We revisit a classic study [D. S. Hall, Phys. Rev. Lett. 81, 1539 (1998)10.1103/PhysRevLett.81.1539] of interpenetrating Bose-Einstein condensates in the hyperfine states |F=1,m{f}=-1 identical with |1 and |F=2,m{f}=+1 identical with |2 of 87Rb and observe striking new nonequilibrium component separation dynamics in the form of oscillating ringlike structures. The process of component separation is not significantly damped, a finding that also contrasts sharply with earlier experimental work, allowing a clean first look at a collective excitation of a binary superfluid. We further demonstrate extraordinary quantitative agreement between theoretical and experimental results using a multicomponent mean-field model with key additional features: the inclusion of atomic losses and the careful characterization of trap potentials (at the level of a fraction of a percent).
We revisit a classic study [D. S. Hall, Phys. Rev. Lett. 81, 1539 (1998)10.1103/PhysRevLett.81.1539] of interpenetrating Bose-Einstein condensates in the hyperfine states |F=1,m{f}=-1 identical with |1 and |F=2,m{f}=+1 identical with |2 of 87Rb and observe striking new nonequilibrium component separation dynamics in the form of oscillating ringlike structures. The process of component separation is not significantly damped, a finding that also contrasts sharply with earlier experimental work, allowing a clean first look at a collective excitation of a binary superfluid. We further demonstrate extraordinary quantitative agreement between theoretical and experimental results using a multicomponent mean-field model with key additional features: the inclusion of atomic losses and the careful characterization of trap potentials (at the level of a fraction of a percent).
In this Thesis we study steady state solutions and dynamical evolutions of two– component atomic Bose–Einstein Condensates. We initially investigate the equilibrium properties of condensate mixtures in harmonic trapping potentials at zero temperature. Subsequently we simulate the coupled growth of these condensates by inclusion of damping terms. Finally, we investigate the evolution of coupled Bose gases via the so-called classical–field method. A recent experiment [D. J. McCarron et al., Phys. Rev. A, 84, 011603(R) (2011)] achieved Bose–Einstein Condensation of a two–species 87Rb–133Cs phase segregated mixture in harmonic trapping potentials. Depending on relative atom numbers of the two species, three distinct regimes of density distributions were observed. For these experimental parameters, we investigate the corresponding time–independent ground state solutions through numerical simulations of the coupled Gross–Pitaevskii equations. By including experimentally relevant shifts between the traps, we observe a range of structures including ‘ball and shell’ formations and axially/radially separated states. These are found to be very sensitive to the trap shifts. For all three experimental regimes, our numerical simulations reveal good qualitative agreement. The observed experimental profiles cannot be guaranteed to be fully equilibrated. This, coupled with the rapid sympathetic cooling of the experimental system, leads to a situation where growth may play a determining factor in the density structures formed. To investigate this further, we introduce phenomenological damping to describe the associated condensate growth/decay, revealing a range of transient structures. However, such a model always predicts the predominance of one condensate species over longer evolution times. Work undertaken by collaborators with the more elaborate Stochastic Projected Gross–Pitaevskii equations, which can describe condensate formation by coupling to a heat bath, predicts the spontaneous formation of dark–bright solitons. Motivated by this, we show how the presence of solitons can affect the condensate distribution, thus highlighting the overall dynamical role in the emerging patterns. Finally, we use classical field methods to analyse the evolution of non trapped Bose gases from strongly nonequilibrium initial distributions. The contrast between miscible (overlapping) and immiscible (phase segregated) components gives rise to important distinctions for condensate fractions and the formation of domains and vortices. In addition, splitting the particles of a single component thermalised state into two components is investigated. We then study the effects of suddenly quenching the strength of the interspecies interactions. Under suitable conditions, this quench generates isotropic vortex tangles. While this tangle subsequently decays over time, we propose how a repeat sequence of quenches at regular intervals could be employed to drive the tangle, thereby potentially providing a novel route to the generation of quantum turbulence.
Ultracold atoms and Bose-Einstein condensates represent a burgeoning and ever exciting area of research which has produced numerous breakthroughs in the last 15 years. Ultracold atoms at nano-Kelvin temperatures, isolated in atom traps from the hot, room temperature environment, exhibit ultimate quantum properties and can serve as pure samples for testing quantum mechanics and performing precision measurements. The research described in this thesis investigates, both theoretically and experimentally, the coherence and dynamical evolution of a two-component Bose-Einstein condensate (BEC). The studies are performed on the |1 › ≡ F = 1,mF = −1 › and |2 › ≡ |F = 2,mF = +1 › hyperfine ground states of a 87Rb BEC trapped on an atom chip. Conventional understanding has been that the fringe contrast in interferometric experiments on a BEC is limited by the mean-field dephasing due to strong interatomic interactions which lead to inhomogeneous collisional shifts. We have discovered using Ramsey interferometry a mean-field driven self-rephasing effect in a trapped twocomponent BEC. When combined with a spin-echo technique, we find that the selfrephasing leads to a coherence time of 2.8 s, the longest ever recorded for an interacting BEC. Secondly, we have developed a new technique based on periodic collective oscillations for precision measurements of the interspecies and intraspecies scattering lengths and derived an analytic mean-field theory for the phase and density dynamics in the twocomponent BEC. This technique has been applied to the measurements of the scattering lengths for the two components, |1i and |2i, in 87Rb with a precision of 0.016%. Additionally, the two-body loss coefficients for these states have been measured. Thirdly, we have developed and applied a new, interferometric method for calibrating the detection system, in order to determine the total atom number precisely for Ramsey interferometric measurements. The calibration coefficient is found to be in a good agreement with that obtained using a conventional calibration technique based on the critical BEC temperature. Finally, we have detected predicted RF-induced Feshbach resonances by monitoring changes in the two-body loss coefficients in the two-component BEC. Conventional Feshbach resonances have been used in many works to tune the s-wave interactions; however, there is no achievable magnetic Feshbach resonance for magnetically trappable states of 87Rb. The RF-induced resonances which we have detected can provide a way to tune the scattering lengths which is important for interferometry and entanglement experiments. The positions of the resonances may provide useful information for predicting the atomic scattering properties of 87Rb.
In the years following the first Bose-Einstein condensation of dilute atomic gases in 1995, several experiments demonstrated many fundamental properties of two-component BEC. Subsequent to these pioneering experiments, almost a decade passed with little experimental activity, relative to investigations of single-component condensates. In somewhat of a renaissance, the initial observations of two-component BEC have been revisited in recent years, consolidating and clarifying results of the early works, and illuminating new and surprising behaviour of these rich quantum fluids. This thesis presents new experimental results on the relative phase evolution of two-component Bose-Einstein condensates (BECs). We approach our study of this system from the dual perspective of binary superfluidity and trapped atom interferometry. We observe nonequilibrium dynamics of the condensate that are deeply connected to the physics of interpenetrating superfluids. These dynamics have consequences for interferometers whose two paths are different internal spin states of the condensate atoms. Using trapped condensates for precision measurement draws upon the benefits of confined atom interferometry - long interrogation times, precise position control to measure near-field potentials - in addition to the unique coherence properties of BECs. Precision measurementwith trapped particles, however, is obstructed by the inherent inhomogeneities associated with the confinement itself. Spatial variation of the external potentials and atomic density can give rise to dephasing during the free evolution and imperfect splitting and recombination of the interferometric paths. In this thesis, we consider the dephasing of the two-componentmean field order parameter, which tends to diminish the interference signal attained with the condensate. The promise of fuhs for atom interferometry lies within using nonclassical many body states to reduce the fundamental noise limit imposed upon measuring the projection of atomic pseudospin. Before the many body quantum properties of two-component condensates can be used to their full potential, the ideal classical limit must be achieved and investigated. As in optical interferometry, the classical ideality of an interference measurement is contingent upon control of the spatialmodes - thematter wave fields, or single particle wave functions. Whilst much attention is currently focused on preparing nonclassical many body states for entanglement and squeezing of the condensate pseudospin, this thesis focuses on the ancillary yet important issue of spatial inhomogeneity of the condensate mean field. Reversal of the spatially inhomogeneous mean field evolution is demonstrated, employing the techniques of nuclear magnetic resonance. A new method is demonstrated to probe pseudospin -1/2 condensates involving microwave adiabatic passage. The technique permits simultaneous, spatially resolved absorption imaging of the spatial mode of each component. Controlled manipulation of the components into Zeeman states with different magnetic moments allows spatial separation using a Stern-Gerlach separation technique, providing a spatially resolved projection of the local condensate pseudospin from a single absorption image. We propose an interferometric technique which employs this imaging method to directly image the relative phase. The miscibility of the two components depends on the relative magnitude of the interactions between various collision partners. The boundary of this miscibility is found to be less pronounced than expected from the commonly applied results of homogeneous super-fluids.The effects of kinetic energy are shown to be significant at the threshold of miscibility, leading to a breakdown in the Thomas-Fermi approximation. Magnetic dipole transitions amongst alkali ground states are often used to prepare, manipulate, and interrogate pseudospin -1/2 condensates. We present a thorough investigation of the two-photonmagnetic dipole transitions between the |F = 1,mF = -1〉 and |F = 2,mF = +1〉 states, and the |F = 1,mF = +1〉 and |F = 2,mF = -1〉 states of 87Rb. Taking into account all 8 Zeeman levels of the electronic ground state reveals markedly different radiative shifts and effects beyond the rotating wave approximation, compared to the three-level formalism commonly used for these transitions.This has implications for Ramsey interferometry using the two-photon magnetic dipole transitions. The unchartered experimental territory offered by two-component condensates is vast, and future directions, supplementary to the work in this thesis, are elucidated.
Bose-Einstein condensates present to us the opportunity to probe into the atomic interac- tions that govern a macroscopic quantum mechanical system. The degenerate hyperfine manifold in the bosonic atoms splits in the presence of an external B-field; radio-frequency induced coupling releases experimentally-attainable knowledge about the Zeeman mani- fold in 87Rb. The purpose of this study is to investigate quantum dynamics in two and three-component Bose-Einstein condensate (BEC) systems. We start with a theoretical analysis of Josephson tunneling dynamics between identical BECs trapped in a double potential well, paying particular attention to the non-linear self-trapping effect observed as a consequence of the intra-well interaction. We present a model for the non-equilibrium dynamics in a two-level system and introduce the Rabi oscillations. This is followed by a numerical and experimental investigation of Rabi oscillations in a three-level 87Rb BEC between the F = 1 hyperfine level spin states mF = {1, 0, 1}. The relation between the observed total Rabi frequency and the detuning, along with its effect on the BEC population dynamics is explored. Finally, we explore the possible suspects for the shift of the resonance at strong Rabi frequencies .
We derive a nonequilibrium finite-temperature kinetic theory for a binary mixture of two interacting atomic Bose-Einstein condensates and use it to explore the degree of hydrodynamicity attainable in realistic experimental geometries. Based on the standard separation-of-time-scales argument of kinetic theory, the dynamics of the condensates of the multicomponent system are shown to be described by dissipative Gross-Pitaevskii equations self-consistently coupled to corresponding quantum Boltzmann equations for the noncondensate atoms: On top of the usual mean-field contributions, our scheme identifies a total of eight distinct collisional processes, whose dynamical interplay is expected to be responsible for the system's equilibration. In order to provide their first characterization, we perform a detailed numerical analysis of the role of trap frequency and geometry on collisional rates for experimentally accessible mixtures of $^{87}\mathrm{Rb}\ensuremath{-}^{41}\mathrm{K}$ and $^{87}\mathrm{Rb}\ensuremath{-}^{85}\mathrm{Rb}$, discussing the extent to which the system may approach the hydrodynamic regime with regard to some of those processes as a guide for future experimental investigations of ultracold Bose gas mixtures.