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arXiv:0810.0659 · Physical Review A

Why the two-pulse photon echo is not a good quantum memory protocol

Jérôme Ruggiero, Jean-Louis Le Gouët, Christoph Simon, T. Chanelière

Published May 27, 2009• 93 citations
arXivHTMLPDF

Abstract

We consider in this paper a two-pulse photon echo sequence in the prospect of quantum light storage. We analyze the conditions where quantum storage could be realistically performed. We simply and analytically calculate the efficiency in that limit, and clarify the role of the exactly $\ensuremath{\pi}$-rephasing pulse in the sequence. Our physical interpretation of the process is well supported by its experimental implementation in a ${\text{Tm}}^{3+}$:yttrium aluminum garnet crystal thanks to an accurate control of the rephasing pulse area. We finally address independently the fundamental limitations of the quantum fidelity. Our work allows us to point out on one side the real drawbacks of this scheme for quantum storage and on the other side its specificities which can be a source of inspiration to conceive more promising procedures with rare-earth ion doped crystals.

DOI
10.1103/physreva.79.053851

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We consider in this paper a two-pulse photon echo sequence in the prospect of quantum light storage. We analyze the conditions where quantum storage could be realistically performed. We simply and analytically calculate the efficiency in that limit, and clarify the role of the exactly \ensuremathπ\ensuremath{\pi}\ensuremathπ-rephasing pulse in the sequence. Our physical interpretation of the process is well supported by its experimental implementation in a Tm3+{\text{Tm}}^{3+}Tm3+:yttrium aluminum garnet crystal thanks to an accurate control of the rephasing pulse area. We finally address independently the fundamental limitations of the quantum fidelity. Our work allows us to point out on one side the real drawbacks of this scheme for quantum storage and on the other side its specificities which can be a source of inspiration to conceive more promising procedures with rare-earth ion doped crystals.
Abstract Photon echo is a fundamental tool for the manipulation of electromagnetic fields. Unavoidable spontaneous emission noise is generated in this process due to the strong rephasing pulse, which limits the achievable signal-to-noise ratio and represents a fundamental obstacle towards their applications in the quantum regime. Here we propose a noiseless photon-echo protocol based on a four-level atomic system. We implement this protocol in a Eu3+:Y2SiO5 crystal to serve as an optical quantum memory. A storage fidelity of 0.952 ± 0.018 is obtained for time-bin qubits encoded with single-photon-level coherent pulses, which is far beyond the maximal fidelity achievable using the classical measure-and-prepare strategy. In this work, the demonstrated noiseless photon-echo quantum memory features spin-wave storage, easy operation and high storage fidelity, which should be easily extended to other physical systems.
Abstract Photon echo is a fundamental tool for the manipulation of electromagnetic fields. Unavoidable spontaneous emission noise is generated in this process due to the strong rephasing pulse, which limits the achievable signal-to-noise ratio and represents a fundamental obstacle towards their applications in the quantum regime. Here we propose a noiseless photon-echo protocol based on a four-level atomic system. We implement this protocol in a Eu3+:Y2SiO5 crystal to serve as an optical quantum memory. A storage fidelity of 0.952 ± 0.018 is obtained for time-bin qubits encoded with single-photon-level coherent pulses, which is far beyond the maximal fidelity achievable using the classical measure-and-prepare strategy. In this work, the demonstrated noiseless photon-echo quantum memory features spin-wave storage, easy operation and high storage fidelity, which should be easily extended to other physical systems.
This thesis describes experiments aimed at developing a key component in applications such as quantum networks and long-distance quantum communication systems: quantum memories. Quantum memories for light using photon-echo and coherent rephrasing techniques have been developed. The work is carried out on rare-earth-ion-doped inorganic crystals. Several properties are associated with these crystals such as long coherence times and long-lived ground state sublevels that are particularly interesting in connection applications in the area of quantum information science. It is demonstrated the preparation of optical inhomogeneous absorption profiles such that the light only interacts with a specific transition at a selected frequency. Narrow absorbing structures with widths of <100 kHz have been prepared with no absorption in the surrounding spectral interval. Most of the experiments were carried out using Pr3+:Y2SiO5. However, in our search for suitable a Λ-system in the material under consideration, we also performed spectral hole-burning spectroscopy in Nd:Y2SiVO4. As part of the search for host materials for Pr, Pr:La2(WO4)3 crystal was characterized using a variety of methods, such as, hole burning and photon-echoes. Electromagnetically induced transparency was also observed in this crystal. The most important criteria for evaluating quantum memory performance and the most important physical requirements are discussed. After investigating the standard photon echo techniques and controlled reversible inhomogeneous broadening (CRIB) for quantum state storage, we considered an efficient multimode quantum memory protocol; the atomic frequency comb (AFC) protocol. Combs with peaks of widths 100-300 kHz and an optical depth of~ 10 were created by optical pumping inside an emptied region of the inhomogeneous profile of Pr3+:Y2SiO5, allowing us to improve the efficiency of light storage. Light storage combining a photon-echo technique based on an AFC and spin-wave storage have been demonstrated, and an experimental AFC scheme for the storage of weak coherent light pulses in Pr3+:Y2SiO5 is presented. Finally, we have investigated superradiance and slow light effects. Both these effects occur in the high optical depth regime and can influence the memory performance. Under certain conditions superradiance results in the immediate re-emission of the stored light in a single burst of coherent radiation, and inside spectrally structured materials, slow light effects may result when storage is performed.
Unlike slow-light-based quantum memories, photon echoes offer the benefit of high speed and wide bandwidth. Over the last decade, the rephasing mechanism of photon echoes has been studied for quantum memories to overcome fundamental limitations in photon echoes, such as population inversion and low retrieval efficiency. Although these limitations have been overcome in modified photon echo schemes, photon storage time is still too short to apply it to long-distance quantum communications. For long-distance quantum communications, ultralong photon storage time of the order of seconds is needed to implement quantum repeaters. In this review article, challenging techniques for ultralong photon storage are presented, where ultralong storage is obtained via a coherence conversion process between optical and spin states by using an optical locking technique. To remove population-inversion-caused quantum noise, a double rephasing scheme is addressed, where rephasing-pulse-caused population inversion hinders photon echoes for quantum memory applications.
Based on new obtained analytical results, the main properties of photon echo quantum memory protocols are analysed and discussed together with recently achieved experimental results. The main attention is paid to studying the influence of spectral dispersion and nonlinear interaction of light pulses with resonant atoms. The distinctive features of the effect of spectral dispersion on the quantum storage of broadband signal pulses in the studied echo protocols are identified and discussed. Using photon echo area theorem, closed analytical solutions for echo protocols of quantum memory are obtained, describing the storage of weak and intense signal pulses, allowing us to find the conditions for the implementation of high efficiency in the echo protocols under strong nonlinear interaction of signal and control pulses with atoms. The key existing practical problems and the ways to solve them in realistic experimental conditions are outlined. We also briefly discuss the potential of using the considered photon echo quantum memory protocols in a quantum repeater.
Coherence rephasing is an essential step in quantum storage protocols that use echo-based strategies. We present a thorough analysis on how two adiabatic rapid passages (ARPs) are able to rephase atomic coherences in an inhomogeneously broadened ensemble. We consider both optical and spin coherences, rephased by optical or radio-frequency (rf) ARPs, respectively. We show how a rephasing sequence consisting of two ARPs in a double-echo scheme is equivalent to the identity operator ( any state can be recovered), as long as certain conditions are fulfilled. Our mathematical treatment of the ARPs leads to a very simple geometrical interpretation within the Bloch sphere that permits a visual comprehension of the rephasing process. We also identify the conditions that ensure the rephasing, finding that the phase of the optical or rf ARP fields plays a key role in the ability of the sequence to preserve the phase of the superposition state. This settles a difference between optical and rf ARPs, since field phase control is not readily guaranteed in the former case. We also provide a quantitative comparison between π -pulse and ARP rephasing efficiencies, showing the superiority of the latter. We experimentally verify the conclusions of our analysis through rf ARP rephasing sequences performed on the rare-earth ion-doped crystal Tm 3+ :YAG, of interest in quantum memories.