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arXiv:0809.1587 · Physical Review A

Non-Markovian dynamics, nonlocality, and entanglement in quantum Brownian motion

K. Shiokawa

Published Jan 9, 2009• 16 citations
arXivHTMLPDF

Abstract

The dynamical aspects of quantum Brownian motion at low temperatures are investigated. Exact calculations of quantum entanglement among two Brownian oscillators are given without invoking the Born-Markov or Born approximation widely used for the study of open systems. Nonlocality due to finite oscillator separation is studied. Our approach is applicable for arbitrary time scale, in particular suitable to probe the short-time regime at cold temperatures where many experiments on quantum information processing are performed. We study separability criteria based on the uncertainty relation, negativity, and entanglement of formation. We found a crossover behavior in a disentanglement process between quantum- and thermal-fluctuation-dominated regimes. The fluctuation-dissipation theorem is violated for two Brownian particles interacting with a common environment. The deviation from the relation originates in the interaction mediated by the environment, which drives two particles into a steady oscillatory state, preventing the system from thermalizing. Consequently there is a residual entanglement at low temperatures for arbitrary coupling strength. This entanglement is generated from the environment nonperturbatively even when two modes are not entangled initially. When the distance between two oscillators is varied, competition between entanglement induced from the environment and modified decoherence due to finite separation leads to the characteristic distance where entanglement is minimized.

DOI
10.1103/physreva.79.012308

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The dynamical aspects of quantum Brownian motion at low temperatures are investigated. Exact calculations of quantum entanglement among two Brownian oscillators are given without invoking the Born-Markov or Born approximation widely used for the study of open systems. Nonlocality due to finite oscillator separation is studied. Our approach is applicable for arbitrary time scale, in particular suitable to probe the short-time regime at cold temperatures where many experiments on quantum information processing are performed. We study separability criteria based on the uncertainty relation, negativity, and entanglement of formation. We found a crossover behavior in a disentanglement process between quantum- and thermal-fluctuation-dominated regimes. The fluctuation-dissipation theorem is violated for two Brownian particles interacting with a common environment. The deviation from the relation originates in the interaction mediated by the environment, which drives two particles into a steady oscillatory state, preventing the system from thermalizing. Consequently there is a residual entanglement at low temperatures for arbitrary coupling strength. This entanglement is generated from the environment nonperturbatively even when two modes are not entangled initially. When the distance between two oscillators is varied, competition between entanglement induced from the environment and modified decoherence due to finite separation leads to the characteristic distance where entanglement is minimized.
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An open quantum system is a quantum system that interacts with some environment whose degrees of freedom have been coarse grained away. This model describes non-equilibrium processes more general than scattering-matrix formulations. Furthermore, the microscopically-derived environment provides a model of noise, dissipation and decoherence far more general than Markovian (white noise) models. The latter are fully characterized by Lindblad equations and can be motivated phenomenologically. Non-Markovian processes consistently account for backreaction with the environment and can incorporate effects such as finite temperature and spatial correlations. We consider linear systems with bilinear coupling to the environment, or quantum Brownian motion, and nonlinear systems with weak coupling to the environment. For linear systems we provide exact solutions with analytical results for a variety of spectral densities. Furthermore, we point out an important mathematical subtlety which led to incorrect master-equation coefficients in earlier derivations, given nonlocal dissipation. For nonlinear systems we provide perturbative solutions by translating the formalism of canonical perturbation theory into the context of master equations. It is shown that unavoidable degeneracy causes an unfortunate reduction in accuracy between perturbative master equations and their solutions. We also extend the famous theorem of Lindblad, Gorini, Kossakowski and Sudarshan on completely positivity to non-Markovian master equations. Our application is primarily to model atoms interacting via a common electromagnetic field. The electromagnetic field contains correlations in both space and time, which are related to its relativistic (photon-mediated) nature. As such, atoms residing in the same field experience different environmental effects depending upon their relative position and orientation. Our more accurate solutions were necessary to assess sudden death of entanglement at zero temperature. In contrast to previous claims, we found that all initial states of two-level atoms undergo finite-time disentanglement. We were also able to access regimes which cannot be described by Lindblad equations and other simpler methods, such as near resonance. Finally we revisit the infamous Abraham-Lorentz force, wherein a single particle in motion experiences backreaction from the electromagnetic field. This leads to a number of well-known problems including pre-acceleration and runaway solutions. We found a more a more-suitable open-system treatment of the nonrelativistic particle to be perfectly causal and dissipative without any extraneous requirements for finite size of the particle, weak coupling to the field, etc..
We solve the model of N quantum Brownian oscillators linearly coupled to an environment of quantum oscillators at finite temperature, with no extra assumptions about the structure of the system-environment coupling. Using a compact phase-space formalism, we give a rather quick and direct derivation of the master equation and its solutions for general spectral functions and arbitrary temperatures. Since our framework is intrinsically nonperturbative, we are able to analyze the entanglement dynamics of two oscillators coupled to a common scalar field in previously unexplored regimes, such as off resonance and strong coupling.
We explore some aspects of nonequilibrium statistical mechanics of classical and quantum systems. Two chapters are devoted to fluctuation theorems which were originally derived for classical systems. The main challenge in formulating them in quantum mechanics is the fact that fundamental quantities of interest, like work, are defined via the classical concept of a phase space trajectory. We utilize the decoherent histories conceptual framework, in which classical trajectories emerge in quantum mechanics as a result of coarse graining, and provide a first-principles analysis of the nonequilibrium work relation of Jarzynski and Crooks's fluctuation theorem for a quantum system interacting with a general environment based on the quantum Brownian motion (QBM) model. We indicate a parameter range at low temperatures where the theorems might fail in their original form. Fluctuation theorems of Jarzynski and Crooks for systems obeying classical Hamiltonian dynamics are derived under the assumption that the initial conditions are sampled from a canonical ensemble, even though the equilibrium state of an isolated system is typically associated with the microcanonical ensemble. We address this issue through an exact analysis of the classical Brownian motion model. We argue that a stronger form of ensemble equivalence than usually discussed in equilibrium statistical mechanics is required for these theorems to hold in the infinite environment limit irrespective of the ensemble used, and proceed to prove it for this model. An exact expression for the probability distribution of work is obtained for finite environments. Intuitively one expects a system to relax to an equilibrium state when brought into contact with a thermal environment. Yet it is important to have rigorous results that provide conditions for equilibration and characterize the equilibrium state. We consider the dynamics of open quantum systems using the Langevin and master equations and rigorously show that under fairly general conditions quantum systems interacting with a heat bath relax to the equilibrium state defined as the reduced thermal state of the system plus environment, even in the strong coupling regime. Our proof is valid to second-order in interaction strength for general systems and exact for the linear QBM model, for which we also show the equivalence of multi-time correlations. In the final chapter we give a sampling of our investigations into macroscopic quantum phenomena. We work out in detail a specific example of how and under what conditions the center of mass (CoM) coordinate of a macroscopic object emerges as the relevant degree of freedom. Interaction patterns are studied in terms of the couplings they induce between the CoM and relative coordinates of two macroscopic objects. We discuss the implications of these interaction patterns on macroscopic entanglement.
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We study entanglement dynamics in quantum Brownian motion (QBM) models. Our main tool is the Wigner function propagator. Time evolution in the Wigner picture is physically intuitive and it leads to a simple derivation of a master equation for any number of system harmonic oscillators and spectral density of the environment. It also provides generalized uncertainty relations, valid for any initial state, that allow a characterization of the environment in terms of the modifications it causes to the system's dynamics. In particular, the uncertainty relations are very informative about the entanglement dynamics of Gaussian states, and to a lesser extent for other families of states. For concreteness, we apply these techniques to a bipartite QBM model, describing the processes of entanglement creation, disentanglement, and decoherence at all temperatures and time scales.