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arXiv:0811.4342

An exact spin liquid state on the kagome lattice with topological order

Zhong Wang, Shaolong Wan

Published Nov 26, 2008• 0 citations
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Abstract

We find an exact spin liquid state without time reversal symmetry on the kagome lattice with odd number of electrons per unit cell and explicit wave functions for all eigenstates. We also obtain that all spin-spin correlations are zero except trivial cases. We then show that there are anyonic excitations in our model. Finally, we demonstrate the existence of ground state degeneracy and gapless edge states indicating nontrivial topological order in our model. We also label all eiginstates on torus by local and global string operators.

DOI
10.48550/arxiv.0811.4342

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We find an exact spin liquid state without time reversal symmetry on the kagome lattice with odd number of electrons per unit cell and explicit wave functions for all eigenstates. We also obtain that all spin-spin correlations are zero except trivial cases. We then show that there are anyonic excitations in our model. Finally, we demonstrate the existence of ground state degeneracy and gapless edge states indicating nontrivial topological order in our model. We also label all eiginstates on torus by local and global string operators.
We study an exactly solvable quantum spin model of Kitaev type on the kagome lattice. We find a rich phase diagram which includes a topological (gapped) chiral spin liquid with gapless chiral edge states, and a gapless chiral spin liquid phase with a spin Fermi surface. The ground state of the current model contains an odd number of electrons per unit cell, which qualitatively distinguishes it from previously studied exactly solvable models with a spin Fermi surface. Moreover, we show that the spin Fermi surface is stable against weak perturbations.
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We apply the symmetric tensor network state (TNS) to study the nearest-neighbor spin-1/2 antiferromagnetic Heisenberg model on the kagome lattice. Our method keeps track of the global and gauge symmetries in the TNS update procedure and in tensor renormalization group (TRG) calculations. We also introduce a very sensitive probe for the gap of the ground state---the modular matrices, which can also determine the topological order if the ground state is gapped. We find that the ground state of the Heisenberg model on the kagome lattice is a gapped spin liquid with the Z2{\mathbb{Z}}_{2}Z2​ topological order (or toric code type), which has a long correlation length $\ensuremath{\xi}\ensuremath{\sim}10$ unit cells. We justify that the TRG method can handle very large systems with thousands of spins. Such a long $\ensuremath{\xi}$ explains the gapless behaviors observed in simulations on smaller systems with less than 300 spins or shorter than the length of 10 unit cells. We also discuss experimental implications of the topological excitations encoded in our symmetric tensors.
Recent years have seen the discovery of a chiral spin liquid state - a bosonic analogue of a fractional Quantum Hall state first put forward by Kalmeyer and Laughlin in 1987 - in several deformations of the Heisenberg model on the Kagome lattice. Here, we apply state-of-the-art numerical techniques to one such model, where breaking of the time-reversal symmetry drives the system into the chiral phase. Our methods allow us to obtain explicit matrix-product state representations of the low-lying excitations of the chiral spin liquid state, including the topologically non-trivial semionic excitation. We characterize these excitations and study their energetics as the model is tuned towards a topological phase transition.
Quantum spin liquids, systems in which quantum fluctuations prevent the magnetic ordering of the spin degrees of freedom down to zero temperature, have been the source of much recent theoretical and experimental interest. These systems are characterised by their long ranged entangled states, preserve symmetries down to zero Kelvin, and have been shown to exhibit fascinating properties such as a topological ground state degeneracy and fractionalised spin excitations. In this thesis, we study several of these phases. The first, Kitaev spin liquids, appear in strongly spin-orbit coupled systems, where the SU(2) spin symmetry is broken. Within our mean field approach, we study the quantum phase transition from the gapless Z 2 spin liquid to a magnetically ordered phase within the Heisenberg-Kitaev model. Beyond the mean field theory, we argue that the gauge structure of the spin liquid plays a crucial role in this transition, leading to a confinement of spinons and the generation of magnetic order. We also discuss the three-dimensional iridate compounds, where the Kitaev spin liquid phase has topologically protected bulk and surface excitations. We next discuss spin liquids appearing on the geometrically frustrated kagome lattice. First, we consider non-Kramers spin liquids, in which the spin structure of the theory is protected by lattice, rather than time-reversal, symmetry. As a result, more phases are allowed, which have different properties than those which transform as Kramers doublets. In addition, these may have positive experimental signatures in the Raman scattering intensity, offering a clear path to detect such a state. Finally, we examine possible spin liquid phases on a breathing kagome lattice, where we find a stable Z2 spin liquid to be the ground state. This may help to guide future numerical studies of the kagome lattice Heisenberg model, and may also be relevant to DQVOF, a recently discovered spin liquid candidate compound.
We establish the existence of a chiral spin liquid (CSL) as the exact ground state of the Kitaev model on a decorated honeycomb lattice, which is obtained by replacing each site in the familiar honeycomb lattice with a triangle. This CSL state spontaneously breaks time reversal symmetry but preserves other symmetries. There are two topologically distinct CSL's separated by a quantum critical point. Interestingly, vortex excitations in the topologically nontrivial (Chern number +/-1) CSL obey non-Abelian statistics.