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arXiv:0808.2687 · Physical Review Letters

Quantum Memory with Optically Trapped Atoms

Chih‐Sung Chuu, Thorsten Straßel, Bo Zhao, Markus Koch, Yu-Ao Chen, Shuai Chen, Zhen-Sheng Yuan, Jörg Schmiedmayer, Jian-Wei Pan

Published Sep 17, 2008• 27 citations
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Abstract

We report the experimental demonstration of quantum memory for collective atomic states in a far-detuned optical dipole trap. Generation of the collective atomic state is heralded by the detection of a Raman scattered photon and accompanied by storage in the ensemble of atoms. The optical dipole trap provides confinement for the atoms during the quantum storage while retaining the atomic coherence. We probe the quantum storage by cross correlation of the photon pair arising from the Raman scattering and the retrieval of the atomic state stored in the memory. Nonclassical correlations are observed for storage times up to 60 mus.

DOI
10.1103/physrevlett.101.120501

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We experimentally demonstrate emission of two quantum-mechanically correlated light pulses with a time delay that is coherently controlled via temporal storage of photonic states in an ensemble of rubidium atoms. The experiment is based on Raman scattering, which produces correlated pairs of spin-flipped atoms and photons, followed by coherent conversion of the atomic states into a different photon beam after a controllable delay. This resonant nonlinear optical process is a promising technique for potential applications in quantum communication.
In this thesis, we explore the quantum dynamics of light interactions with optically thick collections of atoms. We provide a theoretical description of several recent experiments in which some key operations necessary for the implementation of quantum communication networks are demonstrated. Collective Raman scattering from an atomic ensemble is shown to produce probabilistic entanglement between the polarization of a scattered photon and an associated collective atomic excitation. The predicted correlations agree with experimental observations. We also propose a method to use cascade transitions to produce entanglement between a photon with a frequency in the telecom range (ideal for transmission over optical fibers) and a near infrared photon (ideal for storage in an atomic ensemble), and a description of the experimental demonstration is provided. We also propose and describe the implementation of a deterministic source of single photons.\n\nIn addition, we generalize the theory of dark-state polaritons in ensembles of three level Lambda atoms to account for the nuclear spin degeneracy of alkali atoms. This generalized theory provides a description of the first demonstration of single photon storage and retrieval from atomic ensembles. Additionally, in the presence of a uniform magnetic field, we predict the occurrence of collapses and revivals of the photon retrieval efficiency as a function of storage time within the ensemble. These predictions are in very good agreement with subsequent experimental observations. We also exploit the ability of photon storage to entangle remote atomic qubits.
We present the quantum theory for creation of collective atomic memory and generation of nonclassically correlated photon pairs from an ensemble via the protocol of Duan et al. [Nature (London) 414, 413 (2001)]. The temporal evolution of photon numbers, photon statistics, and cross-correlation between the Stokes and anti-Stokes fields is found by solving the equation of motion for atomic spin-wave excitations. We consider a low-finesse cavity model with collectively enhanced signal-to-noise ratio, which remains still considerably large in the free-space limit. Our results describe analytically the dependence of quantum correlations on spin decoherence time and time delay between the write and read lasers and reproduce the observed data very well including the generated pulse shapes, strong violation of Cauchy-Schwarz inequality and conditional generation of anti-Stokes single-photon pulse. The approach we developed may be used also for quantum description of storage and retrieval of quantum information, especially when the statistical properties of nonclassical pulses are studied.
Abstract Quantum entanglement recognized by Einstein, Podolsky, Rosen and Schrodinger is the essence of quantum physics, and has become a real available resource in the laboratory over recent years. The observation of quantum entanglement in macroscopic matters has implications in the fundamental studies of quantum mechanics, as well as the implementations of quantum information technologies, such as quantum communication, enhanced sensing and distributed quantum computing. Here, we report the creation and storage of the heralded entanglement between two different types of broadband quantum memories located on separated platforms at room temperature: a single-photon entangled state delocalized between billions of motional atoms as a collective excitation and an all-optical loop as a flying qubit. The stored entangled state is subsequently retrieved after a programmable storage time, and is verified by measuring the nonclassical correlations, quantum interference, and concurrence of the mapped-out Raman-scattered photons. Our results show that quantum entanglement can be sustained in macroscopic matters at ambient condition, which pushes the fundamental researches of the transition boundary between quantum and classical worlds. Also, the two quantum memories constitute a hybrid memory-built-in quantum network, which highlights the potential of the cooperation between an stationary atomic ensemble and an all-optical loop as quantum nodes at ambient condition, and brings a significant step towards practical quantum networks.
We demonstrate the storage and retrieval of an on-demand single photon generated by a collective Rydberg excitation in an ultra-low noise Raman quantum memory located in a different cold atomic ensemble. We generate single photons on demand by exciting a cold cloud of Rubidium atoms off resonantly to a Rydberg state, with a generation probability up to 15 %\%% per trial. We then show that the single photons can be stored and retrieved with an efficiency of 21 %\%% and a noise floor of pn=2.3(3)×10−4p_n= 2.3(3) \times 10^{-4}pn​=2.3(3)×10−4 per trial in the Raman quantum memory. This leads to a signal-to-noise ratio ranging from 11 to 26 for the retrieved single photon depending on the input photon generation probability, which allows us to observe significant antibunching. We also evaluate the performances of the Raman memory as built-in unbalanced temporal beam splitter, tunable by varying the write-in control pulse intensity. In addition, we demonstrate that the Raman memory can be used to control the single-photon waveshape. These results are a step forward in the implementation of efficient quantum-repeater links using single-photon sources.