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arXiv:0805.4045 · Physical Review E

Transport control in low-dimensional spin- 1∕2 Heisenberg systems

Léa Ferreira dos Santos

Published Sep 19, 2008• 21 citations
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Abstract

We analyze transport of local magnetization and develop schemes to control transport behavior in finite spin-1/2 Heisenberg chains and spin-1/2 Heisenberg two-leg ladders at zero temperature. By adjusting parameters in the Hamiltonians, these quantum systems may show both integrable and chaotic limits. We provide examples of chaotic systems leading to diffusive and to ballistic transport. In addition, methods of coherent quantum control to induce a transition from diffusive to ballistic transport are proposed.

DOI
10.1103/physreve.78.031125

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We analyze transport of local magnetization and develop schemes to control transport behavior in finite spin-1/2 Heisenberg chains and spin-1/2 Heisenberg two-leg ladders at zero temperature. By adjusting parameters in the Hamiltonians, these quantum systems may show both integrable and chaotic limits. We provide examples of chaotic systems leading to diffusive and to ballistic transport. In addition, methods of coherent quantum control to induce a transition from diffusive to ballistic transport are proposed.
We study transport of local magnetization in spin-1/2 Heisenberg chains in integrable and chaotic regimes at zero temperature. A clean Heisenberg chain with only nearest-neighbor interactions is integrable, whereas the addition of frustrating next-nearest neighbor interactions or yet of on-site disorder may lead to the onset of chaos. For a particular initial state far from equilibrium, the dynamics of local magnetization in the chaotic and non-chaotic clean chains is surprisingly similar, but differ significantly from the disordered system. We also discuss how quantum control methods consisting of sequences of magnetic pulses may be used to remove the effects of particular terms of the Hamiltonian, such as defects or unwanted interactions, and therefore induce a desired transport behavior.
We study transport of local magnetization in a Heisenberg spin-1/2 chain at zero temperature. The system is initially prepared in a highly excited pure state far from equilibrium and its evolution is analyzed via exact diagonalization. Integrable and nonintegrable regimes are obtained by adjusting the parameters of the Hamiltonian, which allows for the comparison of transport behaviors in both limits. In the presence of nearest-neighbor interactions only, the transport behavior in the integrable clean system contrasts with the chaotic chain with on-site defects, oscillations in the first suggesting ballistic transport, and a fast decay in the latter indicating diffusive transport. The results for a nonintegrable system with frustration are less conclusive, similarities with the integrable chain being verified. We also show how methods of quantum control may be applied to chaotic systems to induce a desired transport behavior, such as that of an integrable system.
We study magnetization transport at infinite temperature in several spin ladder systems as well as in next-nearest-neighbor coupled spin chains. In the integrable ladder considered we analytically show that the transport is ballistic in sectors with nonzero average magnetization, while numerical simulations of a nonequilibrium stationary setting indicate an anomalous transport in the zero-magnetization sector. For other systems, isotropic Heisenberg ladder and spin chains, showing eigenlevel repulsion typical of quantum chaotic systems, numerical simulations indicate diffusive transport.
This thesis studies transport properties of low-dimensional quantum spin systems with a particular focus on the transport of heat and spin. While the integrable anisotropic spin-1/2 chain exhibits ballistic transport (finite Drude weights), the numerical results of this work show that heat and spin transport of non-integrable models (spin ladder, frustrated and dimerized chain) is not ballistic, characterized by vanishing Drude weights in the thermodynamic limit. The results for the thermal conductivity of spin ladders are compared to experimental data. For the case of the spin-1/2 Heisenberg chain, this work contains detailed results for the temperature and magnetic field dependence of the Drude weights. Finally, bond-disordered spin systems are considered, namely the spin-1/2 chain and the spin ladder. In the first case, the transport coefficients are computed by means of exact diagonalization and discussed as a function of frequency, temperature, and magnetic field. In the second case, spectral properties of the elementary excitation of disordered spin ladders are analyzed using diagrammatic perturbation theory and numerical techniques.
We show that in a nonintegrable spin ladder system with the XX type of coupling along the legs and the XXZ type along the rungs there are invariant subspaces that support ballistic magnetization transport. In the complementary subspace the transport is found to be diffusive. This shows that (i) quantum chaotic systems can possess ballistic subspaces, and (ii) diffusive and ballistic transport modes can coexist in a rather simple nonintegrable model. In the limit of an infinite anisotropy in rungs the system studied is equivalent to the one-dimensional Hubbard model.
In this thesis, I use a quantum Monte Carlo (QMC) method based on the stochastic series expansion (SSE) to study transport, quantum phase diagrams, and dynamics of several one- and quasi-one-dimensional spin systems, including spin-1/2 and spin-1 chains, a frustrated four-leg spin tube, and N-leg spin-1/2 ladders. I establish a diffusive channel for the finite temperature spin transport of the spin-1/2 antiferromagnetic Heisenberg chain. Extensive finite size studies are detailed, allowing to extract the diffusion kernel in the thermodynamic limit. The diffusion is found to exhibit no anomalous exponent, moreover it is shown to survive for finite values of exchange anisotropy and magnetic fields, however with a strong suppression away from the isotropic point and for increasing magnetic fields. In the case of the spin-1 chain, I obtain the quantum phase diagram and spin dynamics in the combined presence of finite single-ion anisotropies and external magnetic fields. I also prove the existence of magnon modes and multi-particle continua and determine their evolutions as a function of anisotropies and magnetic fields. Moreover, I calculate the magnetic field dependence of the nuclear magnetic relaxation as a function of the single ion anisotropy. For the quasi-one-dimensional spin system of a frustrated four-leg tube, I investigate the regime of large rung coupling, where QMC is applicable. I evaluate the uniform spin susceptibility and the dynamic structure factor and show that in this regime the spin-tube exhibts a crossover from a gapped effective antiferromagnetic spin-2 chain behavior with massive magnons to a gapless Luttinger liquid phase with spinon excitations. Finally, I investigate the spin dynamics of N-leg spin-1/2 ladders with spacially isotropic interactions for N=1,..,5. I obtain the low-lying excitations of the spin ladders as a function of the number of legs and show that they exhibt an even-odd oscillation which is consistent with Haldane's conjecture and other known results for the thermodynamics of spin ladders.