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arXiv:0807.0761 · Journal of Physics B Atomic Molecular and Optical Physics

Polarization mixing in optical lattices with uniaxial anisotropy

Hashem Zoubi, Helmut Ritsch

Published Dec 12, 2008• 5 citations
arXivHTMLPDF

Abstract

We study resonant optical excitations of an ultracold gas in an optical lattice in the Mott insulator case. The particles possess anisotropy via an oriented optical transition dipole moment. The anisotropy, prepared by optical pumping into a certain Zeeman sublevel and/or by external static fields, is of a similar type as in uniaxial crystals. Between two mirrors the electronic excitations and the cavity photons of both TE and TM polarizations are coherently mixed to form polariton branches, which can directly be observed in the linear optical spectra. For example, for an incident field of TE polarization we obtain TE and TM transmitted and reflected fields. Also we calculate the phase shift in the TE and TM transmitted and reflected fields relative to the incident field phase, which leads to polarization rotations. Such polarization mixing can serve as a signature of the formation of oriented molecules from spherically symmetric atoms in optical lattices.

DOI
10.1088/0953-4075/42/1/015501

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We study resonant optical excitations of an ultracold gas in an optical lattice in the Mott insulator case. The particles possess anisotropy via an oriented optical transition dipole moment. The anisotropy, prepared by optical pumping into a certain Zeeman sublevel and/or by external static fields, is of a similar type as in uniaxial crystals. Between two mirrors the electronic excitations and the cavity photons of both TE and TM polarizations are coherently mixed to form polariton branches, which can directly be observed in the linear optical spectra. For example, for an incident field of TE polarization we obtain TE and TM transmitted and reflected fields. Also we calculate the phase shift in the TE and TM transmitted and reflected fields relative to the incident field phase, which leads to polarization rotations. Such polarization mixing can serve as a signature of the formation of oriented molecules from spherically symmetric atoms in optical lattices.
We study the resonant electronic excitation dynamics for ultracold atoms trapped in a deep optical lattice prepared in a Mott-insulator state. Excitons in these artificial crystals are similar to Frenkel excitons in noble atom or molecular crystals. They appear when the atomic excited state linewidth is smaller than the exciton bandwidth generated by dipole-dipole coupling. When the atoms are placed within a cavity the electronic excitations and the quantized cavity mode get coupled. In the collective strong coupling regime excitations form two branches of cavity polaritons with Rabi splitting larger than the atomic and the cavity linewidth. To demonstrate their properties we calculate the transmission, reflection, and absorption spectra for an incident weak probe field, which show resonances at the polariton frequencies.
Ultracold atoms uniformly filling an optical lattice can be treated like an artificial crystal. An implementation including the atomic occupation of a single excited atomic state can be represented by a two-component Bose-Hubbard model. Its phase diagram exhibits a quantum phase transition from a superfluid to a Mott insulator phase. The dynamics of electronic excitations governed by electrostatic dipole-dipole interactions in the ordered regime can be well described by wave-like collective excitations called excitons. Here we present an extensive study of such excitons for a wide range of geometries and dimensionality. Their lifetimes can vary over many orders of magnitude from metastable propagation to superradiant decay. Particularly strong effects occur in one dimensional atomic chains coupled to tapered optical fibers. For an optical lattice within a cavity the excitons are coupled to cavity photons and the resulting collective cavity QED model can be efficiently formulated in terms of polaritons. Their properties are explicitly calculated for different lattices and they constitute a non-destructive monitoring tool for important system properties. Even the formation of molecules in optical lattices manifests itself in modified polariton properties as e.g. an anisotropic optical spectrum. Partial dissipation of the exciton energy in the lattice leads to heating, which can be microscopically understood through a mechanism transferring atoms into higher Bloch bands via a resonant excitation transfer among neighboring lattice sites. The presence of lattice defects like vacancies in the Mott insulator induces a characteristic scattering of polaritons, which can be optically observed to monitor the lattice integrity. Our models can be applied to simulate and understand corresponding collective phenomena in solid crystals, where many effects are often masked by noise and disorder.
An important new development in the field of ultracold atomic gases is the study of the properties of these gases in a so-called optical lattice. An optical lattice is a periodic trapping potential for the atoms that is formed by the interference pattern of a few laser beams. A reason for the interest in these systems is that the effects of the interatomic interactions can be strongly enhanced. More specifically, it has been shown in a beautiful experiment by Greiner et al. in 2002 that by loading a Bose-Einstein condensate into an optical lattice it is possible for the system to undergo a quantum phase transition to a new quantum phase of matter, the so-called Mott insulator phase. Within this Mott insulator phase each lattice site is occupied by exactly one atom. This makes the Mott insulator phase especially well suited for applications in the field of quantum computation and quantum information processing. We have theoretically investigated the above mentioned quantum phase transition and our formalism allows for a description of the Mott insulator phase at nonzero temperatures. Another important experimental development in the field of ultracold atomic gases is the use of Feshbach resonances to control the interatomic interactions. Such a resonance occurs whenever two colliding atoms form a long-lived molecule for some time. The crucial point of a Feshbach resonance is that the above mentioned molecule has a magnetic moment that is not equal to twice the magnetic moment of the atom. As a consequence the energy difference between the two atoms and the molecule and hence the interactions between the atoms can be controlled by using an external magnetic field. By combining these two techniques, i.e, by trapping ultracold atomic gases in an optical lattice and by tuning a magnetic field near a Feshbach resonance there can be a new quantum phase transition between two superfluid phases. We gave derived the the theory for the description of these Feshbach resonances in optical lattices and applied it to various systems. To be a bit more precise, if we tune the external magnetic field such that the energy difference between a molecule and two atoms is sufficiently negative, then the gas consists of a Bose-Einstein condensate of molecules. In contrast, if the energy difference is large enough and positive we have a gas that consists primarily of a Bose-Einstein condensate of atoms. It turns out that these two limits are separated by an Ising-like quantum phase transition. By using atomic Bose gases near a Feshbach resonance detailed experimental studies which test the theoretical predictions of the statistical and dynamical properties of these quantum phase transitions can be made.
We study electronic excitations of a degenerate gas of atoms trapped in pairs in an optical lattice. Local dipole-dipole interactions produce a long-lived antisymmetric and a short-lived symmetric superposition of individual atomic excitations as the lowest internal on-site excitations. Due to the much larger dipole moment the symmetric states couple efficiently to neighbouring lattice sites and can be well represented by Frenkel excitons, while the antisymmetric dark states stay localized. Within a cavity only symmetric states couple to cavity photons inducing long-range interactions to form polaritons. We calculate their dispersion curves as well as cavity transmission and reflection spectra to observe them. For a lattice with aspherical sites bright and dark states get mixed and their relative excitation energies depend on photon polarizations.
We study the effect of defects in the Mott insulator phase of ultracold atoms in an optical lattice on the dynamics of resonant electronic excitations. These excitations can be described analogous to Frenkel excitons in solids and form polaritons, when coupled to an optical resonator. Defects, which are empty sites in a singly occupied Mott insulator state or singly occupied sites for a filling factor two, change the exciton dynamics. We show that vacancies behave like hard sphere scatterers, while singly occupied sites in a doubly filled region generate either attractive or repulsive interaction potentials. We suggest cavity polaritons as tools which detect such defects and show how the scattering can be controlled by changing the exciton–photon detuning. In the case of aspherical individual lattice sites, we calculate the effective scattering potential as a function of the cavity photon polarization direction which exhibits a crossover from a repulsive into an attractive potential and should give a clearly observable signal.
We study ultracold atoms trapped in a one-dimensional optical lattice prepared in a Mott insulator state of finite extend and collectively coupled to a single cavity mode. Due to resonant dipole-dipole interactions among the atoms, electronic excitations get delocalized and form excitons . These excitons can be explicitly calculated and divided into two groups: antisymmetric modes which decouple from the cavity mode called dark excitons , and symmetric modes coupled to the cavity mode called bright excitons . In a typical geometry the most uniform exciton is coupled to the cavity photons much stronger than other symmetric bright states and dominates the optical response of the atoms ( superradiant state ). In the strong coupling regime this superradiant state mixes with a cavity photon to form a doublet of polariton states, and the other excitons play only a minor role in the dynamics. We analytically calculate the corresponding collective Rabi splitting including the nearest-neighbor dipole-dipole induced excitonic shifts, which strongly depend on the polarization of the cavity mode with respect to the lattice orientation.