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arXiv:0906.1438 · Optics Express

Atomic Šolc filter: multi-resonant photoemission via periodic poling of atom-cavity coupling constant

Hyun-Gue Hong, Wontaek Seo, Moonjoo Lee, Younghoon Song, Young-Tak Chough, Jai-Hyung Lee, Kyungwon An

Published Aug 17, 2009• 10 citations
arXivHTMLPDF

Abstract

This paper describes a novel atom-cavity interaction induced by periodically poled atom-cavity coupling constant which leads to multiple narrow photoemission bands for an initially inverted two-level atom under the strong coupling condition. The emission bandpass narrowing has a close analogy with the folded Solc filter in the context of quasi-phase matching by periodic poling. We present a closed form solution of the emission probability at the end of interaction and deduce the multiple phase matching condition for this system which is programmable by the interaction time. The Bloch sphere analysis provides a clear understanding of the underlying atomic dynamics associated with the multiple resonances in the semiclassical limit. Furthermore, we show that this interaction can be applied to generation of nonclassical fields with sub-Poisson photon statistics.

DOI
10.1364/oe.17.015455

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This paper describes a novel atom-cavity interaction induced by periodically poled atom-cavity coupling constant which leads to multiple narrow photoemission bands for an initially inverted two-level atom under the strong coupling condition. The emission bandpass narrowing has a close analogy with the folded Solc filter in the context of quasi-phase matching by periodic poling. We present a closed form solution of the emission probability at the end of interaction and deduce the multiple phase matching condition for this system which is programmable by the interaction time. The Bloch sphere analysis provides a clear understanding of the underlying atomic dynamics associated with the multiple resonances in the semiclassical limit. Furthermore, we show that this interaction can be applied to generation of nonclassical fields with sub-Poisson photon statistics.
We report experimental realization of a rudimentary atomic \ifmmode \check{S}\else \v{S}\fi{}olc filter, recently proposed by Hong et al. [Opt. Express 17, 15455 (2009)]. It is realized by employing a bipolar atom-cavity coupling constant in the cavity-QED microlaser operating with a TEM10{}_{10}10​ mode in a strong coupling regime. The polarity flip in the coupling constant dramatically changes the photoemission probability of a two-level atom relative to unipolar coupling, resulting in multiple narrow emission bands in the detuning curve of the microlaser mean photon number. The observed resonance curves are explained well by a two-step, three-dimensional, geodesic-like motion of the Bloch vector in the semiclassical limit.
The radiative properties of atoms inside an optical cavity can be dramatically changed with respect to those in free space. In the strong-coupling limit, the reversible dipole interaction between an atom and the cavity field dominates the irreversible decay resulting from spontaneous emission and cavity damping. In this limit the atom and field can no longer be regarded as separate quantities but instead form a composite dynamic system. To enhance the dipole coupling constant and increase the photon storage time, our experiments are performed with a small cavity 1 mm long, with a finesse of 8 × 104. On average, 0.4 photons are sufficient to saturate the resonance transition at 852 nm for the cesium atoms used, while the cooperativity parameter for a single atom is 2. Optical bistability is studied in this system over the range 3 < N < 65 atoms inside the cavity, with the semiclassical theory predicting bistability for N > 5. We report observations of manifestly quantum effects in this regime, including photon antibunching and sub-Poissonian photon statistics, with the magnitude of these nonclassical effects observed to be largely independent of the number of intracavity atoms.
We investigate properties of a two-level atom coupled to a single cavity mode, and driven by a strong, in general off-resonance, external field. The cavity field is tuned to resonance with a Mollow sideband. We show that the steady-state atomic population may be highly (nearly totally) inverted, a phenomenon forbidden in semiclassical theory, and that a strong enhancement of the resonance fluorescence results. This system is suggested as an alternative approach to create the atomic inversion necessary for laser or maser generation without using additional atomic levels. We also investigate properties of the cavity field, derive an analytical expression for the photon number distribution in the good cavity or strong-coupling limit, and discuss the conditions under which this system acts as a single-atom dressed-state laser.
We show that a simple nonperturbative two-level model of an atom driven by a very strong periodic field, results in a rich picture of very high harmonic generation and related phenomena. It reproduces experimentally observed plateau, yields for the first time simple analytic formulas for the plateau cutoff frequency, critical driving intensity, and saturation, and predicts intensity-induced multi-resonances. One of the most fascinating phenomenon discovered recently in nonlinear interaction of light with atoms and ions, is very high-order (up to 135) odd harmonic generation (HHG) by intense (∼ 1013 W/cm2 and higher) optical laser radiation in rare gasses and some ions [1], The spectra of generated harmonics drasticly deviate from the perturbation theory predictions [2], In particular, intensity of harmonics, falling monotonically with their orders only up to a certain point, levels off forming a so-called “plateau", and falls monotonically again beyond it. Generally, harmonte generation depends on phase-matching conditions and nonlinear response of individual atoms. It has recently become clear however [3,4] that the major features of HHG, in particular the plateau, result mainly from general properties of atomic nonlinear response. The most direct and apparently successful way so far to approach the problem theoretically has been numerical simulation of the Schrödinger [2,5-7] (including an empiric rule [6]) for many-electron atoms using Hartry-Slater approximation. This approach requires, however, tremendous amount of calculations and involves many processes, making it difficult to gain simple insights. An interesting simplified model [8] based on 3-D delta-potential with a single (ground) level [9] produces results in integration form. The idea of retaining a single energy scale (ionization energy) brings one close to an even simpler system: a two-level model atom. A two-level model of HHG [10], however, due to various complications introduced into it, failed to generate simple results, whereas an analytic solution [11] holds for a virtually degenerate two-level model only (see below) which is unapplicable to the experimental conditions [1-4,7,9]; besides, no relaxation was considered in [10,11].
We study the interaction of a small number of resonant two-level atoms in a cavity coupled to a quasi-continuum of cavity modes. During the interaction we induce externally a phase step to one of the atoms. As a result an enhancement in the photon emission to the field is observed. The phase step is obtained by a pulse which causes the atom to be off-resonance for a short time interval. The effect is strongest in cases where the number of atoms is small. The enhancement is not restricted to a small parameter range but should be observable in many systems even though the φ phase shift gives the best enhancement.
The Rabi Hamiltonian, describing the interaction between a two-level atomic system and a single-cavity mode of the electromagnetic field, is one of the fundamental models in quantum optics. The model becomes exactly solvable by considering an atom without permanent dipole moments, whose excitation energy is quasiresonant with the cavity photon energy, and by neglecting the nonresonant (counter-rotating) terms. In this case, after including the decay of either the atom or the cavity mode to a continuum, one can derive the well-known phenomenology of quasiresonant transitions, including the fluorescence triplets. In this work we consider the most general Rabi model, incorporating the effects of permanent atomic electric dipole moments. Based on a perturbative analysis, we compare the intensities of emission lines induced by rotating terms, counter-rotating terms, and parity-symmetry-breaking terms in order to identify the parameter regimes in which these different contributions play a significant role. The analysis reveals that the emission strength related to the existence of permanent dipoles may surpass the one due to the counter-rotating interaction terms but is usually much weaker than the emission due to the main, resonant coupling. This ratio can be modified in systems with a reduced dimensionality or by engineering the energy spectral density of the continuum.