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arXiv:0902.3055 · Physical Review B

Quantum many-body theory of qubit decoherence in a finite-size spin bath. II. Ensemble dynamics

Wen Yang, Ren‐Bao Liu

Published Mar 26, 2009• 103 citations
arXivHTMLPDF

Abstract

Decoherence of a center spin or qubit in a spin bath is essentially determined by the many-body bath evolution. The bath dynamics can start either from a pure state or, more generally, from a statistical ensemble. In the preceding article [W. Yang and R. B. Liu, Phys. Rev. B 78, 085315 (2008)], we developed the cluster-correlation expansion (CCE) theory for the so-called single-sample bath dynamics initiated from a factorizable pure state. Here we present the ensemble CCE theory, which is based on similar ideas of the single-sample CCE. The bath evolution is factorized into the product of all possible cluster correlations, each of which accounts for the authentic (nonfactorizable) collective excitation of a group of bath spins and for the finite-time evolution in the qubit decoherence problem. Convergent results can be obtained by truncating the ensemble CCE by keeping cluster correlations up to a certain size. A difference between the ensemble CCE and single-sample CCE is that the mean-field treatment in the latter formalism of the diagonal part of the spin-spin interaction in the bath is not possible in the former case. The ensemble CCE can be applied to nonfactorizable initial states. The ensemble CCE is checked against the exact solution of an $XY$ spin bath model. For small spin baths, it is shown that single-sample dynamics is sensitive to the sampling of the initial state from a thermal ensemble and hence very different from the ensemble average.

DOI
10.1103/physrevb.79.115320

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Decoherence of a center spin or qubit in a spin bath is essentially determined by the many-body bath evolution. The bath dynamics can start either from a pure state or, more generally, from a statistical ensemble. In the preceding article [W. Yang and R. B. Liu, Phys. Rev. B 78, 085315 (2008)], we developed the cluster-correlation expansion (CCE) theory for the so-called single-sample bath dynamics initiated from a factorizable pure state. Here we present the ensemble CCE theory, which is based on similar ideas of the single-sample CCE. The bath evolution is factorized into the product of all possible cluster correlations, each of which accounts for the authentic (nonfactorizable) collective excitation of a group of bath spins and for the finite-time evolution in the qubit decoherence problem. Convergent results can be obtained by truncating the ensemble CCE by keeping cluster correlations up to a certain size. A difference between the ensemble CCE and single-sample CCE is that the mean-field treatment in the latter formalism of the diagonal part of the spin-spin interaction in the bath is not possible in the former case. The ensemble CCE can be applied to nonfactorizable initial states. The ensemble CCE is checked against the exact solution of an XYXYXY spin bath model. For small spin baths, it is shown that single-sample dynamics is sensitive to the sampling of the initial state from a thermal ensemble and hence very different from the ensemble average.
Decoherence of a center spin or qubit in a spin bath is essentially determined by the many-body bath evolution. We develop a cluster-correlation expansion (CCE) theory for the spin-bath dynamics relevant to the qubit decoherence problem. A cluster-correlation term is recursively defined as the evolution of a group of bath spins divided by the cluster correlations of all the subgroups. This correlation accounts for the authentic (nonfactorizable) collective excitations within a given group. The bath propagator is the product of all possible cluster correlation terms. For a finite-time evolution as in the qubit decoherence problem, a convergent result can be obtained by truncating the expansion up to a certain cluster size. The two-spin cluster truncation of the CCE corresponds to the pair-correlation approximation developed previously [W. Yao et al., Phys. Rev. B 74, 195301 (2006)]. In terms of the standard linked cluster expansion, a cluster-correlation term is the infinite summation of all the connected diagrams with all and only the spins in the group flip-flopped, and thus the expansion is exact whenever convergence occurs. When the individual contribution of each higher-order correlation term to the decoherence is small (while all the terms combined in product could still contribute substantially), as the usual case for relatively large baths, where the decoherence could complete well within the bath spin flip-flop time, the CCE coincides with the cluster expansion [W. M. Witzel and S. Das Sarma, Phys. Rev. B 74, 035322 (2006)]. For small baths, however, the qubit decoherence may not complete within the bath spin flip-flop time scale and thus individual higher-order cluster correlations could become significant. In such cases, only the CCE converges to the exact coherent dynamics of multispin clusters. We check the accuracy of the CCE in an exactly solvable spin-chain model.
We develop a cluster‐correlation expansion theory for the many‐body dynamics of a finite‐size spin bath in a time scale relevant to the decoherence of a center spin or qubit embedded in the bath. By introducing the cluster correlation as the evolution of a group of bath spins divided by the correlations of all the subgroups, the propagator of the whole bath is factorized into the product of all possible cluster correlations. Each cluster‐correlation term accounts for the authentic (non‐factorizable) collective excitations within that group. Convergent results can be obtained by truncating the cluster‐correlation expansion up to a certain cluster size, as verified in an exactly solvable spin‐chain model.
The clock transitions (CTs) or optimal working points (OWPs) of central qubits have long coherence times because their frequency fluctuations vanish in the linear order of external field noise (such as Overhauser fields from nuclear spin baths). Therefore, CTs (or OWPs) are useful for quantum technologies. Also, the quadratic dependence of frequencies on noises makes the CT decoherence an interesting physics problem. Thus we are motivated to study the decoherence of CTs. We consider noise from spin baths, which is one of the most relevant mechanisms of qubit decoherence. Various quantum many-body methods have been developed to study the decoherence of a central spin in spin baths. In particular, the cluster-correlation expansion (CCE) systematically accounts for the many-body correlations that cause the central spin decoherence. However, the CCE cannot be straightforwardly applied to CTs in spin baths, for the expansion may fail to converge due to the effective long-range interactions resulting from the quadratic term of the noise (e.g., the second-order interaction mediated by hyperfine interactions for a nuclear spin bath). In this work, we develop a modified CCE method to tackle this class of decoherence problems. By diagonalizing the central spin Hamiltonian for each bath eigenstate of the hyperfine interaction, we find that the effects of long-range interactions are absorbed as fluctuations of central spin eigenenergies in the form of single-spin correlations. We apply the method to two important systems, namely, nitrogen vacancy center electron spins in near zero magnetic field and the singlet-triplet transition of two electrons in a double quantum dot. The numerical simulation shows that the modified CCE converges rapidly for the CTs. This modified cluster correlation expansion provides a nonperturbative approach to treating the central spin mediated long-range interactions in central spin decoherence problems.
Decoherence of electron spins in nanoscale systems is important to quantum technologies such as quantum information processing and magnetometry. It is also an ideal model problem for studying the crossover between quantum and classical phenomena. At low temperatures or in light-element materials where the spin-orbit coupling is weak, the phonon scattering in nanostructures is less important and the fluctuations of nuclear spins become the dominant decoherence mechanism for electron spins. Since the 1950s, semi-classical noise theories have been developed for understanding electron spin decoherence. In spin-based solid-state quantum technologies, the relevant systems are in the nanometer scale and nuclear spin baths are quantum objects which require a quantum description. Recently, quantum pictures have been established to understand the decoherence and quantum many-body theories have been developed to quantitatively describe this phenomenon. Anomalous quantum effects have been predicted and some have been experimentally confirmed. A systematically truncated cluster-correlation expansion theory has been developed to account for the many-body correlations in nanoscale nuclear spin baths that are built up during electron spin decoherence. The theory has successfully predicted and explained a number of experimental results in a wide range of physical systems. In this review, we will cover this recent progress. The limitations of the present quantum many-body theories and possible directions for future development will also be discussed.
We solve the time-dependent Schrodinger equation for the combination of a spin system interacting with a spin bath environment. In particular, we focus on the time development of the reduced density matrix of the spin system. Under normal circumstances we show that the environment drives the reduced density matrix to a fully decoherent state, and furthermore the diagonal elements of the reduced density matrix approach those expected for the system in the canonical ensemble. We show one exception to the normal case is if the spin system cannot exchange energy with the spin bath. Our demonstration does not rely on time-averaging of observables nor does it assume that the coupling between system and bath is weak. Our findings show that the canonical ensemble is a state that may result from pure quantum dynamics, suggesting that quantum mechanics may be regarded as the foundation of quantum statistical mechanics.
We study the quantum dynamics of a single qubit coupled to a bath of interacting spins as a model for decoherence in solid state quantum memories. The spin bath is described by the Lipkin-Meshkov-Glick model and the bath spins are subjected to a transverse magnetic field. We investigate the qubit interacting via either an Ising- or an XY-type coupling term to subsets of bath spins of differing size. The large degree of symmetry of the bath allows us to find parameter regimes where the initial qubit state is revived at well-defined times after the qubit preparation. These times may become independent of the bath size for large baths and thus enable faithful qubit storage even in the presence of strong coupling to a bath. We analyze a large range of parameters and identify those which are best suited for quantum memories. In general we find that a small number of links between qubit and bath spins leads to less decoherence and that systems with Ising coupling between qubit and bath spins are preferable.