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arXiv:0805.1517 · Physical Review A

Geometrical representation of sum frequency generation and adiabatic frequency conversion

Haim Suchowski, Dan Oron, Ady Arie, Yaron R. Silberberg

Published Dec 15, 2008• 162 citations
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Abstract

We present a geometrical representation of the process of sum frequency generation in the undepleted pump approximation, in analogy with the known optical Bloch equations. We use this analogy to propose a technique for achieving both high efficiency and large bandwidth in sum frequency conversion using the adiabatic inversion scheme. The process is analogous with rapid adiabatic passage in NMR, and adiabatic constraints are derived in this context. This adiabatic frequency conversion scheme is realized experimentally using an aperiodically poled potassium titanyl phosphate (KTP) device, where we achieved high efficiency signal-to-idler conversion over a bandwidth of $140\phantom{\rule{0.3em}{0ex}}\mathrm{nm}$.

DOI
10.1103/physreva.78.063821

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We present a geometrical representation of the process of sum frequency generation in the undepleted pump approximation, in analogy with the known optical Bloch equations. We use this analogy to propose a technique for achieving both high efficiency and large bandwidth in sum frequency conversion using the adiabatic inversion scheme. The process is analogous with rapid adiabatic passage in NMR, and adiabatic constraints are derived in this context. This adiabatic frequency conversion scheme is realized experimentally using an aperiodically poled potassium titanyl phosphate (KTP) device, where we achieved high efficiency signal-to-idler conversion over a bandwidth of 140nm140\phantom{\rule{0.3em}{0ex}}\mathrm{nm}140nm.
We discuss theoretically and demonstrate experimentally the robustness of the adiabatic sum frequency conversion method. This technique, borrowed from an analogous scheme of robust population transfer in atomic physics and nuclear magnetic resonance, enables the achievement of nearly full frequency conversion in a sum frequency generation process for a bandwidth up to two orders of magnitude wider than in conventional conversion schemes. We show that this scheme is robust to variations in the parameters of both the nonlinear crystal and of the incoming light. These include the crystal temperature, the frequency of the incoming field, the pump intensity, the crystal length and the angle of incidence. Also, we show that this extremely broad bandwidth can be tuned to higher or lower central wavelengths by changing either the pump frequency or the crystal temperature. The detailed study of the properties of this converter is done using the Landau-Zener theory dealing with the adiabatic transitions in two level systems.
Abstract The method of adiabatic frequency conversion, in analogy with a two‐level atomic system, has been put forward recently and verified experimentally to achieve robust frequency mixing processes such as sum and difference frequency generation. Here a comparative study of efficient frequency mixing using various techniques of shortcuts to adiabaticity such as counter‐diabatic driving and invariant‐based inverse engineering is presented. It is shown here that it is possible to perform sum frequency generation by properly designing the poling structure of a periodically poled crystal and the coupling between the input lights and the crystal. The required crystal length for frequency conversion significantly decreases beyond the adiabatic limit. This approach significantly improves the robustness of the process against the variation in temperature as well as the signal frequency. By introducing a single parameter control technique with constant coupling and combining with the inverse engineering, perturbation theory, and optimal control, it is shown that the phase mismatch can be further optimized with respect to the fluctuations of input wavelength and crystal temperature that results into a novel experimentally realizable mixing scheme.
Based on the QPM technology and the counter diabatic compensation approach in quantum physics, we propose an optimal scheme that the signal field completely converts into the sum frequency field under the condition of the superadiabaticity. With the geometric rotation plane designed, we subtly reveals the physical mechanism of the systems before and after adding a counter diabatic term. The property of the energy conversion which is analogous to the elastic collision is explained for the addition counter diabatic compensation. With the help of Bloch vectors in atoms physics, we can clearly show the physics process of the complete energy conversion and the physical mechanism for the shortcuts of the superadiabaticity from a new perspective. This new scheme can optimize adiabatic process, shorten the coupling region and nonlinear crystal length, reduce the influence of the dispersion effect, and also implement the robust efficient energy conversion under the condition of relatively weak pump intensity. Not only does this scheme provide a good theoretical basis for the design of nonlinear optical devices, but also its physical thoughts can be widely used in many other fields.
A comprehensive study of two simultaneous three wave mixing processes, a second harmonic generation followed by difference frequency generation, under nonlinear stimulated Raman adiabatic passage (STIRAP) is presented. An input pump is up-converted to its second harmonic, which then gets down-converted to a signal and idler pair with frequencies lying very close to the input pump in such a manner that complete conversion from the pump to the signal and idler takes place without exciting the second harmonic under counterintuitive adiabatic passage. This process involves nonlinear STIRAP with a nonlinear dark state similar to atomic population transfers, and we bring an analogy from atomic systems to our nonlinear dynamics to linearize the problem and analytically obtain the adiabaticity condition required for complete conversion. We also show that the nonlinear STIRAP mechanism results in a large bandwidth of about 380 nm with almost complete conversion of the pump to the signal and idler.
Adiabatic evolution, an important dynamical process in a variety of classical and quantum systems providing a robust way of steering a system into a desired state 1-5, was introduced only recently to frequency conversion 6-9. Adiabatic frequency conversion allowed the achievement of efficient scalable broadband frequency conversion 8, 9 and was applied successfully to the conversion of ultrashort pulses, demonstrating near-100% efficiency for ultrabroadband spectrum 10-16. The underlying analogy between undepleted pump nonlinear processes and coherently excited quantum systems was extended in the past few years to multi-level quantum systems, demonstrating new concepts in frequency conversion, such as complete frequency conversion through an absorption band 17-20. Additionally, the undepleted pump restriction was removed, enabling the exploration of adiabatic processes in the fully nonlinear dynamics regime of nonlinear optics 21-26. In this article, the basic concept of adiabatic frequency conversion is introduced, and recent advances in ultrashort physics, multi-process systems, and the fully nonlinear dynamics regime are reviewed.
The application of the adiabatic geometric phase (AGP) to nonlinear frequency conversion may help to develop new types of all-optical devices, which leads to all-optical modulation of the phase front of one wave by the intensity of other waves. In this paper, we develop the canonical Hamilton equation and a corresponding geometric representation for two schemes of four-wave mixing (FWM) processes (ω1 + ω2 = ω3 + ω4 and ω1 + ω2 + ω3 = ω4), which can precisely describe and calculate the AGP controlled by the quasi-phase matching technique. The AGPs of the idler (ω1) and signal (ω4) waves for these two schemes of FWM are studied systematically when the two pump waves (ω2 and ω3) are in either the undepleted or in the depleted pump cases, respectively. The analysis reveals that the proposed methods for calculating the AGP are universal in both cases. We expect that the analysis of AGP in FWM processes can be applied to all-optically shaping or encoding of ultrafast light pulse.