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arXiv:0804.2396 · Physical Review Letters

Entangled Photon Pairs Produced by a Quantum Dot Strongly Coupled to a Microcavity

R. Johne, Николай Алексеевич Гиппиус, G. Pavlovic, Dmitry D. Solnyshkov, Ivan Andreevich Shelykh, G. Malpuech

Published Jun 18, 2008• 90 citations
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Abstract

We show theoretically that entangled photon pairs can be produced on demand through the biexciton decay of a quantum dot strongly coupled to the modes of a photonic crystal. The strong coupling allows us to tune the energy of the mixed exciton-photon (polariton) eigenmodes and to overcome the natural splitting existing between the exciton states coupled with different linear polarizations of light. Polariton states are moreover well protected against dephasing due to their lifetime of ten to a hundred times shorter than that of a bare exciton. Our analysis shows that the scheme proposed is achievable with the present technology.

DOI
10.1103/physrevlett.100.240404

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We show theoretically that entangled photon pairs can be produced on demand through the biexciton decay of a quantum dot strongly coupled to the modes of a photonic crystal. The strong coupling allows us to tune the energy of the mixed exciton-photon (polariton) eigenmodes and to overcome the natural splitting existing between the exciton states coupled with different linear polarizations of light. Polariton states are moreover well protected against dephasing due to their lifetime of ten to a hundred times shorter than that of a bare exciton. Our analysis shows that the scheme proposed is achievable with the present technology.
A quantum dot strongly coupled to a photonic crystal has been recently proposed as a source of entangled photon pairs [R. Johne et al., Phys. Rev. Lett. 100, 240404 (2008)]. The biexction decay via intermediate polariton states can be used to overcome the natural splitting between the exciton states coupled to the horizontally and vertically polarized light modes so that high degrees of entanglement can be expected. We investigate theoretically the features of realistic dot-cavity systems, including the effect of the different oscillator strength of excitons resonances coupled to the different polarizations of light. We show that in this case, an independent adjustment of the cavity resonances is needed in order to keep a high entanglement degree. We also consider the case when the biexciton-exciton transition is also strongly coupled to a cavity mode. We show that a very fast emission rate can be achieved allowing the repetition rates close to the terahertz range. Such fast emission should however be paid for by a very complex tuning of the many strongly coupled resonances involved and by a loss of quantum efficiency. Altogether a strongly coupled dot-cavity system seems to be very promising as a source of entangled photon pairs.
We present a formal theory of single quantum dot coupling to a planar photonic crystal that supports quasidegenerate cavity modes and use this theory to describe and optimize entangled-photon pair generation via the biexciton-exciton cascade. In the generated photon pairs, either both photons are spontaneously emitted from the dot or one photon is emitted from the biexciton spontaneously while the other is emitted via the leaky cavity mode. In the strong-coupling regime, the generated photon pairs can be maximally entangled in qualitative agreement with the dressed-state predictions of Johne et al. [Phys. Rev. Lett. 100, 240404 (2008)]. We derive useful analytical formulas for the spectrum of the emitted photon pairs in the presence of exciton and biexciton broadening, which is necessary to connect to realistic experiments and demonstrate the important differences with the approximate dressed-state approach. We also present a method for calculating and optimizing the entanglement between the emitted photons, which can account for postsample spectral filtering. Pronounced entanglement values of greater than 80% are demonstrated using experimentally achievable parameters even without spectral filtering.
We present a scheme for the fast generation of entangled photons from a single quantum dot coupled to a planar photonic crystal that support two orthogonally polarized cavity modes. We discuss ``within generation'' and ``across generation'' of entangled photons when both biexciton to exciton, and exciton to ground state transitions, are coupled through cavity modes. In the across generation, the photon entanglement is restored through a time delay between the photons. The two photon concurrence, which is a measure of entanglement, is greater than 0.7 and 0.8 using experimentally achievable parameters in across generation and within generation, respectively. We also show that the entanglement can be distilled in both cases using a simple spectral filter.
We present a scheme for the fast cavity-assisted generation of entangled photon pairs from a single quantum dot coupled to a planar photonic crystal that support two orthogonally polarized cavity modes. We discuss ``within generation'' and ``across generation'' of entangled photons when both the biexciton to exciton, and the exciton to ground-state transitions, are coupled through cavity modes. In the across generation, the photon entanglement is restored through a time delay between the photons. The concurrence, which is a measure of the entanglement between two photons, is greater than 0.7 and 0.8 using experimentally achievable parameters in across generation and within generation, respectively. We also show that the entanglement can be distilled in both cases using a simple spectral filter.
We study the quantum properties and statistics of photons emitted by a quantum-dot biexciton inside a cavity. In the biexciton-exciton cascade, fine-structure splitting between exciton levels degrades polarization-entanglement for the emitted pair of photons. However, here we show that the polarization-entanglement can be preserved in such a system through simultaneous emission of two degenerate photons into cavity modes tuned to half the biexciton energy. Based on detailed theoretical calculations for realistic quantum-dot and cavity parameters, we quantify the degree of achievable entanglement.
Semiconductor quantum dots are promising sources for polarization-entangled photons. As an alternative to the usual cascaded biexciton-exciton emission, direct two-photon emission from the biexciton can be used. With a high-quality optical resonator tuned to half the biexciton energy, a large proportion of the photons can be steered into the two-photon emission channel. In this case the degree of polarization entanglement is inherently insensitive to the exciton fine-structure splitting. In the present work we analyze the biexciton emission with particular emphasis on the influence of coupling of the quantum-dot cavity system to its environment. Especially for a high-quality cavity, the coupling to the surrounding semiconductor material can open up additional phonon-assisted decay channels. Our analysis demonstrates that with the cavity tuned to half the biexciton energy, the potentially detrimental influence of the phonons on the polarization entanglement is strongly suppressed---high degrees of entanglement can still be achieved. We further discuss spectral properties and statistics of the emitted twin photons.