We investigate the spatially dependent relative phase evolution of an elongated two-component Bose-Einstein condensate. The pseudospin-$\frac{1}{2}$ system is comprised of the $|F=1,{m}_{F}=\ensuremath{-}1⟩$ and $|F=2,{m}_{F}=+1⟩$ hyperfine ground states of $^{87}\text{R}\text{b}$, which we magnetically trap and interrogate with radio-frequency and microwave fields. We probe the relative phase evolution with Ramsey interferometry and observe a temporal decay of the interferometric contrast well described by a mean-field formalism. Inhomogeneity of the collective relative phase dominates the loss of interferometric contrast, rather than decoherence or phase diffusion. We demonstrate a technique to simultaneously image each state, yielding subpercent variations in the measured relative number while preserving the spatial mode of each component. In addition, we propose a spatially sensitive interferometric technique to image the relative phase.
We investigate the spatially dependent relative phase evolution of an elongated two-component Bose-Einstein condensate. The pseudospin-21 system is comprised of the ∣F=1,mF=\ensuremath−1⟩ and ∣F=2,mF=+1⟩ hyperfine ground states of 87Rb, which we magnetically trap and interrogate with radio-frequency and microwave fields. We probe the relative phase evolution with Ramsey interferometry and observe a temporal decay of the interferometric contrast well described by a mean-field formalism. Inhomogeneity of the collective relative phase dominates the loss of interferometric contrast, rather than decoherence or phase diffusion. We demonstrate a technique to simultaneously image each state, yielding subpercent variations in the measured relative number while preserving the spatial mode of each component. In addition, we propose a spatially sensitive interferometric technique to image the relative phase.
In the years following the first Bose-Einstein condensation of dilute atomic gases in 1995, several experiments demonstrated many fundamental properties of two-component BEC. Subsequent to these pioneering experiments, almost a decade passed with little experimental activity, relative to investigations of single-component condensates. In somewhat of a renaissance, the initial observations of two-component BEC have been revisited in recent years, consolidating and clarifying results of the early works, and illuminating new and surprising behaviour of these rich quantum fluids. This thesis presents new experimental results on the relative phase evolution of two-component Bose-Einstein condensates (BECs). We approach our study of this system from the dual perspective of binary superfluidity and trapped atom interferometry. We observe nonequilibrium dynamics of the condensate that are deeply connected to the physics of interpenetrating superfluids. These dynamics have consequences for interferometers whose two paths are different internal spin states of the condensate atoms. Using trapped condensates for precision measurement draws upon the benefits of confined atom interferometry - long interrogation times, precise position control to measure near-field potentials - in addition to the unique coherence properties of BECs. Precision measurementwith trapped particles, however, is obstructed by the inherent inhomogeneities associated with the confinement itself. Spatial variation of the external potentials and atomic density can give rise to dephasing during the free evolution and imperfect splitting and recombination of the interferometric paths. In this thesis, we consider the dephasing of the two-componentmean field order parameter, which tends to diminish the interference signal attained with the condensate. The promise of fuhs for atom interferometry lies within using nonclassical many body states to reduce the fundamental noise limit imposed upon measuring the projection of atomic pseudospin. Before the many body quantum properties of two-component condensates can be used to their full potential, the ideal classical limit must be achieved and investigated. As in optical interferometry, the classical ideality of an interference measurement is contingent upon control of the spatialmodes - thematter wave fields, or single particle wave functions. Whilst much attention is currently focused on preparing nonclassical many body states for entanglement and squeezing of the condensate pseudospin, this thesis focuses on the ancillary yet important issue of spatial inhomogeneity of the condensate mean field. Reversal of the spatially inhomogeneous mean field evolution is demonstrated, employing the techniques of nuclear magnetic resonance. A new method is demonstrated to probe pseudospin -1/2 condensates involving microwave adiabatic passage. The technique permits simultaneous, spatially resolved absorption imaging of the spatial mode of each component. Controlled manipulation of the components into Zeeman states with different magnetic moments allows spatial separation using a Stern-Gerlach separation technique, providing a spatially resolved projection of the local condensate pseudospin from a single absorption image. We propose an interferometric technique which employs this imaging method to directly image the relative phase. The miscibility of the two components depends on the relative magnitude of the interactions between various collision partners. The boundary of this miscibility is found to be less pronounced than expected from the commonly applied results of homogeneous super-fluids.The effects of kinetic energy are shown to be significant at the threshold of miscibility, leading to a breakdown in the Thomas-Fermi approximation. Magnetic dipole transitions amongst alkali ground states are often used to prepare, manipulate, and interrogate pseudospin -1/2 condensates. We present a thorough investigation of the two-photonmagnetic dipole transitions between the |F = 1,mF = -1〉 and |F = 2,mF = +1〉 states, and the |F = 1,mF = +1〉 and |F = 2,mF = -1〉 states of 87Rb. Taking into account all 8 Zeeman levels of the electronic ground state reveals markedly different radiative shifts and effects beyond the rotating wave approximation, compared to the three-level formalism commonly used for these transitions.This has implications for Ramsey interferometry using the two-photon magnetic dipole transitions. The unchartered experimental territory offered by two-component condensates is vast, and future directions, supplementary to the work in this thesis, are elucidated.
We experimentally and theoretically study phase coherence in two-component Bose-Einstein condensates of ^{87}Rb atoms on an atom chip. Using Ramsey interferometry we determine the temporal decay of coherence between the |F=1,m_{F}=-1⟩ and |F=2,m_{F}=+1⟩ hyperfine ground states. We observe that the coherence is limited by random collisional phase shifts due to the stochastic nature of atom loss. The mechanism is confirmed quantitatively by a quantum trajectory method based on a master equation which takes into account collisional interactions, atom number fluctuations, and losses in the system. This decoherence process can be slowed down by reducing the density of the condensate. Our findings are relevant for experiments on quantum metrology and many-particle entanglement with Bose-Einstein condensates and the development of chip-based atomic clocks.
Ultracold atoms and Bose-Einstein condensates represent a burgeoning and ever exciting area of research which has produced numerous breakthroughs in the last 15 years. Ultracold atoms at nano-Kelvin temperatures, isolated in atom traps from the hot, room temperature environment, exhibit ultimate quantum properties and can serve as pure samples for testing quantum mechanics and performing precision measurements. The research described in this thesis investigates, both theoretically and experimentally, the coherence and dynamical evolution of a two-component Bose-Einstein condensate (BEC). The studies are performed on the |1 › ≡ F = 1,mF = −1 › and |2 › ≡ |F = 2,mF = +1 › hyperfine ground states of a 87Rb BEC trapped on an atom chip. Conventional understanding has been that the fringe contrast in interferometric experiments on a BEC is limited by the mean-field dephasing due to strong interatomic interactions which lead to inhomogeneous collisional shifts. We have discovered using Ramsey interferometry a mean-field driven self-rephasing effect in a trapped twocomponent BEC. When combined with a spin-echo technique, we find that the selfrephasing leads to a coherence time of 2.8 s, the longest ever recorded for an interacting BEC. Secondly, we have developed a new technique based on periodic collective oscillations for precision measurements of the interspecies and intraspecies scattering lengths and derived an analytic mean-field theory for the phase and density dynamics in the twocomponent BEC. This technique has been applied to the measurements of the scattering lengths for the two components, |1i and |2i, in 87Rb with a precision of 0.016%. Additionally, the two-body loss coefficients for these states have been measured. Thirdly, we have developed and applied a new, interferometric method for calibrating the detection system, in order to determine the total atom number precisely for Ramsey interferometric measurements. The calibration coefficient is found to be in a good agreement with that obtained using a conventional calibration technique based on the critical BEC temperature. Finally, we have detected predicted RF-induced Feshbach resonances by monitoring changes in the two-body loss coefficients in the two-component BEC. Conventional Feshbach resonances have been used in many works to tune the s-wave interactions; however, there is no achievable magnetic Feshbach resonance for magnetically trappable states of 87Rb. The RF-induced resonances which we have detected can provide a way to tune the scattering lengths which is important for interferometry and entanglement experiments. The positions of the resonances may provide useful information for predicting the atomic scattering properties of 87Rb.
Polarization-dependent phase-contrast imaging is used to resolve the spatial magnetization profile of an optically trapped ultracold gas. This probe is applied to Larmor precession of degenerate and nondegenerate spin-1 87Rb gases. Transverse magnetization of the Bose-Einstein condensate persists for the condensate lifetime, with a spatial response to magnetic field inhomogeneities consistent with a mean-field model of interactions. In comparison, the magnetization of the non-condensed gas decoheres rapidly. Rotational symmetry implies that the Larmor frequency of a spinor condensate be density independent, and thus suitable for precise magnetometry with high spatial resolution.
We study the time-evolution of an optically trapped spinor Bose-Einstein condensate under the influence of a dominating magnetic bias field in the z-direction, and a perpendicular smaller field that couples the spinor states. We show that if the bias field depends quadratically on time, the relative phases of the spinor components affect the populations of the final state. This allows one to measure the differences in the time-evolution of the relative phases, thereby realizing a multi-arm interferometer in a spinor Bose-Einstein condensate.
Summary form only given. Following the first observations of Bose-Einstein condensation (BEC) in dilute atomic gases, there has been considerable interest in multiple condensates as a system of interpenetrating quantum fluids. Most recently in our time averaged orbiting potential (TOP) trap, we have created coherent superpositions of condensates in the |F=1, m/sub F/=-1> and |F=2, m/sub F/=1> hyperfine ground states of Rubidium-87. A coupling field connects the states of this two level system. Following evaporative cooling to BEC in the |1,-1> state, a short coupling pulse allows us to transfer an arbitrary proportion of the atoms into the upper |2,1> state. In the first experiments with two component condensates, we have determined the ratio of the intraspecies scattering lengths for the two hyperfine states mentioned above; we have transferred half of the atoms to the upper |2,1> state to investigate the dynamics of the two components separation; and we have found that, in the regions where they overlap, the two condensates retain a well defined phase even after the damping of their relative center of mass motion. To further our studies of double condensates, we have implemented a new, state-sensitive form of nondestructive imaging, a technique first pioneered by Zernike in the field of microscopy, and more recently adapted to the imaging of condensates by the group at MIT. We exploit the state sensitivity of the technique to distinguish the two spin states inside the trap (or, more accurately, to measure their relative density across the cloud).