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arXiv:0807.3111

Simplified contact pseudopotential for anisotropic interactions of polarized particles under harmonic confinement

Andrei Derevianko

Published Jul 19, 2008• 1 citation
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Abstract

Motivated by the recent progress in cooling and trapping polar molecules, we present a simplified version of the rigorous contact pseudopotential for anisotropically-interacting polarized particles [A. Derevianko, Phys. Rev. A 67, 033607 (2003); Phys. Rev. A 72, 039901(E) (2005)]. The simplifications are carried out for a practically important case of harmonically confined particles described by sufficiently smooth wavefunctions. The resulting contact pseudo-potential depends on the K-matrix of the underlying scattering process and is represented as a sum over pairs of partial waves coupled by the collision. The contribution of each pair of the coupled waves (l and l') involves a tensor product of derivatives of orders l and l'. The asymmetry in the derivatives reflects the anisotropy of the original interaction potential: there is a preferential appearance of the derivatives along the polarizing field.

DOI
10.48550/arxiv.0807.3111

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Motivated by the recent progress in cooling and trapping polar molecules, we present a simplified version of the rigorous contact pseudopotential for anisotropically-interacting polarized particles [A. Derevianko, Phys. Rev. A 67, 033607 (2003); Phys. Rev. A 72, 039901(E) (2005)]. The simplifications are carried out for a practically important case of harmonically confined particles described by sufficiently smooth wavefunctions. The resulting contact pseudo-potential depends on the K-matrix of the underlying scattering process and is represented as a sum over pairs of partial waves coupled by the collision. The contribution of each pair of the coupled waves (l and l') involves a tensor product of derivatives of orders l and l'. The asymmetry in the derivatives reflects the anisotropy of the original interaction potential: there is a preferential appearance of the derivatives along the polarizing field.
An anisotropic pseudopotential arising in the context of collisions of two particles polarized by an external field is rigorously derived and its properties are investigated. Such a low-energy pseudopotential may be useful in describing collective properties of dilute quantum gases, such as molecules polarized by an electric field or metastable 3P2{}^{3}{P}_{2}3P2​ atoms polarized by a magnetic field. The pseudopotential is expressed in terms of the reactance (K) matrix and derivatives of the Dirac $\ensuremath{\delta}$ function. In most applications, it may be represented as a sum of a traditional spherically symmetric contact term and an anisotropic part. The former contribution may be parametrized by a generalized scattering length. The anisotropic part of the pseudopotential may be characterized by the off-diagonal scattering length for dipolar interactions and off-diagonal scattering volume for quadrupolar interactions. The two-body matrix element of the pseudopotential in a basis of plane waves is also derived.
We present a zero-range pseudopotential applicable for all partial wave interactions between neutral atoms. For p and d waves, we derive effective pseudopotentials, which are useful for problems involving anisotropic external potentials. Finally, we consider two nontrivial applications of the p-wave pseudopotential: we solve analytically the problem of two interacting spin-polarized fermions confined in a harmonic trap, and we analyze the scattering of p-wave interacting particles in a quasi-two-dimensional system.
Dipolar Bose and Fermi gases, which are currently being studied extensively experimentally and theoretically, interact through anisotropic, long-range potentials. Here, we replace the long-range potential by a zero-range pseudopotential that simplifies the theoretical treatment of two dipolar particles in a harmonic trap. Our zero-range pseudopotential description reproduces the energy spectrum of two dipoles interacting through a shape-dependent potential under external confinement very well, provided that sufficiently many partial waves are included, and readily leads to a classification scheme of the energy spectrum in terms of approximate angular momentum quantum numbers. The results may be directly relevant to the physics of dipolar gases loaded into optical lattices.
Starting from two identical, interacting particles in an isotropic harmonic trap, we employ first-order perturbation theory to derive the effective s-wave pseudopotential operator for a weakly anisotropic trap. It is shown that such a confinement gives rise to a correction of the s-wave scattering length which is proportional to the square of the ratio of the bare scattering length and the oscillator length. The trap pseudopotential depends on the quantum number of the trapped state, and the effect of a weak anisotropy is dominated by its nearest neighbors. Some implications for experiments with cold bosons in tightly confining potentials are discussed briefly.
Ultracold atomic gases have been of great theoretical and experimental interest in the last two decades. In these systems, the de Broglie wavelength of the particles is much greater than the two body van der Waals length. As a result, the details of the two body interaction potential are irrelevant for a large number of applications and the realistic two body interaction potential can be replaced by a simple finite range or zero range model potential that reproduces the scattering quantities of the full interaction potential. This thesis develops zero range pseudopotentials and applies them to trapped two-particle systems. Ultracold gases loaded into optical lattices can be used to realize two particle systems under approximately harmonic confinement. We use pseudopotentials to obtain the eigenspectrum of two particles under external harmonic confinement semi-analytically. Advancements in trapping technology have resulted in the realization of low dimensional systems. We develop pseudopotentials to treat two body interactions in one and two dimensions. We also elaborate on the physics that is unique to one and two dimensional systems. Feshbach resonances allow for the tunability of the effective two body interaction strength in the presence of a magnetic field. To model Feshbach resonances in two and three dimensions we develop coupled two channel zero range potentials. Dipole-dipole interactions in Chromium and polar molecules have been the subject of a lot of recent research. Unlike the interactions between two alkali atoms, these interactions are long range and anisotropic. We explore the scattering properties of two aligned dipoles using a simple shape dependent model potential. To understand a system two aligned dipoles under confinement, we develop a pseudopotential treatment for cylindrically symmetric interaction potentials under cylindrically symmetric harmonic confinement. This pseudopotential can be used to model any cylindrically symmetric interaction potential. Our zero range treatment describes many features of two aligned dipoles under spherically symmetric harmonic confinement accurately but breaks down when applied to two aligned dipoles under cylindrically symmetric harmonic confinement. The breakdown is unique to the long range nature of the dipole-dipole interaction and expected to be absent for short range interactions.
We analytically derive the general pseudo-potential operator of an arbitrary isotropic interaction for particles confined in two-dimensional (2D) systems, using the same frame work developed by Huang and Yang for 3D scattering [Phys. Rev. {\bf 105}, 767 (1957)]. We also analytically derive the low energy dependence of the phase-shift for an arbitrary potential with a power-law decaying tail, V2D(ρ)∝ρ−αV_{\rm 2D}(\rho)\propto \rho^{-\alpha}V2D​(ρ)∝ρ−α (for α>2\alpha>2α>2). We apply our results to the 2D dipolar gases (α=3\alpha=3α=3) as an example, calculating the momentum and dipole moment dependence of the pseudo-potential for both sss- and p-wave scattering channels if the two scattering particles are in the same 2D layer. We also calculate the result for the s-wave scattering between particles in two different (parallel) layers. Our analytic and numerical results can be directly applied to the study of many-body properties of magnetic dipolar atoms and/or polar molecules in a general 2D system.