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arXiv:0704.1413 · Physical Review Letters

Preparation and Detection of Magnetic Quantum Phases in Optical Superlattices

Ana María Rey, Vladimir Gritsev, Immanuel Bloch, Eugene Demler, Mikhail D. Lukin

Published Oct 5, 2007• 43 citations
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Abstract

We describe a novel approach to prepare, detect, and characterize magnetic quantum phases in ultracold spinor atoms loaded in optical superlattices. Our technique makes use of singlet-triplet spin manipulations in an array of isolated double-well potentials in analogy to recently demonstrated control in quantum dots. We also discuss the many-body singlet-triplet spin dynamics arising from coherent coupling between nearest neighbor double wells and derive an effective description for such systems. We use it to study the generation of complex magnetic states by adiabatic and nonequilibrium dynamics.

DOI
10.1103/physrevlett.99.140601

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•Jan 1, 2012•1 citation
We describe a novel approach to prepare, detect, and characterize magnetic quantum phases in ultracold spinor atoms loaded in optical superlattices. Our technique makes use of singlet-triplet spin manipulations in an array of isolated double-well potentials in analogy to recently demonstrated control in quantum dots. We also discuss the many-body singlet-triplet spin dynamics arising from coherent coupling between nearest neighbor double wells and derive an effective description for such systems. We use it to study the generation of complex magnetic states by adiabatic and nonequilibrium dynamics.
We report on the controlled creation of a valence bond state of delocalized effective-spin singlet and triplet dimers by means of a bichromatic optical superlattice. We demonstrate a coherent coupling between the singlet and triplet states and show how the superlattice can be employed to measure the singlet-fraction employing a spin-blockade effect. Our method provides a reliable way to detect and control nearest-neighbor spin correlations in many-body systems of ultracold atoms. Being able to measure these correlations is an important ingredient in studying quantum magnetism in optical lattices. We furthermore employ a SWAP operation between atoms which are part of different triplets, thus effectively increasing their bond-length. Such a SWAP operation provides an important step towards the massively parallel creation of a multiparticle entangled state in the lattice.
We propose a method for controllable generation of nonlocal entangled pairs using spinor atoms loaded in an optical superlattice. Our scheme iteratively increases the distance between entangled atoms by controlling the coupling between the double wells. When implemented in a finite linear chain of 2N2N2N atoms, it creates a triplet valence bond state with large persistency of entanglement (of the order of NNN). We also study the nonequilibrium dynamics of the one-dimensional ferromagnetic Heisenberg Hamiltonian and show that the time evolution of a state of decoupled triplets on each double well leads to the formation of a highly entangled state where short-distance antiferromagnetic correlations coexist with longer-distance ferromagnetic ones. We present methods for detection and characterization of the various dynamically generated states. These ideas are a step forward toward the use of atoms trapped by light as quantum-information processors and quantum simulators.
We study how well magnetic models can be implemented with ultracold bosonic atoms of two different hyperfine states in an optical superlattice. The system is captured by a two-species Bose-Hubbard model, but realizes in a certain parameter regime actually the physics of a spin-1/2 Heisenberg magnet, describing the second-order hopping processes. Tuning of the superlattice allows for controlling the effect of fast first-order processes versus the slower second-order ones. Using the density-matrix renormalization-group method, we provide the evolution of typical experimentally available observables. The validity of the description via the Heisenberg model, depending on the parameters of the Hubbard model, is studied numerically and analytically. The analysis is also motivated by recent experiments [S. F\"olling et al., Nature (London) 448, 1029 (2007); S. Trotzky et al., Science 319, 295 (2008)] where coherent two-particle dynamics with ultracold bosonic atoms in isolated double wells were realized. We provide theoretical background for the next step, the observation of coherent many-particle dynamics after coupling the double wells. Contrary to the case of isolated double wells, relaxation of local observables can be observed. The tunability between the Bose-Hubbard model and the Heisenberg model in this setup could be used to study experimentally the differences in equilibration processes for nonintegrable and Bethe ansatz integrable models. We show that the relaxation in the Heisenberg model is connected to a phase averaging effect, which is in contrast to the typical scattering driven thermalization in nonintegrable models. We discuss the preparation of magnetic ground states by adiabatic tuning of the superlattice parameters.
We present a protocol to prepare decoherence-free cluster states using ultracold atoms loaded in a two dimensional superlattice. The superlattice geometry leads to an array of $2\ifmmode\times\else\texttimes\fi{}2$ plaquettes, each of them holding four spin-1∕21∕21∕2 particles that can be used for encoding a single logical qubit in the twofold singlet subspace, insensitive to uniform magnetic field fluctuations in any direction. Dynamical manipulation of the supperlattice yields distinct inter- and intraplaquette interactions and permits us to realize one qubit and two qubit gates with high fidelity, leading to the generation of universal cluster states for measurement based quantum computation. Our proposal based on inter- and intraplaquette interactions also opens the path to study polymerized Hamiltonians which support ground states describing arbitrary quantum circuits.
The exchange coupling between quantum mechanical spins lies at the origin of quantum magnetism. We report on the observation of nearest-neighbor magnetic spin correlations emerging in the many-body state of a thermalized Fermi gas in an optical lattice. The key to obtaining short-range magnetic order is a local redistribution of entropy within the lattice structure. This is achieved in a tunable-geometry optical lattice, which also enables the detection of the magnetic correlations. We load a low-temperature two-component Fermi gas with repulsive interactions into either a dimerized or an anisotropic simple cubic lattice. For both systems the correlations manifest as an excess number of singlets as compared to triplets consisting of two atoms with opposite spins. For the anisotropic lattice, we determine the transverse spin correlator from the singlet-triplet imbalance and observe antiferromagnetic correlations along one spatial axis. Our work paves the way for addressing open problems in quantum magnetism using ultracold fermions in optical lattices as quantum simulators.
In this thesis we study various aspects of spinor Bose-Einstein condensates in optical superlattices using a Bose-Hubbard Hamiltonian that takes spin effects into account. We decouple the unit cells of the superlattice via a mean-field approach and take into account the dynamics within the unit cell exactly. In this way we derive the ground-state phase diagram of spinor bosons in superlattices. The system supports Mott-insulating as well as superfluid phases. The transitions between these phases are second-order for spinless bosons and second- or first-order for spin-1 bosons. Antiferromagnetic interactions energetically penalize high-spin configurations and elongate all Mott lobes, especially the ones corresponding to an even atom number on each lattice site. We find that the quadratic Zeeman effect lifts the degeneracy between different polar superfluid phases leading to additional metastable phases and first-order phase transitions. A change of magnetic fields can drive quantum phase transitions in the same way as a change in the tunneling amplitude does. Furthermore we study the physics of spin-1 atoms in superlattices deep in the Mott insulating phase when the superlattice decomposes into isolated double-well potentials. Assuming that a small number of spin-1 bosons is loaded in an optical double-well potential, we study single-particle tunneling that occurs when one lattice site is ramped up relative to a neighboring site. Spin-dependent effects modify the tunneling events in a qualitative and quantitative way. Depending on the asymmetry of the double well different types of magnetic order occur, making the system of spin-1 bosons in an optical superlattice a model for mesoscopic magnetism with an unprecedented control of the parameters. Homogeneous and inhomogeneous magnetic fields are applied and the effects of the linear and the quadratic Zeeman shifts are examined. We generalize the concept of bosonic staircases to connected double-well potentials. We show that an energy offset between the two sites of the unit cell in an extended superlattice induces a staircase of single-atom resonances in \nthe same way as in isolated double well. We also examine single-atom resonances in the superfluid regime and find clear fingerprints of them in the superfluid density. We also investigate the bipartite entanglement between the sites and construct states of maximal entanglement. The entanglement in our system is due to both orbital and spin degrees of freedom. We calculate the contribution of orbital and \nspin entanglement and show that the sum of these two terms gives a lower bound for the total entanglement.