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arXiv:0907.2884

Decoherence via induced dipole collisions in an ultracold gas

Anthony Gorges, Mathew Hamilton, Jacob Roberts

Published Jul 16, 2009• 0 citations
arXivHTMLPDF

Abstract

We have studied the effects of loading $^{87}$Rb into a far off resonant trap (FORT) in the presence of an ultracold cloud of $^{85}$Rb. The presence of the $^{85}$Rb resulted in a marked decrease of the $^{87}$Rb load rate. This decrease is consistent with a decrease in the laser cooling efficiency needed for effective loading. While many dynamics which disrupt loading efficency arise when cooling in a dense cloud of atoms (reabsorption, adverse optical pumping, etc.), the large detuning between the transitions of $^{85}$Rb and $^{87}$Rb should isolate the isotopes from these effects. For our optical molasses conditions we calculate that our cooling efficiencies require induced ground-state coherences. We present data and estimates which are consistent with heteronuclear long-ranged induced dipole-dipole collisions disrupting these ground state coherences, leading to a loss of optical trap loading efficiency.

DOI
10.48550/arxiv.0907.2884

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We have studied the effects of loading 87^{87}87Rb into a far off resonant trap (FORT) in the presence of an ultracold cloud of 85^{85}85Rb. The presence of the 85^{85}85Rb resulted in a marked decrease of the 87^{87}87Rb load rate. This decrease is consistent with a decrease in the laser cooling efficiency needed for effective loading. While many dynamics which disrupt loading efficency arise when cooling in a dense cloud of atoms (reabsorption, adverse optical pumping, etc.), the large detuning between the transitions of 85^{85}85Rb and 87^{87}87Rb should isolate the isotopes from these effects. For our optical molasses conditions we calculate that our cooling efficiencies require induced ground-state coherences. We present data and estimates which are consistent with heteronuclear long-ranged induced dipole-dipole collisions disrupting these ground state coherences, leading to a loss of optical trap loading efficiency.
Examination of loading the isotopes 85^{85}85Rb and 87^{87}87Rb simultaneously into a shallow far-off-resonance trap (FORT) has revealed an unexpected decrease in maximum atom number loaded as compared to loading either isotope alone. The simultaneous loading of the FORT will be affected by additional homonuclear and heteronuclear light-assisted collisional losses. However, these losses are measured and found to be insufficient to explain the observed drop in total number of atoms loaded into the FORT. We find that our observations are consistent with a decrease in loading rate caused by inter-isotope disruptions of the efficient laser cooling required to load atoms into the optical trap.
Measurements of the temperature dependence of trap loss collisions of laser-cooled rubidium atoms are presented. A significant suppression of the rate of collisions between ground- and excited-state atoms is observed for temperatures below $\\sim$70 mu\\mumuK. In such inelastic collisions, the atomic excitation takes place at long range and must survive against spontaneous decay to short range. Our results are consistent with recent predictions for the low temperature suppression of these collisions due to reduced survival of atomic excitation at low collision velocities.^ We report on measurements of trap loss collisions between ultracold Rb atoms which are confined in a magneto-optical trap. Both isotopes sp85\\sp{85}sp85Rb and sp87\\sp{87}sp87Rb have been studied over wide range of trap laser intensities and detunings. The trap loss collision rates exhibit variations over 3 orders of magnitude. We observe significant differences between the isotopes. At large detunings the ability of the trap to recapture products of the hyperfine-changing collisions is significantly diminished. This finding is supported by our numerical simulations of the recapture process. The trap loss rates due to collisions with room temperature background gas have also been measured.^ Using laser light tuned to a repulsive molecular potential, we have been able to suppress inelastic ground-state hyperfine changing collisions between ultracold sp87\\sp{87}sp87Rb atoms. Adiabatic excitation to the repulsive curve alters the atomic trajectories and prevents the atoms from approaching close enough for the hyperfine change to occur. Experimental results show suppressions up to $\\sim$50% and are in reasonable agreement with a simple Landau-Zener model.^ Finally, we have observed a significant cooperative effect in ultracold trap loss collisions induced by two separate lasers. One laser, tuned close to the atomic resonance, excites the atom pair to an attractive potential at long range. The resulting acceleration and deflection give rise to an enhancement in the collisional flux of ground-state atoms reaching short range, as probed by a second laser. Enhancements up to a factor of $\\sim$3 have been observed. ^
We have studied heteronuclear and homonuclear excited-state--ground-state collisions by loading both 85Rb^{85}\mathrm{Rb}85Rb and 87Rb^{87}\mathrm{Rb}87Rb into a far off resonant trap (FORT). Because of the relatively weak confinement of the FORT, we expect the hyperfine structure of the different isotopes to play a crucial role in the collision rates. This dependence on hyperfine structure allows us to measure collisions associated with long-range interatomic potentials of different structures, such as long and short ranged; or such as purely attractive, purely repulsive, or mixed attractive and repulsive. We observe significantly different loss rates for different excited-state potentials. Additionally, we observe that some collisional channels' loss rates are saturated at our operating intensities (15mW∕cm2)(15\phantom{\rule{0.3em}{0ex}}\mathrm{mW}∕{\mathrm{cm}}^{2})(15mW∕cm2). These losses are important limitations in loading dual isotope optical traps.
This dissertation reports on the design, construction, and investigation of a pulsed optical dipole force trap which uses laser light to confine ultracold rubidium (Rb) atoms. Because the laser frequency is detuned far from the atomic resonance frequency, the optical dipole force trap is also called a "far-off-resonance trap" (FORT). The use of pulsed laser light to create an optical trap may find application in expanding the number of atomic species which can be confined. The experiments reported here are principally aimed, however, at understanding the physics of pulsed FORT dynamics in anticipation of using the free electron laser (FEL) at Jefferson Lab (Jlab) to construct a FORT. The Jlab FEL will provide a tunable, high power laser light source enabling the realization of spatially large and/or energetically deep traps which are not presently accessible with table-top laser sources. Here, a mode-locked Nd:YAG laser is used as a pulsed laser source. Since the conservative optical dipole force trap does not cool Rb atoms, ultracold atoms must be loaded into the FORT. The optical dipole force trap is formed at the focus of a Gaussian, 1.06 μm Nd:YAG laser beam which is located at the center of a high vacuum chamber and superimposed onto the center of a pre-cooled Rb atom cloud that has been previously accumulated in a magneto-optic trap (MOT). The performance of the pulsed FORT is compared to a continuous wave mode (cw) FORT which is built using the same laser beam; the operation of the two kinds of FORTs can be switched easily without disturbing the experimental alignment. The dependencies of FORT loading efficiency to FORT and MOT parameters such as FORT laser power, loading time, storage/holding time, detuning of the primary MOT laser frequency, and repump laser intensity are investigated. There are about 1.5×107 ultracold rubidium atoms in the MOT. At 7 Watts FORT laser power, about 8% of the atoms are loaded successfully into the cw FORT and about 5% into the pulsed FORT under similar, but not identical, conditions. In most respects both the cw and pulsed FORTs show comparable behavior. The behavior of both FORTs depends strongly on FORT laser power. As expected, at higher power, more atoms can be loaded into the FORT. Both FORTs also depend on the loading time and holding time.
We have examined loading of 85Rb^{85}\mathrm{Rb}85Rb atoms into a shallow far-off-resonance trap (FORT) from an optical molasses stage following a magneto-optical trap (MOT) stage and compared it to loading from a MOT stage only. Substantially more atoms could be loaded into the FORT using an optical molasses. To determine why this was the case, we measured the rate of atoms loaded into the FORT and the losses from the FORT during both loading processes over a range of detunings and hyperfine pump powers. We found that the losses induced during MOT loading were essentially the same as the losses induced during molasses loading and decreased with increased red detuning; however, we found that the differences in load rate caused an optical molasses to optimize at a greater detuning, improving the number of atoms we could trap by a factor of 2 over that of optimal loading from a MOT.
We report on measurements of trap-loss collisions between ultracold Rb atoms that are confined in a magneto-optical trap. Both isotopes, 85Rb{}^{85}\mathrm{Rb}85Rb and 87Rb,{}^{87}\mathrm{Rb},87Rb, have been studied over a wide range of trap laser intensities and detunings. The trap-loss collisional rate constant exhibits variations over three orders of magnitude. At low intensities and/or large detunings, the trap loss is dominated by ground-state hyperfine-changing collisions, while at high intensities and small detunings, collisions involving excited atoms are more important. We see significant differences between the isotopes in both regimes. At large detunings, the ability of the trap to recapture products of a hyperfine-changing collision is significantly diminished. This finding is supported by our numerical simulations of the recapture process. The trap loss rates due to collisions with room-temperature background gas have also been measured. A surprisingly large increase in this rate is seen when the confining power of the trap is reduced.