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arXiv:0805.0301 · Physical Review Letters

Josephson Effect through an Isotropic Magnetic Molecule

Minchul Lee, Thibaut Jonckheere, Thierry Martin

Published Oct 1, 2008• 35 citations
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Abstract

We study the Josephson effect through a quantum dot magnet whose spin is isotropic and which is coupled to the dot electron spin via exchange coupling. We calculate the Andreev levels and the supercurrent and examine the intertwined effect of the exchange coupling, Kondo correlation, and superconductivity. The former suppresses Kondo correlations, which triggers phase transitions from the 0 to the pi state, but strong antiferromagnetic coupling restores the 0 state. The asymmetric phase diagram in the exchange coupling suggests that the coupling sign could be determined in experiments.

DOI
10.1103/physrevlett.101.146804

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We study the Josephson effect through a quantum dot magnet whose spin is isotropic and which is coupled to the dot electron spin via exchange coupling. We calculate the Andreev levels and the supercurrent and examine the intertwined effect of the exchange coupling, Kondo correlation, and superconductivity. The former suppresses Kondo correlations, which triggers phase transitions from the 0 to the pi state, but strong antiferromagnetic coupling restores the 0 state. The asymmetric phase diagram in the exchange coupling suggests that the coupling sign could be determined in experiments.
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The case of a quantum dot connected to two superconducting leads is studied by using the narrow-band limit to describe the superconducting degrees of freedom. The model provides a simple theoretical framework, almost analytical, to analyze the interplay between the Kondo effect, superconductivity, and finite temperature. In the quantum dot Kondo regime, the model is completely characterized by the ratio $\ensuremath{\Delta}/J$, with $\ensuremath{\Delta}$ the superconducting gap and JJJ an effective antiferromagnetic exchange coupling between the dot and the leads. The model allows us to calculate, at any temperature TTT, the equilibrium Josephson current through the dot in a very straightforward way as a function of $\ensuremath{\Delta}/J$. The behavior of the current allows us to distinguish the four types of hybrid junctions: 0, ${0}^{\ensuremath{'}},{\ensuremath{\pi}}^{\ensuremath{'}}$, and $\ensuremath{\pi}$. The presence of the 0- and ${0}^{\ensuremath{'}}$-junction configurations are intrinsically linked to the Kondo effect in the quantum dot, while the $\ensuremath{\pi}$- and ${\ensuremath{\pi}}^{\ensuremath{'}}$-junction configurations are driven by the superconductivity in the leads. The Josephson critical current has a non-monotonic behavior with temperature, that may be used for the experimental characterization of the fundamental $0\ensuremath{-}\ensuremath{\pi}$ transition. The model allows us to obtain easily a phase diagram $\ensuremath{\Delta}/J$ vs temperature, from where we can obtain an overall picture on the stability of the different types of junctions. From the explicit analytical expressions for the ground-state, low-energy excitations, free energy, and Josephson current, it is easy to understand the physical nature of the main features of the critical current and the phase diagram. The results, obtained with a minimum of numerical effort, are in a good qualitative agreement with more demanding calculational approaches aimed to solve the full model.
We investigate the influence of the Fano effect on the Josephson current through a quantum dot (QD) coupled to two identical superconductors (SCs). Our attention is focused on the situation where the Kondo spin singlet survives the superconductivity and the finite- U slave-boson mean-field method is adopted to treat the Kondo correlation. With the direct coupling between the two SCs increased, the Josephson current varies in different manners in different regimes. This is consistent with the variation of Josephson coupling, which exhibits characteristics similar to those shown by the conductance through a QD connected to normal leads. But unlike the normal conductance, a negative Josephson coupling region is formed in the dip of the characteristic asymmetric peak–dip structure. Accompanying this 0–π transition, a new kind of intermediate states is found, which are different from those caused by effective ferromagnetic interaction. This 0–π transition and the intermediate states are yielded entirely by the Fano effect.
We investigate the superconducting Anderson impurity model for interacting quantum dot Josephson junctions with spin-orbit coupling and a term accounting for tunnelling through higher-energy orbitals. These elements establish the conditions required for spin polarization in the absence of external magnetic field at finite superconducting phase bias. This Hamiltonian has been previously used to model the Andreev spin qubit, where quantum information is encoded in spinful odd-parity subgap states. Here we instead analyse the even-parity sector, i.e., the Andreev pair qubit based on Andreev bound states (ABS). The model is solved using the zero-bandwidth approximation and the numerical renormalization group, with further insight from variational calculations. Electron-electron interaction admixes single-occupancy Yu-Shiba-Rusinov (YSR) components into the ABS states, thereby strongly enhancing spin transitions in the presence of spin-orbit coupling. The ABS states can thus become sensitive to local magnetic field fluctuations, which has implications for decoherence in Andreev pair qubits. For strong interaction U U , especially in the cross-over region between the ABS and YSR regimes for U \sim 2\Delta U ∼ 2 Δ , charge, spin, and inductive transitions can all become strong, offering avenues for spin control and quantum transduction.
We analyze the ground state properties of an array of quantum dots connected in series between superconducting electrodes. This system is represented by a finite Hubbard chain coupled at both ends to BCS superconductors. The ground state is obtained using the Lanczos algorithm within a low energy theory in which the bulk superconductors are replaced by effective local pairing potentials. We study the conditions for the inversion of the sign of the Josephson coupling ($\ensuremath{\pi}$-junction behavior) as a function of the model parameters. Results are presented in the form of phase diagrams, which provide a direct overall view of the general trends as the size of the system is increased, exhibiting a strong even-odd effect. The analysis of the spin-spin correlation functions and local charges give further insight into the nature of the ground state and how it is transformed by the presence of superconductivity in the leads. Finally, we study the scaling of the Josephson current with the system size and relate these results with previous calculations of Josephson transport through a Luttinger liquid.
We investigate electronic transport through a parallel double quantum dot (DQD) system with strong on-site Coulomb interaction and capacitive interdot coupling. By applying the numerical renormalization group (NRG) method, the ground state of the system and the transmission probability at zero temperature have been obtained. For a system of quantum dots with degenerate energy levels and small interdot tunnel coupling, the spin correlations between the DQDs is ferromagnetic and the ground state of the system is a spin-1 triplet state. The linear conductance will reach the unitary limit (2e(2)/h) due to the underscreened Kondo effect at low temperature. As the interdot tunnel coupling increases, there is a quantum phase transition from ferromagnetic to antiferromagnetic spin correlation in DQDs and the linear conductance is strongly suppressed.