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arXiv:0902.1862 · Physical Review A

Orientation-dependent spontaneous emission rates of a two-level quantum emitter in any nanophotonic environment

Willem L. Vos, A. Femius Koenderink, Ivan S. Nikolaev

Published Nov 2, 2009• 64 citations
arXivHTMLPDF

Abstract

We study theoretically the spontaneous emission rate of a two-level quantum emitter in any nanophotonic system. We derive a general representation of the rate on the orientation of the transition dipole by only invoking symmetry of the Green function. The rate depends quadratically on orientation and is determined by rates along three principal axes, which greatly simplifies visualization: emission rate surfaces provide insight on how preferred orientations for enhancement (or inhibition) depend on emission frequency and location, as shown for a mirror, a plasmonic sphere, and a photonic band-gap crystal. Moreover, insight is provided on means to ``switch'' the emission rates by actively controlling the orientation of the emitters' transition dipole.

DOI
10.1103/physreva.80.053802

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We study theoretically the spontaneous emission rate of a two-level quantum emitter in any nanophotonic system. We derive a general representation of the rate on the orientation of the transition dipole by only invoking symmetry of the Green function. The rate depends quadratically on orientation and is determined by rates along three principal axes, which greatly simplifies visualization: emission rate surfaces provide insight on how preferred orientations for enhancement (or inhibition) depend on emission frequency and location, as shown for a mirror, a plasmonic sphere, and a photonic band-gap crystal. Moreover, insight is provided on means to ``switch'' the emission rates by actively controlling the orientation of the emitters' transition dipole.
We develop a framework that computes two-photon spontaneous emission (TPSE) spectra of a quantum emitter near an arbitrarily shaped nanostructure. The model considers the interaction up to the electric quadrupolar order, which is relevant for nanophotonic structures sustaining strongly confined fields that are used to enhance and to tailor spontaneous emission processes. Moreover, we consider interference effects between multipolar two-photon emission channels, for the first time to our knowledge. First, we show for a s → s transition of a hydrogen atom placed under a silver plasmonic nanodisk a substantial enhancement in the photon-pair emission rates by 5 and 11 orders of magnitude for the two-electric dipole (2ED) and two-electric quadrupole (2EQ) transitions, respectively. Then for the same emitter under a plasmonic graphene nanotriangle, we demonstrate a breakdown of the electric dipole approximation in the TPSE process where the interference between the 2ED and 2EQ transitions is important, as it increases the total rate by 63 %. Third, we explore platforms where entangled photons of different energy are emitted in the far-field in different directions. In the end, our framework is a complete tool to design emitters and nanostructures for the TPSE process, leading to a rich assortment of functional nanoantennas.
We consider the spontaneous emission of a two-level quantum emitter, such as an atom or a quantum dot, in a modulated time-dependent environment with a photonic band gap. An example of such an environment is a dynamical photonic crystal or any other environment with a band gap whose properties are modulated in time, in the effective mass approximation. After introducing our model of a dynamical photonic crystal, we show that it allows new possibilities to control and tailor the physical features of the emitted radiation, specifically its frequency spectrum. In the weak-coupling limit and in an adiabatic case, we obtain the emitted spectrum and we show the appearance of two lateral peaks due to the presence of the modulated environment, separated from the central peak by the modulation frequency. We show that the two side peaks are not symmetric in height, and that their height ratio can be exploited to investigate the density of states of the environment. Our results show that a dynamical environment can give further possibilities to modify the spontaneous emission features, such as its spectrum and emission rate, with respect to a static one. Observability of the phenomena we obtain is discussed, as well as relevance for tailoring and engineering radiative processes.
Impressive progress has been achieved in controlling the spontaneous emission rate for emitters in Nanophotonic structures, such as microcavities, photonic crystals and nano-antennas. In all cases, however, the modification of the emission is stationary in time. Thus, the emission rate is time-independent and the distribution of photon emission times are stochastic and follow an exponential distribution in the weak coupling regime. In this paper, by using fast all-optical switching of a microcavity, the cavity resonance is tuned within tens of picosesonds. This drastically changes the local optical density of states at the emission frequency within the emission lifetime of the emitters. This paper theoretically studied an ensemble of two-level sources with a time dependent decay rate and have derived the excited state population and emitted intensity as a function of time for continuous wave and pulsed excitation. Deterministic bursts of dramatically enhanced or inhibited emission intensity within short intervals. Thereby, we control the photon distribution to show behavior that strongly deviates from single exponential decay. This can be used to protect quantum information systems against decoherence and to realize non-Markovian dynamics in cavity quantum electrodynamics.
We analyze the two-time intensity correlation function of the fluorescent field emitted by a three-level V-type quantum emitter located in the vicinity of a two-dimensional periodic plasmonic nanostructure. Due to the interaction of the quantum emitter with an electromagnetic field, the ground state population is excited to the upper levels, presenting decay due to spontaneous emission. The distinctive characteristic of this system is that the decay rates for a quantum emitter with dipole orientation perpendicular and normal to the surface of the nanostructure array exhibit large differences which vary with the distance between the quantum emitter and the two-dimensional nanoparticle array. This leads to simulation of quantum interference effects in spontaneous emission. By studying the dependence of the two-time intensity correlation function on specific physical parameters of the hybrid structure, including the intensity of the applied field, the detuning from resonance, the distance between the quantum emitter and the plasmonic nanostructure, as well as the spacing between the upper levels, we demonstrate a strong modification of the two-time intensity correlation functions. We also identify the conditions under which the two-time intensity correlation function is maximized, an effect which is associated to the bunching to antibunching transition of the emitted photons.
The spontaneous emission (SE) of the excited atoms in a two-dimensional (2D) arbitrary inhomogeneous environment has been systematically studied. The local density of states, which determines the radiation dynamics of a point source (for 3D) or a line source (for 2D), in particular, the SE rate, is represented by the electric dyadic Green's function. The numerical solution of the electric Green's tensor has been accurately obtained with the finite-difference frequency-domain method with the proper approximations of the monopole and dipole sources. The SE of atoms in photonic crystal and plasmonic metal plates has been comprehensively and comparatively investigated. For both the photonic crystal and plasmonic plates systems, the SEs depend on their respective dispersion relations and could be modified by the finite-structure or finite-size effects. This work is important for SE engineering and the optimized design of optoelectronic devices.