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arXiv:0712.3703 · Reviews of Modern Physics

Optics and interferometry with atoms and molecules

Alexander D. Cronin, Jörg Schmiedmayer, David E. Pritchard

Published Jul 28, 2009• 1,427 citations
arXivHTMLPDF

Abstract

Interference with atomic and molecular matter waves is a rich branch of atomic physics and quantum optics. It started with atom diffraction from crystal surfaces and the separated oscillatory fields technique used in atomic clocks. Atom interferometry is now reaching maturity as a powerful art with many applications in modern science. In this review the basic tools for coherent atom optics are described including diffraction by nanostructures and laser light, three-grating interferometers, and double wells on atom chips. Scientific advances in a broad range of fields that have resulted from the application of atom interferometers are reviewed. These are grouped in three categories: (i) fundamental quantum science, (ii) precision metrology, and (iii) atomic and molecular physics. Although some experiments with Bose-Einstein condensates are included, the focus of the review is on linear matter wave optics, i.e., phenomena where each single atom interferes with itself.

DOI
10.1103/revmodphys.81.1051

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Interference with atomic and molecular matter waves is a rich branch of atomic physics and quantum optics. It started with atom diffraction from crystal surfaces and the separated oscillatory fields technique used in atomic clocks. Atom interferometry is now reaching maturity as a powerful art with many applications in modern science. In this review the basic tools for coherent atom optics are described including diffraction by nanostructures and laser light, three-grating interferometers, and double wells on atom chips. Scientific advances in a broad range of fields that have resulted from the application of atom interferometers are reviewed. These are grouped in three categories: (i) fundamental quantum science, (ii) precision metrology, and (iii) atomic and molecular physics. Although some experiments with Bose-Einstein condensates are included, the focus of the review is on linear matter wave optics, i.e., phenomena where each single atom interferes with itself.
We describe the state of the art in preparing, manipulating and detecting coherent molecular matter. We focus on experimental methods for handling the quantum motion of compound systems from diatomic molecules to clusters or biomolecules.Molecular quantum optics offers many challenges and innovative prospects: already the combination of two atoms into one molecule takes several well-established methods from atomic physics, such as for instance laser cooling, to their limits. The enormous internal complexity that arises when hundreds or thousands of atoms are bound in a single organic molecule, cluster or nanocrystal provides a richness that can only be tackled by combining methods from atomic physics, chemistry, cluster physics, nanotechnology and the life sciences.We review various molecular beam sources and their suitability for matter-wave experiments. We discuss numerous molecular detection schemes and give an overview over diffraction and interference experiments that have already been performed with molecules or clusters.Applications of de Broglie studies with composite systems range from fundamental tests of physics up to quantum-enhanced metrology in physical chemistry, biophysics and the surface sciences.Nanoparticle quantum optics is a growing field, which will intrigue researchers still for many years to come. This review can, therefore, only be a snapshot of a very dynamical process.
The measurement of physical quantities and measurement units standard promote the development of metrology. Especially, the developments of laser interference and atomic frequency standard bring a revolutionary leap for metrology. Many precision measurement techniques have been proposed and experimentally demonstrated, such as gravitational wave measurements and laser gyroscopes based on laser interferometry, and atomic clocks and atomic gyroscopes based on the atom interferometry. Recently, a new branch of science, quantum metrology, has grown up to further explore and exploit the quantum techniques for precision measurement of physical quantities.#br#This paper will focus on recent developments in quantum metrology and interference based on coherence and correlation of light and atom. Firstly, we briefly review the development of metrology. Then, we introduce our own researches in recent years, including quantum-correlation SU(1,1) optical interferometer based on four wave mixing process in atomic vapor and the atom-light hybrid interferometer based on Raman scattering in atomic vapor.#br#Interferometer is a powerful tool to measure physical quantities sensitive to the inference wave with high precision, and has been widely used in scientific research, industry test, navigation and guidance system. For example, the laser interferometer is able to measure optical phase sensitive quantities, including length, angular velocity, gravitational wave and so on. Meanwhile, the atom interferometer is sensitive to the change of atomic phase caused by the light, gravity, electric and magnetic fields. As a new type of interferometry, the atom-light hybrid interferometer, is sensitive to both the optical phase and atomic phase. Furthermore, SU(1,1) interferometer and nonlinear atom-light hybrid interferometer have the ability to beat the standard quantum limit of phase sensitivity. Quantum interference technology, whose phase measurement accuracy can break through the limit of standard quantum limit, is the core of quantum metrology and quantum measurement technology.
Optics and interferometry with matter waves is the art of coherently manipulating the translational motion of particles like neutrons, atoms and molecules. Coherent atom optics is an extension of techniques that were developed for manipulating \emph{internal} quantum states. Applying these ideas to translational motion required the development of techniques to localize atoms and transfer population coherently between distant localities. In this view position and momentum are (continuouse) quantum mechanical degree of freedom analogous to discrete internal quantum states. In our contribution we start with an introduction into matter-wave optics in section 1, discuss coherent atom optics and atom interferometry techniques for molecular beams in section 2 and for trapped atoms in section 3. In section 4 we then describe tools and experiments that allow us to probe the evolution of quantum states of many-body systems by atom interference.
Atom Optics is a new branch of Atomic Physics, where one tries to act upon atoms, likewise one can act upon light (photons) in ordinary optics. The goal is therefore to reflect, focus, diffract, make interfere atoms1 .Afew years ago, this was considered as a fundamental goal, as had been the case decades ago for electron optics, or neutron optics. Indeed, it is always important to investigate the quantum behaviour of larger and larger objects, and studying the wave like behaviour of atoms has attracted a lot of attention. Moreover, atoms are objects that are coupled with the environment in a controlable way, in particular via quasi-resonant interaction with light. There is thus a hope to investigate how this coupling with the environment is relevant to the old problem of the division between the quantum world and the classical world2 ,and how it is related to the question of quantum decoherence. To keep in the domain of Atom Optics, the question of the preservation of coherence of the de Brogue waves describing the atomic motion is crucial. Another basic issue is the question of the collisions between atoms, or between an atom and a surface, when the atom is described as a matter-wave. From this point of view, the very interesting recent results in the domain of cold atoms collisions are only a part of what will probably come out, and new approaches may be fruitful. For instance, some collision effects may be considered as non-linear effects of atom optics... On the other hand, almost from the start, Atom Optics has been a domain where the question of applications has been raised. The experience of the many useful applications existing in the domain of electron and neutron optics has clearly shown the way. A first reason for expecting interesting applications to atom optics is the small value of the de Brogue wavelength, in the nanometer range or below, even at very low energies. This opens for instance the possibility of high resolution lithography, or of nanoprobes, at energies low enough to have a soft, non damaging interaction with a surface. Another important class of applications is in atomic interferometry. It can be shown that atomic interferometers (using atoms of mass Mat) are much more sensitive to inertial or gravitational effects3 than photonic interferometers (using photon of energy hw), by a ratio of the order of MatC2 / ho) . Note that this statement is true only under the condtion that the atomic and photonic interferometers under comparison have equivalent geometries, so that present day interferometers do not yet take full advantage of the 1011 factor of potential improvement. However, impressive results have already be demonstrated6. As a matter of fact, many of the papers presented in this symposium are linked to applications, either with atomic interferometers, or related to the possibility of deep focusing of an atomic beams. Most of these applications a Unite de recherche associée au CNRS can be easily understood by analogy with photon optics. However, there are also several features of atom optics that have no analogy in photon optics. The most important one is probably the possibility to increase the luminosity of an atomic beam (i.e. the flux of atoms per per unit time, surface, and solid angle) or —equivalently — to increase the atomic density in the phase space. This is possible by use of laser cooling, which is a dissipative process, and therefore is not constrained by the Liouville theorem. Another distinctive feature of atom optics —this one not particularly an advantage —is the lack of a sudden interface, that would be analogous to a glass-vacuum interface for light. By sudden interface, we mean that some characteristic parameter relevant to the propagation (the index of refraction in the case of light) changes on a scale small compared to the wavelength of the waves that propagate. In atom optics, the interfaces are usually soft, since the potentials acting on the atomic motion usually change on a scale large compared to the de Broglie wavelengths. In this overview, I intend to recall some basic principles of atom optics, and to point out some important analogies and differences with photon optics4 .Iexpect this discussion to be illustrated by the various presentations at this symposium, for which I hope to offer a framework. In addition, I will take the liberty to illustrate my presentation by some examples chosen among results obtained recently in my laboratory, on the subject of atomic mirrors. The comparison between atom optics and photon optics would of course be incomplete if I would not adress the question of the impact of Bose Einstein condensates onto Atom Optics. As many of us, I am convinced that we are assisting to a revolution as important for Atom Optics as the invention of the laser in the domain of Photon Optics, and we are lucky to have a full session on this hot subject.
Matter - wave interferometry began with the development of electron interferometers and neutron interferometers in the 1950s and 1960s, but it wasn't until 1991 that the first atom matter - wave interferometer was realized. This was followed by a surge of activity sparked by the advent of sources of ultracold laser-cooled atoms. Some of the potential advantages of atom interferometry over neutron interferometry include: much higher particle fluxes, lower particle velocities, larger particle masses, particles with internal states, and laboratory-based sources. This volume is the first text on atom interferometry. It consists of ten comprehensive review articles by leading researchers in the field, many of whom pioneered the first atom interferometers in 1991. The articles describe the different types of atom interferometers developed to date, ranging from the three-grating Mach - Zehnder interferometer based on nanofabricated grating structures (MIT) or standing-wave light-field gratings (Innsbruck), to the Talbot - Lau atom interferometer (Berkeley and Michigan), to atom interferometers based on internal-state labelling such as separated light-field interferometers (PTB, Hannover and Paris-Nord) and light-pulse interferometers (Stanford). Some of the recent applications of atom interferometry described in the articles include high precision measurements of rotations, the gravitational acceleration, and the fine structure constant (Stanford); measurements of topological phases (PTB and Hannover); correlation experiments with atoms and photons (Konstanz) and with pairs of atoms (Tokyo); holographic manipulation of atoms (Tokyo); and experiments on the quantum theory of measurement (Garching, Harvard and Texas A&M). In summary, this volume provides an excellent up-to-date account of atom interferometry and is recommended as essential reading for all researchers and would-be researchers in the field. At the same time it contains sufficient background material and theory to serve as an excellent introduction for the non-specialist. The field is presently moving at such a rapid pace, however, that many of the latest results reported in this volume will already have been superseded by the time it reaches the library shelves.
Our ability to manipulate the coherence properties of light has been at the heart of many of the most important scientific and technological innovations of this century. There can hardly be a home in this country that does not possess a laser in the form of a compact disc player or a CDROM. When we talk on the phone, or send messages on the Internet, there is a high probability that our message will be encoded by a laser into pulses of light to be passed through optical fibres. In the last few years physicists have been discovering that it is possible to control the coherence properties of atoms, and are now developing tools analogous to those which have been developed to take advantage of the coherence properties of light. In the next decade we can look forward to seeing the application of lasers, fibres, mirrors and waveguides for atoms. Already we have been able to construct interferometry experiments using beams of atoms and these have proved to be extremely sensitive measurement devices, allowing us to test physical theories and measure fundamental constants to a level of precision not previously possible. Will these developing technologies ever be as ubiquitous as their optical forebears? In this paper we discuss the anticipated uses of this technology for both fundamental science and industrial applications. Starting from an explanation of the meaning of coherence and a comparison of the properties of photons and atoms, we describe the development of the science of atom optics. The tortuous route towards the great achievement of producing a Bose–Einstein condensate is described, and we explain why this is the most important step towards a laser–like source of atoms. Numerous other optical elements for atoms have been built or are on the drawing board, and we describe how these may be used to manipulate atoms with a precision that has never before been achieved, and look ahead to what we can learn about physics using these tools and at how they can be put to practical use.