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arXiv:0711.3460 · Physical Review Letters

Square-Lattice Algebraic Spin Liquid with SO(5) Symmetry

Cenke Xu, Subir Sachdev A

Published Apr 2, 2008• 24 citations
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Abstract

We propose a critical spin liquid ground state for S=1/2 antiferromagnets on the square lattice. In a renormalization group analysis of the "staggered flux" algebraic spin liquid, we examine perturbations, present in the antiferromagnet, which break its global SU(4) symmetry to SO(5). At physical parameter values, we find an instability towards a fixed point with SO(5) symmetry. We discuss the possibility that this fixed point describes a transition between the Néel and valence bond solid states, and the relationship to the SO(5) nonlinear sigma model of Tanaka and Hu.

DOI
10.1103/physrevlett.100.137201

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We propose a critical spin liquid ground state for S=1/2 antiferromagnets on the square lattice. In a renormalization group analysis of the "staggered flux" algebraic spin liquid, we examine perturbations, present in the antiferromagnet, which break its global SU(4) symmetry to SO(5). At physical parameter values, we find an instability towards a fixed point with SO(5) symmetry. We discuss the possibility that this fixed point describes a transition between the Néel and valence bond solid states, and the relationship to the SO(5) nonlinear sigma model of Tanaka and Hu.
The theory for the vanishing of N\'eel order in the spin S=1/2S=1/2S=1/2 square lattice antiferromagnet has been the focus of attention for many decades. A consensus appears to have emerged in recent numerical studies on the antiferromagnet with first and second neighbor exchange interactions (the ${J}_{1}\text{\ensuremath{-}}{J}_{2}$ model): A gapless spin liquid is present for a narrow window of parameters between the vanishing of the N\'eel order and the onset of a gapped valence bond solid state. We propose a deconfined critical SU(2) gauge theory for a transition into a stable Z2{\mathbb{Z}}_{2}Z2​ spin liquid with massless Dirac spinon excitations; on the other side of the critical point, the SU(2) spin liquid (the `$\ensuremath{\pi}$-flux' phase) is presumed to be unstable to confinement to the N\'eel phase. We identify a dangerously irrelevant coupling in the critical SU(2) gauge theory, which contributes a logarithm-squared renormalization. This critical theory is also not Lorentz invariant and weakly breaks the SO(5) symmetry which rotates between the N\'eel and valence bond solid order parameters. We also propose a distinct deconfined critical U(1) gauge theory for a transition into the same gapless Z2{\mathbb{Z}}_{2}Z2​ spin liquid; on the other side of the critical point, the U(1) spin liquid (the `staggered flux' phase) is presumed to be unstable to confinement to the valence bond solid. This critical theory has no dangerously irrelevant coupling, dynamic critical exponent $z\ensuremath{\ne}1$, and no SO(5) symmetry. All of these phases and critical points are unified in a SU(2) gauge theory with Higgs fields and fermionic spinons which can naturally realize the observed sequence of phases with increasing J2/J1{J}_{2}/{J}_{1}J2​/J1​: N\'eel, gapless Z2{\mathbb{Z}}_{2}Z2​ spin liquid, and valence bond solid.
We study the instabilities caused by four-fermion interactions on algebraic spin liquids. Renormalization group (RG) is used for three types of previously proposed spin liquids on the square lattice: the staggered flux state of SU(2) spin system, the $\ensuremath{\pi}$-flux state of SU(4) spin system, and the $\ensuremath{\pi}$-flux state of SU(2) spin system. The low-energy field theories of the first two types of spin liquids are QED3 with emerged SU(4) and SU(8) flavor symmetries, the low-energy theory of the $\ensuremath{\pi}$-flux SU(2) spin liquid is the QCD3 with SU(2) gauge field and emergent Sp(4) [SO(5)] flavor symmetry. Suitable large-NNN generalization of these spin liquids are discussed, and a systematic 1/N1/N1/N expansion is applied to the RG calculations. The most relevant four-fermion perturbations are identified, and the possible phases driven by relevant perturbations are discussed.
We resolve the nature of the quantum phase transition between antiferromagnetic and valence-bond solid ground states in square-lattice spin-1/2 magnets - the putative deconfined quantum-critical point. Using quantum Monte Carlo simulations of J-Q models, in which Heisenberg exchange J competes with multi-spin interactions Qn formed by n singlet projectors, we demonstrate first-order discontinuities increasing with n. For n=2 and n=3, the first-order signatures are very weak and we extract universal scaling dimensions of a proximate multicritical point. Their values coincide closely with known bounds for an SO(5) symmetric conformal field theory (CFT) containing a relevant SO(5) singlet operator that destabilizes the generic deconfined critical point. We characterize the emergent SO(5) symmetry by its scaling dimensions of the leading irrelevant perturbations. Using the J-Q2-Q6 model, we tune the transition from weak to stronger first-order and find scaling of the coexisting order parameters with a large exponent beta ~ 0.85, in agreement with the relevant scaling dimensions of the multicritical point. The exponent that had previously been identified with the correlation length does not have a corresponding CFT level, and we explain it as pseudo-critical length scale of bubbles of one phase inside the other that are compressed in size by an SO(5)-violating irrelevant repulsive interaction between the two order parameters. The bubble scale reflects a hierarchy of excitation gaps generated by the SO(5) perturbation in the neighborhood of the first-order transition, akin to a Higgs mechanism. We argue that the multicritical point is the tip of a gapless spin liquid phase in frustrated Heisenberg models into which the J-Q models can be deformed, but the spin liquid, and perhaps the multicritical point itself, exist outside the regime amenable to sign-free simulations.
We show numerically that the "deconfined" quantum critical point between the Néel antiferromagnet and the columnar valence-bond solid, for a square lattice of spin 1/2, has an emergent SO(5) symmetry. This symmetry allows the Néel vector and the valence-bond solid order parameter to be rotated into each other. It is a remarkable (2+1)-dimensional analogue of the SO(4)=[SU(2)×SU(2)]/Z(2) symmetry that appears in the scaling limit for the spin-1/2 Heisenberg chain. The emergent SO(5) symmetry is strong evidence that the phase transition in the (2+1)-dimensional system is truly continuous, despite the violations of finite-size scaling observed previously in this problem. It also implies surprising relations between correlation functions at the transition. The symmetry enhancement is expected to apply generally to the critical two-component Abelian Higgs model (noncompact CP(1) model). The result indicates that in three dimensions there is an SO(5)-symmetric conformal field theory that has no relevant singlet operators, so is radically different from conventional Wilson-Fisher-type conformal field theories.
The nature of quantum spin liquids is studied for the spin-1/21/21/2 antiferromagnetic Heisenberg model on a square lattice containing exchange interactions between nearest-neighbor sites, J1J_1J1​, and those between next-nearest-neighbor sites, J2J_2J2​. We perform variational Monte Carlo simulations together with the quantum-number-projection technique and clarify the phase diagram in the ground state together with its excitation spectra. We obtain the nonmagnetic phase in the region 0.4<J2/J1≤0.60.4< J_2/J_1\le 0.60.4<J2​/J1​≤0.6 sandwiched by the staggered and stripe antiferromagnetic (AF) phases. Our direct calculations of the spin gap support the notion that the triplet excitation from the singlet ground state is gapless in the range of 0.4<J2/J1≤0.50.4 < J_2/J_1 \le 0.50.4<J2​/J1​≤0.5, while the gapped valence-bond-crystal (VBC) phase is stabilized for 0.5<J2/J1≤0.60.5 < J_2/J_1 \le 0.60.5<J2​/J1​≤0.6. The VBC order is likely to have the columnar symmetry with a spontaneous symmetry breaking of the C4vC_{4v}C4v​ symmetry. The power-law behaviors of the spin-spin and dimer-dimer correlation functions in the gapless region are consistent with the emergence of the algebraic quantum-spin-liquid phase (critical phase). The exponent of the spin correlation ⟨S(0)S(r)⟩∝1/rz+η\langle S(0)S(r)\rangle \propto 1/r^{z+η}⟨S(0)S(r)⟩∝1/rz+η at a long distance rrr appears to increase from z+η∼1z+η\sim 1z+η∼1 at J2/J1∼0.4J_2/J_1\sim0.4J2​/J1​∼0.4 toward the continuous transition to the VBC phase at J1/J1∼0.5J_1/J_1\sim0.5J1​/J1​∼0.5. Our results, however, do not fully exclude the possibility of a direct quantum transition between the staggered AF and VBC phases with a wide critical region and deconfined criticality.
The algebraic spin liquid is a long-sought-after phase of matter characterized by the absence of quasiparticle excitations, a low-energy description in terms of emergent Dirac fermions and gauge fields interacting according to (2+1)(2+1)(2+1)-dimensional quantum electrodynamics (QED3)({\mathrm{QED}}_{3})(QED3​), and power-law correlations with universal exponents. The prototypical algebraic spin liquid is the Affleck-Marston $\ensuremath{\pi}$-flux phase, originally proposed as a possible ground state of the spin-12\frac{1}{2}21​ Heisenberg model on the two-dimensional square lattice. While the latter model is now known to order antiferromagnetically at zero temperature, recent sign-problem-free quantum Monte Carlo simulations of spin-12\frac{1}{2}21​ fermions coupled to a compact U(1)\text{U}(1)U(1) gauge field on the square lattice have shown that quantum fluctuations can destroy N\'eel order and drive a direct quantum phase transition to the $\ensuremath{\pi}$-flux phase. We show this transition is in the universality class of the chiral Heisenberg QED3{\mathrm{QED}}_{3}QED3​-- Gross-Neveu-Yukawa model with a single SU(2)\text{SU}(2)SU(2) doublet of four-component Dirac fermions (i.e., Nf=1){N}_{f}=1)Nf​=1), pointing out important differences with the corresponding putative transition on the kagome lattice. Using an $\ensuremath{\epsilon}$ expansion below four space-time dimensions to four-loop order, and a large-Nf{N}_{f}Nf​ expansion up to second order, we show the transition is continuous and compute various thermodynamic and susceptibility critical exponents at this transition, setting the stage for future numerical determinations of these quantities. As a by-product of our analysis, we also obtain charge-density-wave and valence-bond-solid susceptibility exponents at the semimetal-N\'eel transition for interacting fermions on the honeycomb lattice.