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arXiv:0901.3439 · Acta Physica Slovaca Reviews and Tutorials

An introduction to the quantum theory of nonlinear optics

Mark S. Hillery

Published Feb 1, 2009• 45 citations
arXivHTMLPDF

Abstract

An introduction to the quantum theory of nonlinear optics This article is provides an introduction to the quantum theory of optics in nonlinear dielectric media. We begin with a short summary of the classical theory of nonlinear optics, that is nonlinear optics done with classical fields. We then discuss the canonical formalism for fields and its quantization. This is applied to quantizing the electromagnetic field in free space. The definition of a nonclassical state of the electromagnetic field is presented, and several examples are examined. This is followed by a brief introduction to entanglement in the context of field modes. The next task is the quantization of the electromagnetic field in an inhomogeneous, linear dielectric medium. Before going on to field quantization in nonlinear media, we discuss a number of commonly employed phenomenological models for quantum nonlinear optical processes. We then quantize the field in both nondispersive and dispersive nonlinear media. Flaws in the most commonly used methods of accomplishing this task are pointed out and discussed. Once the quantization has been completed, it is used to study a multimode theory of parametric down conversion and the propagation of quantum solitons.

DOI
10.2478/v10155-010-0094-8

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An introduction to the quantum theory of nonlinear optics This article is provides an introduction to the quantum theory of optics in nonlinear dielectric media. We begin with a short summary of the classical theory of nonlinear optics, that is nonlinear optics done with classical fields. We then discuss the canonical formalism for fields and its quantization. This is applied to quantizing the electromagnetic field in free space. The definition of a nonclassical state of the electromagnetic field is presented, and several examples are examined. This is followed by a brief introduction to entanglement in the context of field modes. The next task is the quantization of the electromagnetic field in an inhomogeneous, linear dielectric medium. Before going on to field quantization in nonlinear media, we discuss a number of commonly employed phenomenological models for quantum nonlinear optical processes. We then quantize the field in both nondispersive and dispersive nonlinear media. Flaws in the most commonly used methods of accomplishing this task are pointed out and discussed. Once the quantization has been completed, it is used to study a multimode theory of parametric down conversion and the propagation of quantum solitons.
Before discussing nonlinear optics with quantized fields, it is useful to have a look at what happens with classical electromagnetic fields in nonlinear dielectric media. The theory of nonlinear optics was originally developed using classical fields by Armstrong, Bloembergen, Ducuing and Pershan in 1962, stimulated by an experiment by Franken, Hill, Peters and Weinreich in which a second harmonic of a laser field was produced by shining the laser into a crystal. This classical theory is sufficient for many applications. For the most part, quantized fields were introduced later, although a quantum theory for the parametric amplifier, a nonlinear device in which three modes are coupled, was developed by Louisell, Yariv and Siegman as early as 1961. In any case, a study of the classical theory will give us an idea of some of the effects to look for when we formulate the more complicated quantum theory. What we will present here is a very short introduction to the subject. Our intent is to use the classical theory to present some of the basic concepts and methods of nonlinear optics. Further information can be found in the list of additional reading at the end of the chapter. The discussion here is based primarily on the presentations in the books by N. Bloembergen and by R. W. Boyd. Linear polarizability We wish to survey some of the effects caused by the linear polarizability of a dielectric medium. When an electric field E ( r , t ) is applied to a dielectric medium, a polarization, that is, a dipole moment per unit volume, is created in the medium.
Starting with the canonical quantization procedure for the electromagnetic field inside an effective (linear or nonlinear) medium, we present a direct-space formulation of the theory of quantum optics. This approach does not use the conventional modal decomposition of the field, but relies on the electromagnetic momentum operator defined in terms of local electric- and magnetic-field operators. The momentum operator contains all the information on the spatial characteristics of the field, and can describe the translation of a short light pulse in a nonlinear medium, without a modal analysis of the pulse. Propagation is described through an operatorial wave equation that relates the temporal evolution of an electromagnetic pulse to its spatial progression. Through this equation, the direct-space approach to quantum optics can treat traveling-wave nonlinear-optical phenomena and, at the same time, account for their quantum statistics. The theory is applied to squeezed-light generation by the parametric down-conversion of a short laser pulse, as an illustration.
In Chapter 1, we treated the electromagnetic field as classical. Henceforth, we will want to treat it as a quantum field. In order to do so, we will first present some of the formalism of quantum field theory. This formalism is very useful in describing many-particle systems and processes in which the number of particles changes. Why this is important to a quantum description of nonlinear optics can be seen by considering a parametric amplifier of the type discussed in the last chapter. A pump field, consisting of many photons, amplifies idler and signal fields by means of a process in which a pump photon splits into two lower-energy photons, one at the idler frequency and one at the signal frequency. Therefore, what we would like to do in this chapter is to provide a discussion of some of the basics of quantum field theory that will be useful in the treatment of the quantization of the electromagnetic field. In particular, we will begin with a summary of quantum theory notation, and a discussion of many-particle Hilbert spaces. These provide the arena in which all of the action takes place. We will then move on to a treatment of the canonical quantization procedure for fields. This will allow us to develop a scattering theory for fields, which is ideally what we need. This relates the properties of a field entering a medium to those of the field leaving it, and this corresponds to what is done in an experiment.
We present a canonical quantum theory of radiation in nonlinear media taking into account the effects of linear dispersion and absorption in a consistent way. We start from a microscopic model and apply recently developed concepts of the quantization of radiation in dispersive and absorbing linear media and extend the theory in order to include nonlinear optical processes. We derive propagation equations in space and time for the quantized radiation field, with special emphasis on the propagation of quantum-light pulses in Kerr media. In particular, the method enables us to derive systematically the noise sources that arise naturally in the nonlinear terms.
The electromagnetic field is quantized in nonlinear media whose dielectric functions and nonlinear susceptibilities may vary with space. Given the dielectric function and nonlinear susceptibilities, the Hamiltonian of the electromagnetic field is determined completely by this quantization method. From Heisenberg equations we prove that Maxwell's equations are satisfied for the field operators. When the nonlinearity goes to zero, this quantization method returns to the generalized canonical quantization procedure developed in Ref.[1] for linear inhomogeneous media. The general formalism is illustrated by applications to quantization of the second-order and third-order nonlinear quasi-steady-state processes.