured temperature and critical current noise in Al-AlOx-Al junctions, we show that, despite excellent temperature stability, temperature fluctuations induce observable critical current fluctuations. Particularly, because $1/f$ critical current noise has decreased with improved fabrication techniques in recent years, it is important to understand and eliminate this additional noise source.Next, we introduce a numerical method of calculating the mean square flux noise $Phisq$ from independently fluctuating spins on the surface of thin-film loops of arbitrary geometry. By reciprocity, $Phisq$ is proportional to $langleBbf(rbf)^2rangle$, where $Bbf(rbf)$ is the magnetic field generated by a circulating current around the loop and $rbf$ varies over the loop surface. By discretizing the loop nonuniformly, we efficiently and accurately compute the current distribution and resulting magnetic field, which may vary rapidly across the loop. We use this method to compute $Phisq$ in a number of scenarios in which we systematically vary physical parameters of the loop. We compare our simulations to an earlier analytic result predicting that $Phisq propto R/W$ in the limit where the loop radius $R$ is much greater than the linewidth $W$. We further show that the previously neglected contribution of edge spins to $Phisq$ is significant---even dominant---in narrow-linewidth loops.To calculate theoretical dephasing rates in qubits, we consider flux noise with a spectral density $S_Phi(f) = A^2/(f/1~hbox{Hz})^alpha$, where $A$ is of the order of 1~$muPhi_0 , hbox{Hz}^{-1/2}$ and $0.6 leq alpha leq 1.2$; $Phi_{0}$ is the flux quantum. For a qubit with an energy level splitting linearly coupled to the applied flux, our calculations of the dependence of the pure dephasing time $tau_phi$ of Ramsey and echo pulse sequences on $alpha$ for fixed $A$ show that $tau_phi$ decreases rapidly as $alpha$ is reduced. We find that $tau_phi$ is relatively insensitive to the noise bandwidth, $f_1 leq f leq f_2$, for all $alpha$ provided the ultraviolet cutoff frequency $f_2 > 1/tau_phi$. We calculate the ratio $tau_{phi,E} / tau_{phi,R}$ of the echo ($E$) and Ramsey ($R$) sequences, and the dependence of the decay function on $alpha$ and $f_2$. We investigate the case in which $S_Phi(f_0)$ is fixed at the ``pivot frequency'' $f_0 neq 1$~Hz while $alpha$ is varied, and find that the choice of $f_0$ can greatly influence the sensitivity of $tau_{phi,E}$ and $tau_{phi,R}$ to the value of $alpha$.Finally, we conclude with a brief review of our principal results and conclusions. We also comment on promising avenues of future research.

•Jan 1, 2013•0 citations
The origin of magnetic flux noise in superconducting quantum interference devices with a power spectrum scaling as 1/f (f is frequency) has been a puzzle for over 20 years. This noise limits the decoherence time of superconducting qubits. A consensus has emerged that the noise arises from fluctuating spins of localized electrons with an areal density of 5x10(17) m(-2). We show that, in the presence of potential disorder at the metal-insulator interface, some of the metal-induced gap states become localized and produce local moments. A modest level of disorder yields the observed areal density.
In the present study we investigate the selected local aspects of the metal-induced gap states (MIGSs) at the disordered metal-insulator interface, that were previously proposed to produce magnetic moments responsible for the magnetic flux noise in some of the superconducting qubit modalities. Our analysis attempts to supplement the available studies and provide new theoretical contribution toward their validation. In particular, we explicitly discuss the behavior of the MIGSs in the momentum space as a function of the onsite energy deviation, that mimics random potential disorder at the interface in the local approximation. It is found, that when the difference between the characteristic electronic potentials in the insulator increases, the corresponding MIGSs become more localized. This effect is associated with the increasing degree of the potential disorder that was earlier observed to produce highly localized MIGSs in the superconducting qubits. At the same time, the presented findings show that the disorder-induced localization of the MIGSs can be related directly to the decay characteristics of these states as well as to the bulk electronic properties of the insulator. As a result, our study reinforces plausibility of the previous corresponding investigations on the origin of the flux noise, but also allows to draw future directions toward their better verification.
Flux noise in superconducting quantum interference devices (SQUIDs) is produced by spins on the surface of metals. We have modeled these with Monte Carlo simulations of 2D and 3D Ising spin glasses that produce magnetization noise SMconsistent with flux noise. The frequency dependence of the magnetization noise goes as 1/fαwhere the exponent a varies slightly with temperature. In 3D the noise power spectrum in the order parameter q goes as 1/ f1.4at Tc. The low frequency noise in both q and the magnetization is a maximum at Tc.
We propose a model for 1/f flux noise in superconducting devices (f is frequency). The noise is generated by the magnetic moments of electrons in defect states which they occupy for a wide distribution of times before escaping. A trapped electron occupies one of the two Kramers-degenerate ground states, between which the transition rate is negligible at low temperature. As a result, the magnetic moment orientation is locked. Simulations of the noise produced by randomly oriented defects with a density of 5x10(17) m(-2) yield 1/f noise magnitudes in good agreement with experiments.
The magnetic flux noise caused by surface spin fluctuations in superconducting quantum interference devices (SQUIDs) limits their development. In this work, we report that different adsorbents such as H, O 2, NO, and NO 2 that adsorb on the surfaces of Mg-based and Pb-based SQUIDs, respectively, producing large local magnetic moments ranging from 0.7–1.6 μ B, with energy barriers for thermal spin fluctuation as low as 10–30 mK. Moreover, we observe that the presence of H atoms on the surface of MgO can cause the coadsorption of other molecules, which generates additional spin sources. Monte Carlo simulations of the weakly coupled spin on a two-dimensional square lattice produce a low-frequency flux noise spectrum. We suggest eliminating the surface magnetism by coating the surface with monolayer indium phosphide or protecting the surface from other molecules by nonmagnetic preoccupants with a larger adsorption energy. The work provides important physical insights and feasible strategies for reducing magnetic noise sources in superconducting circuits.
Superconducting Quantum Interference Devices (SQUIDs) are currently being used as flux qubits and read-out detectors in a variety of solid-state quantum computer architectures. The main limitation of SQUID qubits is that they have a coherence time of the order of 10 us, due to the presence of intrinsic flux noise that is not yet fully understood. The origin of flux noise is currently believed to be related to spin impurities present in the materials and interfaces that form the device. Here we present a novel numerical method that enables calculations of the flux produced by spin impurities even when they are located quite close to the SQUID wire. We show that the SQUID will be particularly sensitive to spins located at its wire edges, generating flux shifts of up to 4 nano flux quanta, much higher than previous calculations based on the software package FastHenry. This shows that spin impurities in a particular region along the wire's surface play a much more important role in producing flux noise than other spin impurities located elsewhere in the device.
For over three decades, the presence of magnetic flux noise with a power spectral density scaling roughly as SPhi(f)propto1/falphaS_Phi(f) propto 1/f^alphaSP​hi(f)propto1/falpha, where alphalesssim1alpha lesssim 1alphalesssim1, has been known to limit the low-frequency performance of dc superconducting quantum interference devices (SQUIDs). In recent years, experiments indicate that this same noise persists to frequencies up to 1~GHz and is a dominant source of dephasing in flux-sensitive superconducting quantum bits (qubits). Thus, the reduction of flux noise presents a major hurdle towards the successful realization of scalable quantum computers that are based on flux-based qubits. In this thesis, we present experimental measurements, theoretical analyses, and numerical simulations that support a more detailed understanding of both the microscopic and macroscopic properties of flux noise.Our experimental work begins with flux noise measurements of a large number of SQUIDs in the temperature range from 0.1~K to 4~K. We report on measurements of ten SQUIDs with systematically varied geometries and show that alphaalphaalpha increases as the temperature is lowered; in so doing, each spectrum pivots about a nearly constant frequency. The mean square flux noise, inferred by integrating the power spectra, grows rapidly with temperature and at a given temperature is approximately independent of the outer dimension of a given SQUID washer. We show that these results are incompatible with a model based on the random reversal of independent, spins that are located at the surface of the SQUID washer.In the course of our flux noise measurements, we became aware of a spurious contribution to low-frequency critical current noise in Josephson junctions---normally attributed to charge trapping in the barrier---arising from temperature instabilities inherent in cryogenic systems. These temperature fluctuations modify the critical current via its temperature dependence. By computing cross-correlations between measured temperature and critical current noise in Al-AlOx-Al junctions, we show that, despite excellent temperature stability, temperature fluctuations induce observable critical current fluctuations. Particularly, because 1/f1/f1/f critical current noise has decreased with improved fabrication techniques in recent years, it is important to understand and eliminate this additional noise source.Next, we introduce a numerical method of calculating the mean square flux noise PhisqPhisqPhisq from independently fluctuating spins on the surface of thin-film loops of arbitrary geometry. By reciprocity, PhisqPhisqPhisq is proportional to langleBbf(rbf)2ranglelangleBbf(rbf)^2ranglelangleBbf(rbf)2rangle, where Bbf(rbf)Bbf(rbf)Bbf(rbf) is the magnetic field generated by a circulating current around the loop and rbfrbfrbf varies over the loop surface. By discretizing the loop nonuniformly, we efficiently and accurately compute the current distribution and resulting magnetic field, which may vary rapidly across the loop. We use this method to compute PhisqPhisqPhisq in a number of scenarios in which we systematically vary physical parameters of the loop. We compare our simulations to an earlier analytic result predicting that PhisqproptoR/WPhisq propto R/WPhisqproptoR/W in the limit where the loop radius RRR is much greater than the linewidth WWW. We further show that the previously neglected contribution of edge spins to PhisqPhisqPhisq is significant---even dominant---in narrow-linewidth loops.To calculate theoretical dephasing rates in qubits, we consider flux noise with a spectral density SPhi(f)=A2/(f/1 hboxHz)alphaS_Phi(f) = A^2/(f/1~hbox{Hz})^alphaSP​hi(f)=A2/(f/1 hboxHz)alpha, where AAA is of the order of 1~muPhi0,hboxHz−1/2muPhi_0 , hbox{Hz}^{-1/2}muPhi0​,hboxHz−1/2 and 0.6leqalphaleq1.20.6 leq alpha leq 1.20.6leqalphaleq1.2; Phi0Phi_{0}Phi0​ is the flux quantum. For a qubit with an energy level splitting linearly coupled to the applied flux, our calculations of the dependence of the pure dephasing time tauphitau_phitaup​hi of Ramsey and echo pulse sequences on alphaalphaalpha for fixed AAA show that tauphitau_phitaup​hi decreases rapidly as alphaalphaalpha is reduced. We find that tauphitau_phitaup​hi is relatively insensitive to the noise bandwidth, f1leqfleqf2f_1 leq f leq f_2f1​leqfleqf2​, for all alphaalphaalpha provided the ultraviolet cutoff frequency f2>1/tauphif_2 > 1/tau_phif2​>1/taup​hi. We calculate the ratio tauphi,E/tauphi,Rtau_{phi,E} / tau_{phi,R}tauphi,E​/tauphi,R​ of the echo (EEE) and Ramsey (RRR) sequences, and the dependence of the decay function on alphaalphaalpha and f2f_2f2​. We investigate the case in which SPhi(f0)S_Phi(f_0)SP​hi(f0​) is fixed at the ``pivot frequency'' f0neq1f_0 neq 1f0​neq1~Hz while alphaalphaalpha is varied, and find that the choice of f0f_0f0​ can greatly influence the sensitivity of tauphi,Etau_{phi,E}tauphi,E​ and tauphi,Rtau_{phi,R}tauphi,R​ to the value of alphaalphaalpha.Finally, we conclude with a brief review of our principal results and conclusions. We also comment on promising avenues of future research.