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arXiv:0902.0327 · Physical Review A

Classical and quantum analysis of a heterotriatomic molecular Bose-Einstein-condensate model

Arlei Prestes Tonel, C. C. N. Kuhn, G. Santos, Angela Foerster, I. Roditi, Zeila Virginia Torres Santos

Published Jan 26, 2009• 7 citations
arXivHTMLPDF

Abstract

We investigate an integrable Hamiltonian modeling a heterotriatomic molecular Bose-Einstein condensate. This model describes a mixture of two species of atoms in different proportions, which can combine to form a triatomic molecule. Beginning with a classical analysis, we determine the fixed points of the system. Bifurcations of these points separate the parameter space into different regions. Three distinct scenarios are found, varying with the atomic population imbalance. This result suggests the ground-state properties of the quantum model exhibit a sensitivity on the atomic population imbalance, which is confirmed by a quantum analysis using different approaches, such as the ground-state expectation values, the behavior of the quantum dynamics, the energy gap, and the ground-state fidelity.

DOI
10.1103/physreva.79.013624

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We investigate an integrable Hamiltonian modeling a heterotriatomic molecular Bose-Einstein condensate. This model describes a mixture of two species of atoms in different proportions, which can combine to form a triatomic molecule. Beginning with a classical analysis, we determine the fixed points of the system. Bifurcations of these points separate the parameter space into different regions. Three distinct scenarios are found, varying with the atomic population imbalance. This result suggests the ground-state properties of the quantum model exhibit a sensitivity on the atomic population imbalance, which is confirmed by a quantum analysis using different approaches, such as the ground-state expectation values, the behavior of the quantum dynamics, the energy gap, and the ground-state fidelity.
This work contains a detailed analysis of the properties of the ground state of a two-component two-site Bose-Hubbard model, which captures the physics of a binary mixture of Bose-Einstein condensates trapped in a double-well potential. The atom-atom interactions within each species and among the two species are taken as variable parameters, while the hopping terms are kept fixed. To characterize the ground state, we use observables such as the imbalance of population and its quantum uncertainty. The quantum many-body correlations present in the system are further quantified by studying the degree of condensation of each species, the entanglement between the two sites, and the entanglement between the two species. The latter is measured by means of the Schmidt gap, the von Neumann entropy, or the purity obtained after tracing out a part of the system. A number of relevant states are identified, e.g., Schr\"odinger catlike many-body states, in which the outcome of the population imbalance of both components is completely correlated, and other states with even larger von Neumann entropy which have a large spread in Fock space.
The ground state and spectral properties of Bose gases in double-well potentials are studied in two different scenarios: (i) an interacting atomic Bose gas, and (ii) a mixture of an atomic gas interacting with diatomic molecules. A ground state second-order quantum phase transition is observed in both scenarios. For large attractive values of the atom-atom interaction, the ground state is degenerate. For repulsive and small attractive interaction, the ground state is not degenerate and is well approximated by a boson coherent state. Both systems depict an excited state quantum phase transition. In both cases, a critical energy separates a region in which all the energy levels are degenerate in pairs, from another region in which there are no degeneracies. For the atomic system, the critical point displays a singularity in the density of states, whereas this behavior is largely smoothed for the mixed atom-molecule system.
A study of coherent photoassociation is presented for the case of an atomic Bose-Einstein condensate. It is shown that the phenomenon is analogous to coherent optical transient in a few-level system, with a difference that the participating levels have Bose enhanced populations. A second-quantized Hamiltonian in momentum and position representation is developed to describe photoassociation. A classical version of the field theory for atoms and molecules is used to demonstrate that in the presence of photoassociating light, a joint atom-molecule condensate is unstable against the growth of the density fluctuations. ^ A simple mean-field model of atom-molecule Bose-Einstein condensate is constructed and it is shown that in the model there is no collapse, irrespective of the sign of the effective atom-atom scattering length. The properties of the two most important eigenstates, the ground state and the twin state, are determined for different values of the system parameters δ and K, the detuning and the atom-molecule coupling, respectively. It is shown that in a coupled atom-molecule system a collapse is replaced by a dynamical instability. The lines in the parameter space where these instabilities occur are in fact fractures where the underlying eigenstates discontinuously change. The features of instability are in good qualitative agreement with the experimental observations of collapse. ^
Abstract We investigate the chaotic dynamics of a coupled three-level atom–molecular Bose–Einstein condensate system composed by one molecular mode and two atomic modes. With the increase of atom–molecular coupling strength, we reveal the emergence of chaotic oscillations of the relative population difference between two atomic modes, which can be proven by the broad windows with a huge number of frequencies in spectral density and the chaotic trajectories in phase space diagrams. The different effects of initial states on atomic population oscillations are revealed, where for more particles in the initial state of the molecular model, chaos appears in the larger parameter region of system dynamics. Furthermore, we find that strong intermolecular interaction strength can suppress chaos resulting from strong atom–molecule coupling. This is due to the difficult transformation between atomic and molecular modes, as well as the relatively independent dynamic evolution of atoms and molecules.
We study the effect of atom-molecule internal tunneling on the ground state of atom-molecule Bose-Einstein condensates in a double-well potential. In the absence of internal tunneling between atomic and molecular states, the ground state is symmetric, which has equal-particle populations in two wells. From the linear stability analysis, we show that the symmetric stationary state becomes dynamically unstable at a certain value of the atom-molecule internal tunneling strength. Above the critical value of the internal tunneling strength, the ground state bifurcates to the particle-localized ground states. The origin of this transition can be attributed to the effective attractive interatomic interaction induced by the atom-molecule internal tunneling. This effective interaction is similar to that familiar in the context of BCS-BEC crossover in a Fermi gas with Feshbach resonance. Furthermore, we point out the possibility of reentrant transition in the case of the large detuning between the atomic and molecular states.